Related papers: A numerical ab initio study of harmonic generation…
In this work the extreme nonlinear optical response of a giant fullerene molecule C$_{240}$ in strong laser field is studied. The investigation of high-order harmonic generation in such quantum nanostructure is presented modeling the…
We theoretically investigate high-order harmonic generation (HHG) in Rydberg atoms driven by spatially inhomogeneous laser fields, induced, for instance, by plasmonic enhancement. It is well known that the laser intensity should to exceed…
Thermotropic liquid crystals are versatile optical materials that exhibit a state of matter intermediate between liquids and solids. Their properties can change significantly with temperature, pressure, or other external factors, leading to…
The present work reports on the generation of short-pulse coherent extreme ultraviolet radiation of controlled polarization. The proposed strategy is based on high-order harmonics generated in pre-aligned molecules. Field-free molecular…
Using Time-Dependent Density Functional Theory (TDDFT) nonlinear nonperturbative response of the molecular system is studied for photoisomerization reaction. The 1,3-cyclohexadiene photoisomerization is probed by the high-harmonic…
The random laser action with coherent feedback by second-harmonic generation (SHG) was experimentally demonstrated in this paper. Compared with the conventional random laser action based on photoluminescence effect, which needs strong…
High-harmonic generation is a light up-conversion process occurring in a strong laser field, leading to coherent bursts of extreme ultrashort broadband radiation [1]. As a new perspective, we propose that ultrafast strong-field electronic…
Recent reports on intense-field pump-probe experiments for high harmonic generation from coherently rotating linear molecules, have revealed remarkable characteristic effects of the simultaneous variation of the polarization geometry and…
We theoretically study high-harmonic generation (HHG) from solids driven by intense laser pulses using a one-dimensional model periodic crystal. By numerically solving the time-dependent Schr\"{o}dinger equation directly on a real-space…
Two different induced effects of a laser falling edge on high-order harmonic generation are resolved by solving numerically full-dimensional electronic time-dependent Schr\"{o}dinger equation beyond the Born-Oppenheimer approximation. The…
High-harmonic generation (HHG) in liquids is opening new opportunities for attosecond light sources and attosecond time-resolved studies of dynamics in the liquid phase. In gas-phase HHG, few-cycle pulses are routinely used to create…
The long standing issue of separating resonant from non-resonant processes in extreme nonlinear optics is resolved. The theoretical formalism is applied to high harmonic generation (HHG) in solids and reveals a deeper view into the dominant…
We observe the generation of high harmonics in the plane perpendicular to the driving laser polarization and show that these are driven by the spin-orbit interaction. Using R-Matrix with time-dependence theory, we demonstrate that for…
In this report, a novel methodology based on the static coherent states approach is introduced with the capability of calculating various strong-field laser-induced nonlinearities in full dimensional single-electron molecular systems; an…
We produce oriented rotational wave packets in CO and measure their characteristics via high harmonic generation. The wavepacket is created using an intense, femtosecond laser pulse and its second harmonic. A delayed 800 nm pulse probes the…
The growing requirements of pump-probe techniques and nonlinear optics experiments greatly promote the studies of two-color free-electron lasers (FELs). We propose a new method to generate coherent two-color pulses in a high-gain harmonic…
The harmonic generation has always been of fundamental interest in studying the nonlinear nature of any physical system. In the present study, Particle - In - Cell (PIC) simulations have been carried out to explore the harmonic generation…
We study the effect of gas pressure on the generation of high-order harmonics where harmonics due to individual atoms are calculated using the recently developed quantitative rescattering theory, and the propagation of the laser and…
A three step model for high harmonic generation from impurities in solids is developed. The process is found to be similar to high harmonic generation in atomic and molecular gases with the main difference coming from the non-parabolic…
We investigate the electron quantum path interference effects during high harmonic generation in atomic gas medium driven by ultrashort chirped laser pulses. To achieve that, we identify and vary the different experimentally relevant…