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Electromagnetic radiation in the mid- to far-infrared spectral range represents an indispensable tool for the study of numerous types of collective excitations in solids and molecules. Short and intense pulses in this THz spectral range…

Mesoscale and Nanoscale Physics · Physics 2022-05-03 T. Janssen , C. S. Davies , M. Gidding , V. Chernyy , J. M. Bakker , A. Kirilyuk

We describe an ultrafast time resolved pump-probe spectroscopy setup aimed at studying the switching of nanophotonic structures. Both fs pump and probe pulses can be independently tuned over broad frequency range between 3850 and 21050…

Optics · Physics 2010-11-02 Tijmen G. Euser , Philip J. Harding , Willem L. Vos

Tunable mid-infrared lasers are essential for optical sensing and imaging. Existing technologies, however, face challenges in simultaneously achieving broadband spectral tunability and ultra-rapid scan rates, limiting their utility in…

Optics · Physics 2025-01-20 Xiaoshuai Ma , Tianjian Lv , Xudong Zhu , Ming Yan , Heping Zeng

Synchrotron radiation light sources produce intense beam of X-ray with ultra-short pulse and nanosecond period. This of-fers the opportunities for the time resolution experiments. Achieving higher counting rate and faster arriving time is…

Instrumentation and Detectors · Physics 2015-11-05 Zhen-jie Li , Qiu-ju Li , Peng Liu , Shan-feng Wang , Wei-wei Dong , Yang-fan Zhou

Super-resolution microscopy in the visible is an established powerful tool in several disciplines. In the infrared (IR) spectral range, however, no comparable schemes have been demonstrated to date. In this work, we experimentally…

We combine different wavelengths from an intense high-order harmonics source with variable delay at the focus of a split-mirror interferometer to conduct pump-probe experiments on gas-phase molecules. We report measurements of the time…

Chemical Physics · Physics 2015-05-27 T. K. Allison , T. W. Wright , A. M. Stooke , C. Khurmi , J. van Tilborg , Y. Liu , R. W. Falcone , A. Belkacem

The paper describes a time- and angle-resolved photoemission apparatus consisting of a hemispherical analyzer and a pulsed laser source. We demonstrate 1.48-eV pump and 5.90-eV probe measurements at the >10.5-meV and >240-fs resolutions by…

Materials Science · Physics 2016-12-16 Y. Ishida , T. Togashi , K. Yamamoto , M. Tanaka , T. Kiss , T. Otsu , Y. Kobayashi , S. Shin

We describe a setup for time- and angle-resolved photoemission spectroscopy with wavelength-tunable excitation and extreme ultraviolet probe. It is enabled by using the 10 kHz twin Ti:sapphire amplifiers seeded by the common Ti:sapphire…

Materials Science · Physics 2025-02-11 Takeshi Suzuki , Yigui Zhong , Kecheng Liu , Teruto Kanai , Jiro Itatani , Kozo Okazaki

Synchrotrons are powerful and productive in revealing the spatiotemporal complexities in matter. However, X-ray pulses produced by the synchrotrons are predetermined in specific patterns and widths, limiting their operational flexibility…

Accelerator Physics · Physics 2022-11-08 Jian Zhou , Jinxing Jiang , Donald A. Walko , Dafei Jin , Daniel López , David A. Czaplewski , Jin Wang

While mid-infrared radiation can be used to identify and quantify numerous chemical species, contemporary broadband mid-IR spectroscopic systems are often hindered by large footprints, moving parts and high power consumption. In this work,…

Strong-field mid-infrared pump--terahertz (THz) probe spectroscopy has been proven as a powerful tool for light control of different orders in strongly correlated materials. We report the construction of an ultrafast broadband infrared…

Instrumentation and Detectors · Physics 2017-10-10 S. J. Zhang , Z. X. Wang , T. Dong , N. L. Wang

Microcavity-based microlasers are the kernel light sources for integrating photonics and optoelectronics. The traditional pump light frequency locking mainly utilizes a complex system with optoelectronic feedback, which requires a high-cost…

We report a singly resonant continuous-wave optical parametric oscillator (SRO), which is pumped by a semiconductor laser system and operates in the mid-infrared region (2.9 to 3.6 {\mu}m). Fast tuning of the mid-infrared output wavelength…

Optics · Physics 2018-07-06 Ville Ulvila , Markku Vainio

Spectral imaging in the mid-infrared (MIR) range provides simultaneous morphological and chemical information of a wide variety of samples. However, current MIR technologies struggle to produce high-definition images over a broad spectral…

Supercontinua generated in highly non-linear fibers by ultrashort-pulse lasers can be used for high resolution Fourier transform absorption spectroscopy. The practical advantages of these bright ultrabroadband light sources for spectroscopy…

High resolution and fast detection of molecular vibrational absorption is important for organic synthesis, pharmaceutical process and environmental monitoring, and is enabled by mid-infrared (mid-IR) laser frequency combs via dual-comb…

Intense ultrashort pulse lasers are used for fs resolution pumpprobe experiments more and more at large scale facilities, such as free electron lasers (FEL). Measurement of the arrival time of the laser pulses and stabilization to the…

Instrumentation and Detectors · Physics 2023-07-19 Marta Csatari Divall , Patrick Mutter , Edwin J. Divall , Christoph P. Hauri

Near-infrared (NIR) hyperspectral imaging is widely used to reveal morphological and chemical information. However, conventional spectral imagers usually rely on costly focal plane arrays and suffer from data redundancy and inefficiencies…

Optics · Physics 2026-05-26 Ben Sun , Kun Huang , Zhibin Zhao , Beibei Dong , Jianan Fang , Heping Zeng

Ultrafast lasers ($< 500$ fs) have enabled laser-matter interactions at intensities exceeding $10^{18} \rm{Wcm}^{-2}$ with only millijoules of laser energy. However, as pulse durations become shorter, larger spectral bandwidths are…

The availability of intense, ultrashort coherent radiation sources in the infrared region of the spectrum is enabling the generation of attosecond X-ray pulses via high harmonic generation, pump-probe experiments in the "molecular…