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Thermally excited capillary waves at fluid interfaces in binary liquid mixtures exhibit simultaneously both density and composition fluctuations. Based on a density functional theory for inhomogeneous binary liquid mixtures we derive an…

Soft Condensed Matter · Physics 2009-11-11 Thorsten Hiester , S. Dietrich , Klaus Mecke

We study a two-dimensional fluid of particles interacting through a spherically-symmetric and marginally soft two-body repulsion. This model can exist in three different crystal phases, one of them with square symmetry and the other two…

Soft Condensed Matter · Physics 2012-09-13 Santi Prestipino , Franz Saija , Paolo V. Giaquinta

We consider homogeneous crystallisation rates in confocal microscopy experiments on colloidal nearly hard spheres at the single particle level. These we compare with Brownian dynamics simuations by carefully modelling the softness in the…

Soft Condensed Matter · Physics 2017-12-27 Jade Taffs , Stephen R. Williams , Hajime Tanaka , C. Patrick Royall

Experiments and computer simulations have established that liquid water's surfaces can deviate in important ways from familiar bulk behavior. Even in the simplest case of an air-water interface, distinctive layering, orientational biases,…

Soft Condensed Matter · Physics 2022-07-15 Nathan L. Odendahl , Phillip L. Geissler

In this work we examine thermodynamics of fluid with "molecules" represented by two fused hard spheres, decorated by the attractive square-well sites. Interactions between these sites are of short-range and cause association between the…

Soft Condensed Matter · Physics 2016-03-24 M. Kastelic , Yu. V. Kalyuzhnyi , V. Vlachy

The dynamics of sharp interfaces separating two non-hydrostatically stressed solids is analyzed using the idea that the rate of mass transport across the interface is proportional to the thermodynamic potential difference across the…

Materials Science · Physics 2009-11-13 Luiza Angheluta , Espen Jettestuen , Joachim Mathiesen

The theory of interfacial properties in liquid-liquid or liquid-vapour systems is nearly 200 years old. The advent of computational tools has greatly advanced the field, mainly through the use of Molecular Dynamics simulations. Despite the…

Soft matters whose constituents are deformable are ubiquitous in nature especially in biological systems-including cells and their organelles-as well as in foams and emulsions. The capacity for deformation in these soft materials gives rise…

Soft Condensed Matter · Physics 2026-03-05 Padmanabha Bose , Smarajit Karmakar

In this work, we perform a systematic computer simulation study of ice premelting, and explore the thickness and structure of quasi-liquid layers formed at the interface of ice with substrates of different hydrophilicity. Our study shows…

Soft Condensed Matter · Physics 2024-10-30 Łukasz Baran , Pablo Llombart , Luis G. MacDowell

We use replica exchange Monte-Carlo simulations to measure the equilibrium equation of state of the disordered fluid state for a binary hard sphere mixture up to very large densities where standard Monte-Carlo simulations do not easily…

Statistical Mechanics · Physics 2011-02-04 Gerardo Odriozola , Ludovic Berthier

The efficiency of soft particles to stabilize emulsions is examined by measuring their desorption free energy, i.e., the mechanical work required to detach the particle from a fluid interface. Here, we consider rubber-like elastic as well…

Soft Condensed Matter · Physics 2020-08-20 Hadi Mehrabian , Jacco H. Snoeijer , Jens Harting

We investigate the formation of cluster crystals with multiply occupied lattice sites on a spherical surface in systems of ultra-soft particles interacting via repulsive, bounded pair potentials. Not all interactions of this kind lead to…

Soft Condensed Matter · Physics 2018-07-31 Stefano Franzini , Luciano Reatto , Davide Pini

Interfacial fluctuations in a two-phase binary fluid mixture reveal signatures of underlying physical processes that occur within each phase and on a range of spatial and temporal scales. In this study, we investigate a model binary fluid…

Fluid Dynamics · Physics 2026-03-04 Samuel Z Khiangte , Triparna Sanyal , Sumantra Sarkar , Nairita Pal

Effects of scale coupling between mesoscopic slowly-varying envelopes of liquid-solid profile and the underlying microscopic crystalline structure are studied in the phase-field-crystal (PFC) model. Such scale coupling leads to nonadiabatic…

Materials Science · Physics 2015-06-12 Zhi-Feng Huang

Recent studies of melting in hard disks have confirmed the existence of a hexatic phase occurring in a narrow window of density which is separated from the isotropic liquid phase by a first-order transition, and from the solid phase by a…

Statistical Mechanics · Physics 2017-09-20 John Russo , Nigel B. Wilding

Compared to pure fluids, binary mixtures display a very diverse phase behavior, which depends sensitively on the parameters of the microscopic potential. Here we investigate the phase diagrams of simple model mixtures by use of a…

Soft Condensed Matter · Physics 2009-11-07 A. Parola , D. Pini , L. Reatto , M. Tau

Using molecular dynamics simulation, we investigate the slow dynamics of a supercooled binary mixture of soft particles interacting with a generalized Hertzian potential. At low density, it displays typical slow dynamics near its glass…

Soft Condensed Matter · Physics 2016-10-18 Ryoji Miyazaki , Takeshi Kawasaki , Kunimasa Miyazaki

The interface formation model is applied to describe the initial stages of the coalescence of two liquid drops in the presence of a viscous ambient fluid whose dynamics is fully accounted for. Our focus is on understanding (a) how this…

Fluid Dynamics · Physics 2015-06-22 James E. Sprittles , Yulii D. Shikhmurzaev

Liquid crystals in two dimensions undergo a first-order isotropic-to-quasi-nematic transition, provided the particle interactions are sufficiently ``sharp and narrow''. This implies phase coexistence between isotropic and quasi-nematic…

Statistical Mechanics · Physics 2009-11-13 R. L. C. Vink

The wetting dynamics of liquid particles, from coated droplets to soft capsules, holds significant technological interest. Motivated by the need to simulate liquid metal droplet with an oxidize surface layer, in this work we introduce a…

Fluid Dynamics · Physics 2024-02-14 Francesca Pelusi , Fabio Guglietta , Marcello Sega , Othmane Aouane , Jens Harting