Related papers: Harmonic generation in ring-shaped molecules
The physics of intense laser-matter interactions is described by treating the light pulses classically, anticipating no need to access optical measurements beyond the classical limit. However, the quantum nature of the electromagnetic…
Two different induced effects of a laser falling edge on high-order harmonic generation are resolved by solving numerically full-dimensional electronic time-dependent Schr\"{o}dinger equation beyond the Born-Oppenheimer approximation. The…
Energy-angular distributions of electron-positron pair creation in collisions of a laser beam and a nonlaser photon are calculated using the $S$-matrix formalism. The laser field is modeled as a finite pulse, similar to the formulation…
We study numerically the Bloch electron wave-packet dynamics in periodic potentials to simulate laser-solid interactions. We introduce a quasi-classical model in the \emph{k} space combined with the energy band structure to understand the…
Vector beams with spatially structured polarization and intertwined spin-orbital angular momentum (SAM-OAM) provide powerful degrees of freedom for tailoring light-matter interactions. While such structured beams are well established in the…
Based on high-order harmonic generation (HHG) spectra obtained from solving the time-dependent Schrodinger equation for atoms, we established quantitatively that the HHG yield can be expressed as the product of a returning electron wave…
High order harmonic generation by extremely intense, interacting, electromagnetic waves in the quantum vacuum is investigated within the framework of the Heisenberg-Euler formalism. Two intersecting plane waves of finite duration are…
In strong field laser physics it is a common practice to use the high-order harmonic cutoff to estimate the laser intensity of the pulse that generates the harmonic radiation. Based on the semiclassical arguments it is possible to find a…
High harmonic generation is a convenient way to obtain extreme ultraviolet light from table-top laser systems and the experimental tools to exploit this simple and powerful light source for time-resolved spectroscopy are being developed by…
Although the frequency shift and odd-even intensity modulation in high-order harmonic generation (HHG) have both been observed for asymmetric laser-target systems, they are typically studied as two separate phenomena. In this Letter, we…
We theoretically investigate high-harmonic generation in hexagonal boron nitride with linearly polarized laser pulses. We show that imperfect recollisions between electron-hole pairs in the crystal give rise to an electron-hole-pair…
A thin layer of overdense plasma is created when an electromagnetic pulse interacts with a rapidly ionizing thin foil. This layer will reflect the incoming pulse, forming a so-called plasma mirror. A simple realistic model based on paired…
Non Born-Oppenheimer quantum dynamics of H$_{2}^{+}$ excited by shaped one-cycle laser pulses linearly polarized along the molecular axis have been studied by the numerical solution of the time-dependent Schr\"odinger equation within a…
We present a new theory that the molecular high order harmonic generation in an intense laser field is determined by molecular internal symmetry and momentum distribution of the tunneling-ionized electron. The molecular internal symmetry…
A study of the Mode-locking lasing pulse formation in closed cavities is presented within a statistical mechanical framework where the onset of laser coincides with a thermodynamic phase transition driven by the optical power pumped into…
In this Letter, it is experimentally and theoretically shown that weak odd harmonics generated during the propagation of an infrared ultrashort ultra-intense pulse unexpectedly modify the nonlinear properties of the medium and lead to a…
A thin and dense plasma layer is created when a sufficiently strong laser pulse impinges on a solid target. The nonlinearity introduced by the time-dependent electron density leads to the generation of harmonics. The pulse duration of the…
Effects of the laser pulse wavelength and intensity on the HHG production from the \textit{ionic} and \textit{homolytic} pre-ionization transient states of the two-electron H$_{2}$ system exposed to ultrashort intense laser pulses are…
We show that the Floquet approach with a Sturmian basis means an efficient description of high-order harmonic generation with monochromatic excitation. This method, although involves numerical calculations, is close to analytic approaches…
Using a quantum mechanical three-step model we present numerical calculations on the high-harmonic generation from four polyatomic molecules. Ethylene (C$_2$H$_4$) serves as an example where orbital symmetry directly affects the harmonic…