Related papers: Nonlinear, ground-state, pump-probe spectroscopy
A theory of pump-probe spectroscopy is developed in which optical fields drive two-photon Raman transitions between ground states of an ensemble of three-level $\Lambda $ atoms. Effects related to the recoil the atoms undergo as a result of…
We report on cw measurements of probe beam absorption and four-wave-mixing spectra in a $^{85}$Rb magneto-optical trap taken while the trap is in operation. The trapping beams are used as pump light. We concentrate on the central feature of…
We investigate a singly-charged quantum dot under a strong optical driving field by probing the system with a weak optical field. When the driving field is detuned from the trion transition, the probe absorption spectrum is shifted from the…
We consider the quantum field theory for a scalar model of the electromagnetic field interacting with a system of two-level atoms. In this setting, we show that it is possible to uniquely determine the density of atoms from measurements of…
Quantum spectroscopy seeks to probe chemical systems using nonclassical light, which has properties that are qualitatively and quantitatively different than conventional light sources. One promising technique uses intensity-correlated twin…
Optical signals obtained by the material response to classical laser fields are given by nonlinear response functions which can be expressed by sums over various quantum pathways of matter. We show that some pathways can be selected by…
The classical or quantum nature of optical spectroscopy signals is a topic that has attracted great attention recently. Spectroscopic techniques have been classified as quantum or classical depending on the light-source used in their…
Traditionally, spectroscopy is performed by examining the position of absorption lines. However, at frequencies near the transition frequency, additional information can be obtained from the phase shift. In this work we consider the…
We experimentally study the absorption spectroscopy from a collection of gaseous $^87 Rb$ atoms at room temperature irradiated with three fields. Two of these fields are in a pump probe saturation absorption configuration. The third field…
A cascade of two-level superconducting artificial atoms -- a source and a probe -- strongly coupled to a semi-infinite waveguide is a promising tool for observing nontrivial phenomena in quantum nonlinear optics. The probe atom can scatter…
Nonlinear optics experiments measuring phase shifts induced in a weak probe pulse by a strong pump pulse must account for coherent effects that only occur when the pump and probe pulses are temporally overlapped. It is well known that a…
A nonlinear planar waveguide pumped by a beam orthogonal to its surface may serve as a versatile source of photon pairs. Changing pump-pulse duration, pump-beam transverse width, and angular decomposition of pump-beam frequencies…
We present a novel quantum phenomenon named electromagnetically induced entanglement in the conventional Lambda-type three-level atomic system driven by a strong pump field and a relatively weak probe field. Nearly perfect entanglement…
The Raman gain of a probe light in a three-state $\Lambda $-scheme placed into a defect of a one-dimensional photonic crystal is studied theoretically. We show that there exists a pump intensity range, where the transmission and reflection…
A theory of optical emission of quantum dot arrays in quantum microcavities is developed. The regime of the strong coupling between the quantum dots and photonic mode of the cavity is considered. The quantum dots are modeled as two-level…
We consider nonlinear spectroscopic effects - interaction-enhanced double resonance and spectrum instability - that appear in ultracold quantum gases owing to collisional frequency shift of atomic transitions and, consequently, due to the…
Coherence phenomena in four-level atomic system, cyclicly driven by three coherent fields, are investigated thoroughly at zero and weak magnetic fields. Each strongly interacting atomic state is converted to a triplet due to a dynamical…
Optical pump-probe spectroscopy is a powerful tool for the study of non-equilibrium electronic dynamics and finds wide applications across a range of fields, from physics and chemistry to material science and biology. However, a shortcoming…
Nonlinear spectroscopy with quantum entangled photons is an emerging field of research that holds the promise to achieve a superior signal-to-noise ratio and effectively isolate many-body interactions. Photon sources used for this purpose…
In virtual-state spectroscopy, information about the energy-level structure of an arbitrary sample is retrieved by Fourier transforming sets of measured two-photon absorption probabilities of entangled photon pairs where the degree of…