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Partition density functional theory is a formally exact procedure for calculating molecular properties from Kohn-Sham calculations on isolated fragments, interacting via a global partition potential that is a functional of the fragment…

Other Condensed Matter · Physics 2015-05-13 Peter Elliott , Kieron Burke , Morrel H. Cohen , Adam Wasserman

We extend the density functional perturbation theory formalism to the case of non-collinear magnetism. The main problem comes with the exchange-correlation (XC) potential derivatives, which are the only ones that are affected by the…

Computational Physics · Physics 2019-05-15 Fabio Ricci , Sergei Prokhorenko , Marc Torrent , Matthieu J. Verstraete , Eric Bousquet

In a homogeneous medium, the far-field generated by a localized source can be expanded in terms of multipoles; the coefficients are determined by the moments of the localized charge distribution. We show that this structure survives to some…

Analysis of PDEs · Mathematics 2017-08-28 Peter Bella , Arianna Giunti , Felix Otto

Stochastic spectral methods are efficient techniques for uncertainty quantification. Recently they have shown excellent performance in the statistical analysis of integrated circuits. In stochastic spectral methods, one needs to determine a…

Computational Engineering, Finance, and Science · Computer Science 2016-11-18 Zheng Zhang , Tarek A. El-Moselhy , Ibrahim , M. Elfadel , Luca Daniel

We showcase the advantages of orbital-free density-potential functional theory (DPFT), a more flexible variant of Hohenberg-Kohn density functional theory. DPFT resolves the usual trouble with the gradient-expanded kinetic energy functional…

Quantum Gases · Physics 2021-06-16 Martin-Isbjörn Trappe , Jun Hao Hue , Berthold-Georg Englert

We develop convergent variational perturbation theory for quantum statistical density matrices. The theory is applicable to polynomial as well as nonpolynomial interactions. Illustrating the power of the theory, we calculate the…

Quantum Physics · Physics 2009-10-31 M. Bachmann , H. Kleinert , A. Pelster

We give formulas for the density of the measure of orthogonality for orthonormal polynomials with unbounded recurrence coefficients. The formulas involve limits of appropriately scaled Tur\'an determinants or Christoffel functions. Exact…

Classical Analysis and ODEs · Mathematics 2017-02-07 Grzegorz Świderski

In this work we give a comprehensive derivation of an exact and numerically feasible method to perform ab-initio calculations of quantum particles interacting with a quantized electromagnetic field. We present a hierachy of…

We present an amelioration of current known algorithms for optimal spectral partitioning problems. The idea is to use the advantage of a representation using density functions while decreasing the computational time. This is done by…

Optimization and Control · Mathematics 2017-05-25 Beniamin Bogosel

In the framework of the Density Functional Theory for superconductors, we study the restoration of the particle number symmetry by means of the projection technique. Conceptual problems are outlined and numerical difficulties are discussed.…

Nuclear Theory · Physics 2008-12-18 J. Dobaczewski , M. V. Stoitsov , W. Nazarewicz , P. -G. Reinhard

We analyse a path to construct density functionals for the dispersion interaction energy from an expression in terms of the ground state densities and exchange-correlation holes of the isolated fragments. The expression is based on a…

Chemical Physics · Physics 2021-01-27 Derk P. Kooi , Paola Gori-Giorgi

This article is concerned with the mathematical analysis of the perturbation method for extended Kohn-Sham models, in which fractional occupation numbers are allowed. All our results are established in the framework of the reduced…

Mathematical Physics · Physics 2017-04-04 Eric Cancès , Nahia Mourad

We use density-functional methods to study the effects of an external magnetic field on two-dimensional quantum dots with a rectangular hard-wall confining potential. The increasing magnetic field leads to spin polarization and formation of…

Strongly Correlated Electrons · Physics 2009-11-10 E. Räsänen , A. Harju , M. J. Puska , R. M. Nieminen

We present a simple formalism for the calculation of the derivatives of the electronic density matrix at any order, within density functional theory. Our approach, contrary to previous ones, is not based on the perturbative expansion of the…

Materials Science · Physics 2009-11-10 Michele Lazzeri , Francesco Mauri

Many high-dimensional uncertainty quantification problems are solved by polynomial dimensional decomposition (PDD), which represents Fourier-like series expansion in terms of random orthonormal polynomials with increasing dimensions. This…

Numerical Analysis · Mathematics 2018-04-06 Sharif Rahman

Fractional occupation numbers can produce open-shell degeneracy in density functional theory. We develop the corresponding perturbation theory by requiring that a differentiable map connects the initial and perturbed states. The degenerate…

Materials Science · Physics 2016-07-22 Mark C. Palenik , Brett I. Dunlap

The macroscopic properties of a quantum system strongly depend on the spreading of the physical eigenfunctions (wavefunctions) of its Hamiltonian operador over its confined domain. The wavefunctions are often controlled by classical or…

Mathematical Physics · Physics 2013-05-17 Jesus S. Dehesa , A. Guerrero , Pablo Sánchez-Moreno

A hypergeometric type equation satisfying certain conditions defines either a finite or an infinite system of orthogonal polynomials. We present in a unified and explicit way all these systems of orthogonal polynomials, the associated…

Quantum Physics · Physics 2009-11-10 Nicolae Cotfas

Hexagon relations are combinatorial or algebraic realizations of four-dimensional Pachner moves. We introduce some simple set-theoretic hexagon relations and then `quantize' them using what we call `polynomial hexagon cohomologies'. Based…

Mathematical Physics · Physics 2018-01-08 Igor G. Korepanov , Nurlan M. Sadykov

Inspired by the works in [1] and [8] we introduce what we call $k$-th-order fluctuation fields and study their scaling limits. This construction is done in the context of particle systems with the property of orthogonal self-duality. This…

Probability · Mathematics 2020-04-21 Mario Ayala , Gioia Carinci , Frank Redig
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