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We develop a density matrix formalism to describe coupled electron-nuclear dynamics. To this end we introduce an effective Hamiltonian formalism that describes electronic transitions and small (quantum) nuclear fluctuations along a…

Chemical Physics · Physics 2020-09-07 Eugene Stolyarov , Alexander White , Dmitry Mozyrsky

The collective response of an atomic ensemble is shaped by its macroscopic environment. We demonstrate this effect in the near-resonant transmission of light through a thermal rubidium vapor confined in a planar nanocavity. Our model…

Atomic Physics · Physics 2020-09-30 Helge Dobbertin , Robert Löw , Stefan Scheel

A novel mixed quantum-classical approach to simulating nonadiabatic dynamics of molecules at metal surfaces is presented. The method combines the numerically exact hierarchical equations of motion approach for the quantum electronic degrees…

Mesoscale and Nanoscale Physics · Physics 2024-05-06 Samuel L. Rudge , Christoph Kaspar , Robin L. Grether , Steffen Wolf , Gerhard Stock , Michael Thoss

We study the adiabatic time evolution of quantum resonances over time scales which are small compared to the lifetime of the resonances. We consider three typical examples of resonances: The first one is that of shape resonances…

Mathematical Physics · Physics 2007-05-23 Walid K. Abou Salem , Juerg Froehlich

This review is focused on various properties of quantum phase transitions (QPTs) in the Interacting Boson Model (IBM) of nuclear structure. The model in its infinite-size limit exhibits shape-phase transitions between spherical, deformed…

Nuclear Theory · Physics 2008-12-18 Pavel Cejnar , Jan Jolie

We present an approach for carrying out non-adiabatic molecular dynamics simulations of systems in which non-adiabatic transitions arise from the coupling between the classical atomic motions and a quasi-continuum of electronic quantum…

Computational Physics · Physics 2018-11-21 Jerome Daligault , Dmitry Mozyrsky

Low-lying quadrupole shape dynamics is a typical manifestation of large amplitude collective motion in finite nuclei. To describe the dynamics on a microscopic foundation, we have formulated a consistent scheme in which the Bohr collective…

Nuclear Theory · Physics 2015-06-18 M. Matsuo , N. Hinohara , K. Sato , K. Matsuyanagi , T. Nakatsukasa , K. Yoshida

We explore topological transitions in parameter space in order to enable adiabatic passages between regions adiabatically disconnected within a given parameter manifold. To this end, we study the Hamiltonian of two coupled qubits…

Mesoscale and Nanoscale Physics · Physics 2016-09-14 Tiago Souza , Michael Tomka , Michael Kolodrubetz , Steven Rosenberg , Anatoli Polkovnikov

We investigate a simple and robust scheme for choosing the phases of adiabatic electronic states smoothly (as a function of geometry) so as to maximize the performance of ab initio non-adiabatic dynamics methods. Our approach is based upon…

Chemical Physics · Physics 2019-09-26 Zeyu Zhou , Zuxin Jin , Tian Qiu , Andrew M. Rappe , Joseph Eli Subotnik

Strongly correlated many-body systems often display the emergence of simple patterns and regular behaviour of their global properties. Phenomena such as clusterization, collective motion and appearance of shell structures are commonly…

Nuclear Experiment · Physics 2020-08-10 R. F. Garcia Ruiz , A. R. Vernon

The operation of near-term quantum technologies requires the development of feasible, implementable, and robust strategies of controlling complex many body systems. To this end, a variety of techniques, so-called "shortcuts to adiabaticty",…

Quantum Physics · Physics 2022-10-21 Artur Soriani , Eduardo Miranda , Sebastian Deffner , Marcus V. S. Bonança

Shape-controlled synthesis of multiply twinned nanostructures is heavily emphasized in nanoscience, in large part due to the desire to control the size, shape, and terminating facets of metal nanoparticles for applications in catalysis.…

Self-assembly kinetics is usually described by approaches which assume that the shape of the aggregates has a definite form (e.g., spherical, cylindrical, cubic, etc), however that is unlikely to be the case in many finite-sized…

Soft Condensed Matter · Physics 2022-07-13 L. F. Trugilho , L. G. Rizzi

We investigate path-wise observables in experiments on driven colloids in a periodic light field to dissect selected intricate transport features, kinetics, and transition-path time statistics out of thermodynamic equilibrium. These…

We investigate the use of an operatorial basis in a self-consistent theory of large amplitude collective motion. For the example of the pairing-plus-quadrupole model, which has been studied previously at equilibrium, we show that a small…

Nuclear Theory · Physics 2009-11-10 Daniel Almehed , Niels R. Walet

We formulate a microscopic theory of the decay of a compound nucleus through fission which generalizes earlier microscopic approaches of fission dynamics performed in the framework of the adiabatic hypothesis. It is based on the constrained…

Nuclear Theory · Physics 2010-02-17 K. Dietrich , J. -J. Niez , J. -F. Berger

Using confocal-microscopy we investigate the structure of binary mixtures of colloidal hard spheres with size ratio q=0.61. As a function of the packing fraction of the two particle species, we observe a marked change of the dominant…

Soft Condensed Matter · Physics 2007-10-04 Jörg Baumgartl , Roel P. A. Dullens , Marjolein Dijkstra , Roland Roth , Clemens Bechinger

Collective motion is a manifestation of emergent phenomena in medium-heavy and heavy nuclei. A relatively large number of constituent nucleons contribute coherently to nuclear excitations (vibrations, rotations) that are characterized by…

Nuclear Theory · Physics 2022-03-18 Z. P. Li , D. Vretenar

The shape phase structure and its transition of the nucleus in the transitional region between the U(5) and SU(3) symmetries is restudied within the framework of coherent-state theory with angular momentum projection in IBM-1. The certain…

Nuclear Theory · Physics 2007-05-23 Liang-zhu Mu , Yu-xin Liu

The challenging nuclear many-body problem is discussed along with classifications and qualitative descriptions of existing methods and models. We present detailed derivations of a new method where cluster correlations co-exist with an…

Nuclear Theory · Physics 2018-07-04 D. Hove , E. Garrido , P. Sarriguren , D. V. Fedorov , H. O. U. Fynbo , A. S. Jensen , N. T. Zinner