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We study theoretically the two-center interferences occurring in high harmonic generation from diatomic molecules. By solving the time-dependent Schroedinger equation, either numerically or with the molecular strong-field approximation, we…

The generation of high harmonics in laser-irradiated light homonuclear diatomics (H2+, N2 and O2) compared to that in atomic counterparts (of nearly identical binding energy) is studied within the velocity gauge version of conventional…

Atomic Physics · Physics 2009-11-11 Vladimir I. Usachenko , Pavel E. Pyak , Shih-I Chu

This Letter brings together two topics that, until now, have been the focus of intense but non-overlapping research efforts. The first concerns high harmonic generation in solids, which occurs when intense light field excites highly…

Strongly Correlated Electrons · Physics 2022-04-06 R. E. F. Silva , Igor V. Blinov , Alexey N. Rubtsov , O. Smirnova , M. Ivanov

Using a high-frequency field superposed to a linearly polarized bichromatic laser field composed by a wave with frequency $\omega $ and a wave with frequency $2\omega $, we show it is possible to enhance the intensity of a group of high…

Atomic Physics · Physics 2009-11-06 C. Figueira de Morisson Faria , M. L. Du

We present a theoretical model of high-harmonic generation from diatomic molecules. The theory includes effects of alignment as well as nuclear motion and is used to predict results for N$_2$, O$_2$, H$_2$ and D$_2$. The results show that…

Atomic Physics · Physics 2007-05-23 Christian Bruun Madsen , Lars Bojer Madsen

By employing the exact diagonalization method, we investigate the high-harmonic generation (HHG) of the correlated systems under the strong laser irradiation. For the extended Hubbard model on a periodic chain, HHG close to the quantum…

Strongly Correlated Electrons · Physics 2022-03-07 Can Shao , Hantao Lu , Xiao Zhang , Chao Yu , Takami Tohyama , Ruifeng Lu

The optical phase of the driving field in the process of high harmonic generation and the coherence properties of the harmonics are fundamental concepts in attosecond physics. Here, we consider to drive the process by incoherent classical…

Quantum Physics · Physics 2024-09-16 Philipp Stammer

Using one-dimensional simulations analyzed through the lens of open quantum systems, we study the photoelectron's strong-field dynamics from an atom surrounded by a scattering environment stochastically structured. We theoretically…

Quantum Physics · Physics 2026-05-21 Simon His , Camille Lévêque , Jérémie Caillat , Richard Taïeb , Jonathan Dubois

We present a study of the possibility to significantly enhance the efficiency of high-order harmonic generation (HHG) using few-cycle optical waveforms obtained by superposing two laser pulses of different color delayed optimally relative…

Optics · Physics 2024-12-11 O. V. Meshkov , M. Yu. Emelin , M. Yu. Ryabikin

High harmonic generation in solids is becoming an important method for strong field solid state physics research. The power scale relationship between high harmonics and the driving laser is investigated both experimentally and…

Optics · Physics 2022-08-23 Shuai Wang , Xinkui He , Yueying Liang , Yabei Su , Shaobo Fang , Zhiyi Wei

Fully quantum treatment explicitly presents the high harmonic generation as a three-step process: (i) above threshold ionization (ATI) is followed by (ii) electron propagation in a laser-dressed continuum. Subsequently (iii) stimulated (or…

Atomic Physics · Physics 2009-10-31 M. Yu. Kuchiev , V. N. Ostrovsky

High-harmonic generation is typically thought of as a sub-laser-cycle process, with the electron's excursion in the continuum lasting a fraction of the optical cycle. However, it was recently suggested that long-lived Rydberg states can…

We theoretically study high-harmonic generation (HHG) from solids driven by intense laser pulses using a one-dimensional model periodic crystal. By numerically solving the time-dependent Schr\"{o}dinger equation directly on a real-space…

We utilize few-level model systems to analyze the polarization and phase properties of below-threshold harmonics generated from aligned molecules. In a two-level system, we find that the phase of emitted harmonics undergoes a distinct…

Quantum Physics · Physics 2026-05-06 Samuel Schöpa , Falk-Erik Wiechmann , Franziska Fennel , Dieter Bauer

The bi-circular scheme for high harmonic generation, which combines two counter-rotating circular fields with frequency ratio 2:1, has recently permitted to generate high harmonics with essentially circular polarization, opening the way for…

We study theoretically and experimentally High Harmonic Generation (HHG) using two non collinear driving fields focused in gases. We show that these two fields form a non stationary blazed active grating in the generation medium. The…

Optics · Physics 2019-03-13 C. Chappuis , D. Bresteau , T. Auguste , O. Gobert , T. Ruchon

Harmonic generation by an atom in a laser field is described by the three-step mechanism as proceeding via above-threshold ionization (ATI) followed by the electron propagation in the laser-dressed continuum and the subsequent laser…

Atomic Physics · Physics 2009-11-06 M. Yu. Kuchiev , V. N. Ostrovsky

We present studies of high-order harmonic generation (HHG) at laser intensities well above saturation. We use driving laser pulses which present a particular electron dynamics in the turn-on stage. Our results predict an increasing on the…

Atomic Physics · Physics 2015-06-19 J. A. Pérez-Hernández , M. F. Ciappina , M. Lewenstein , A. Zaïr , L. Roso

The cut-off regime of high-order harmonic generation (HHG) by atoms in an intense laser field is studied numerically and analytically. We find that the cut-off regime is characterized by equal dephasing between the successive harmonics. The…

Atomic Physics · Physics 2016-04-27 M. A. Khokhlova , V. V. Strelkov

High-order harmonic generation (HHG) from aligned acetylene molecules interacting with mid infra-red (IR), linearly polarized laser pulses is studied theoretically using a mixed quantum-classical approach in which the electrons are…

Atomic Physics · Physics 2018-05-18 Peter Mulholland , Daniel Dundas