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Standard optical pump-probe methods analyze a system's temporal response to a laser pulse within sub-femtoseconds to several nanoseconds, constrained by the optical delay line's length. While resistance is a sensitive detector in various…

Instrumentation and Detectors · Physics 2024-04-26 M. I. Blumenau , A. Yu. Kuntsevich

Soliton self-compression is demonstrated during the propagation of high spatial modes in hollow core fibers in the near-infrared spectral region, taking advantage of their negative dispersion response. We have found that there is always an…

Mid-infrared hyperspectral imaging has become an indispensable tool to spatially resolve chemical information in a wide variety of samples. However, acquiring three-dimensional data cubes is typically time-consuming due to the limited speed…

Optics · Physics 2026-05-29 Jianan Fang , Kun Huang , Ruiyang Qin , Yan Liang , E Wu , Ming Yan , Heping Zeng

We report on the spatially resolved full amplitude and phase characterization of mid-infrared high intensity laser pulses generated in a three stage OPA. We use a spatially-encoded arrangement (SEA-)SPIDER with spectral filters for ancilla…

Supercontinuum (SC) generation based on ultrashort pulse compression constitutes one of the most promising technologies towards an ultra-wide bandwidth, high-brightness and spatially coherent light sources for applications such as…

The infrared beamline at BESSY II storage ring was upgraded recently to extend capabilities of infrared microscopy. The end-stations available at the beamline are now facilitating improved characterization of molecules and materials at…

Optics · Physics 2024-05-09 Alexander Veber , Ljiljana Puskar , Janina Kneipp , Ulrich Schade

Each successive generation of x-ray machines has opened up new frontiers in science, such as the first radiographs and the determination of the structure of DNA. State-of-the-art x-ray sources can now produce coherent high brightness keV…

Infrared (IR) spectroscopy, a well established tool for chemical analysis of diverse materials, has significant potential in biomedical applications. While the spatial resolution of traditional IR spectroscopy is limited by the wavelength…

Periodically poled thin film lithium niobate waveguides provide simultaneous access to efficient second and third order nonlinear processes, enabling broadband generation of coherent laser light. Here, we demonstrate the generation of a…

Ultrafast laser pump-probe spectroscopy is an important and growing field of physical chemistry that allows the measurement of chemical dynamics on their natural timescales, but undergraduate laboratory courses lack examples of such…

Physics Education · Physics 2023-07-25 Ilana J Porter , Michael W. Zuerch , Anne M. Baranger , Stephen R. Leone

Singly ionized nitrogen molecules in ambient air pumped by near-infrared femtosecond laser give rise to superradiant emission. Here we demonstrate coherent control of this superradiance by injecting a pair of resonant seeding pulses inside…

Laser pulses in the near-infrared spectral range with a high repetition rate and high pulse energy offer the possibility to perform strong-field experiments such as high-order harmonic generation in gases or strong-field photoemission from…

Nanophotonic waveguides with sub-wavelength mode confinement and engineered dispersion profiles are an excellent platform for application-tailored nonlinear optical interactions at low pulse energies. Here, we present fully air clad…

We present a method for acquiring a sequence of time-resolved images in a single shot, called Single-Shot Non-Synchronous Array Photography (SNAP). In SNAP, a pulsed laser beam is split by a diffractive optical element into an array of…

Broadband mid-infrared (MIR) molecular spectroscopy demands a bright and broadband light source in the molecular fingerprint region. To this end, intra-pulse difference frequency generation (IDFG) has shown excellent properties among…

We experimentally demonstrate in a difference-frequency generation mid-infrared frequency comb source the effect of temporal overlap between pump- and signal- pulse to the relative intensity noise (RIN) of the idler pulse. When scanning the…

Generating energetic femtosecond mid-IR pulses is crucial for ultrafast spectroscopy, and currently relies on parametric processes that, while efficient, are also complex. Here we experimentally show a simple alternative that uses a single…

Optics · Physics 2015-04-10 B. B. Zhou , H. R. Guo , M. Bache

We extend the technique of multiplex coherent Raman spectroscopy with two femtosecond mode-locked lasers to oscillators of a pulse repetition frequency of 1 GHz. We demonstrate spectra of liquids, which span 1100 cm$^{-1}$ of Raman shifts.…

Characterizing and controlling electronic properties of quantum materials require direct measurements of non-equilibrium electronic band structures over large regions of momentum space. Here, we demonstrate an experimental apparatus for…

Single-photon detectors (SPDs) at near infrared wavelengths with high system detection efficiency (> 90%), low dark count rate (< 1 counts per second, cps), low timing jitter (< 100 ps), and short reset time (< 100 ns) would enable landmark…

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