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Photo-induced phase-transitions (PIPTs) driven by highly cooperative interactions are of fundamental interest as they offer a way to tune and control material properties on ultrafast timescales. Due to strong correlations and interactions,…

Materials Science · Physics 2022-11-03 Sangeeta Rajpurohit , Jacopo Simoni , Liang Z. Tan

A theory of electrical transport through molecular wires is used to estimate the electronic factor in the intramolecular electron transfer (ET) in porphyrin-nitrobenzene supermolecules, and to analyze its structure. The chosen molecules…

Soft Condensed Matter · Physics 2007-05-23 Natalya Zimbovskaya , Godfrey Gumbs

Photosynthesis transfers energy efficiently through a series of antenna complexes to the reaction center where charge separation occurs. Energy transfer in vivo is primarily monitored by measuring fluorescence signals from the small…

The geometry-dependent energy transfer rate from an electrically pumped inorganic semiconductor quantum well into an organic molecular layer is studied theoretically. We focus on F\"orster-type nonradiative excitation transfer between the…

Mesoscale and Nanoscale Physics · Physics 2018-04-20 Judith Specht , Eike Verdenhalven , Björn Bieniek , Patrick Rinke , Andreas Knorr , Marten Richter

Atomic intercalation in two dimensional (2D) layered materials can engineer the electronic structure at the atomic scale, bringing out tunable physical and chemical properties which are quite distinct in comparison with pristine one. Among…

Strongly Correlated Electrons · Physics 2018-03-23 Zahir Muhammad , Kejun Mu , Haifeng Lv , Chuanqiang Wu , Zia ur Rehman , Muhammad Habib , Zhe Sun , Xiaojun Wu , Li Song

Electron transfer (ET) in molecular donor-acceptor dye systems is crucial for charge transport in organic semiconductors. Classically, ET rates should decrease with increasing donor-acceptor distance while the microscopic mechanism is more…

We consider the dependence of the electron transfer in photosynthetic complexes on correlation properties of random fluctuations of the protein environment. The electron subsystem is modeled by a finite network of connected electron…

Biological Physics · Physics 2015-06-23 Alexander I. Nesterov , Gennady P. Berman

Interfacial ultrafast electron migration processes are simulated in finite cluster models of dye-sensitized solar cells within a single active electron approach. Initially, three different donor-acceptor $\pi$-conjugated dyes supported on…

Chemical Physics · Physics 2017-07-06 Gunter Hermann , Felix Witte , Jean Christophe Tremblay

Photosynthesis is arguably the fundamental process of Life, since it enables energy from the Sun to enter the food-chain on Earth. It is a remarkable non-equilibrium process in which photons are converted to many-body excitations which…

Soft Condensed Matter · Physics 2015-05-19 Felipe Caycedo-Soler , Ferney J. Rodríguez , Luis Quiroga , Neil F. Johnson

Exact stationary solutions of the electron-photon Dirac equation are obtained to describe the strong interaction between massless Dirac fermions in graphene and circularly polarized photons. It follows from them that this interaction forms…

Mesoscale and Nanoscale Physics · Physics 2010-04-26 O. V. Kibis

We have grown nitrogen-doped ZnO films grown by two kinds of epitaxial methods on lattice-matched ScAlMgO$_4$ substrates. We measured the photoluminescence (PL) of the two kinds of ZnO:N layers in the donor-acceptor-pair transition region.…

Materials Science · Physics 2009-11-11 Takayuki Makino , A. Tsukazaki , A. Ohtomo , M. Kawasaki , H. Koinuma

Electron relaxation is studied in endofullerene Mg@C60, after an initial localized photoexcitation in Mg, by nonadiabtic molecular dynamics simulations. To ensure reliability, two methods are used: i) an independent particle approach with a…

Atomic and Molecular Clusters · Physics 2021-06-08 Mohamed El-Amine Madjet , Esam Ali , Marcelo Carignano , Oriol Vendrell , Himadri S. Chakraborty

Photoionization of an atom $A$, in the presence of a neighboring atom $B$, can proceed via resonant excitation of $B$ with subsequent energy transfer to $A$ through two-center electron-electron correlation. We demonstrate that this…

Atomic Physics · Physics 2015-05-19 B. Najjari , A. B. Voitkiv , C. Müller

The interaction between free electrons and optical modes underlies a variety of quantum and nanoscale light-matter phenomena, yet the associated momentum exchange with the sample largely remained overlooked. Here, we experimentally…

Optics · Physics 2026-05-01 Akira Yasuhara , Yamato Kirii , Takumi Sannomiya

Spatially indirect Type-II band alignment in magnetically-doped quantum dot (QD) structures provides unexplored opportunities to control the magnetic interaction between carrier wavefunction in the QD and magnetic impurities. Unlike the…

Mesoscale and Nanoscale Physics · Physics 2018-01-17 P. Zhang , T. Norden , J. M. Pientka , R. Oszwałdowski , A. Najafi , B. Barman , Y. Tsai , W-C. Fan , W-C. Chou , J. E. Han , I. Žutić , B. D. McCombe , A. Petrou

The photoelectron momentum shifts along the laser propagation are investigated by the time-dependent perturbation theory for diatomic molecules, such as H$_2^+$, N$_2$ and O$_2$. Such longitudinal momentum shifts characterize the photon…

Optics · Physics 2016-06-08 Di Lao , Pei-Lun He , Feng He

A linear chain of connected electron sites with two asymmetric sinks, one attached to each end, is used as a simple model of quantum electron transfer in photosynthetic bio-complexes. For a symmetric initial population in the middle of the…

Quantum Physics · Physics 2014-03-31 D. Ferrari , G. L. Celardo , G. P. Berman , R. T. Sayre , F. Borgonovi

The radiation of photons by electrons is investigated in the framework of quantum electrodynamics up to the second order in the coupling constant $e$. The $N$-particle, coherent, and thermal initial states are considered and the forms of…

High Energy Physics - Theory · Physics 2022-09-08 P. O. Kazinski , T. V. Solovyev

In this paper, we have explored the charge transfer mechanism in transition metal dichalcogenide (TMDC) quantum dots (QDs) of molybdenum disulfide ($\rm{MoS_2}$) and tungsten disulfide ($\rm{WS_2}$). Rhodamine 6G (R6G), a dye from the…

Applied Physics · Physics 2024-09-20 Praveen Mishra , Arun Singh Patel , Sanjay Kumar Chauhan , Anirban Chakraborti

Electrical transients enabled by optical excitation and electric detection provide a distinctive opportunity to study the charge transport, recombination and even the hysteresis of a solar cell in a much wider time window ranging from…

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