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Related papers: Single-Particle Properties from Kohn-Sham Green's …

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In this paper, we propose a new Green's function embedding method called PEXSI-$\Sigma$ for describing complex systems within the Kohn-Sham density functional theory (KSDFT) framework, after revisiting the physics literature of Green's…

Computational Physics · Physics 2016-10-20 Xiantao Li , Lin Lin , Jianfeng Lu

We present a new charge self-consistent scheme combining Density Functional and Dynamical Mean Field Theory, which uses Green's function of multiple scattering-type. In this implementation the many-body effects are incorporated into the…

Strongly Correlated Electrons · Physics 2017-10-11 A. Östlin , L. Vitos , L. Chioncel

A systematic strategy for the calculation of density functionals (DFs) consists in coding informations about the density and the energy into polynomials of the degrees of freedom of wave functions. DFs and Kohn-Sham potentials (KSPs) are…

Nuclear Theory · Physics 2011-08-25 B. G. Giraud , S. Karataglidis

Kohn-Sham density functional theory is the base of modern computational approaches to electronic structures. Their accuracy vitally relies on the exchange-correlation energy functional, which encapsulates electron-electron interaction…

Computational Physics · Physics 2019-11-04 Ryo Nagai , Ryosuke Akashi , Osamu Sugino

We propose a general machine learning-based framework for building an accurate and widely-applicable energy functional within the framework of generalized Kohn-Sham density functional theory. To this end, we develop a way of training…

Computational Physics · Physics 2020-12-14 Yixiao Chen , Linfeng Zhang , Han Wang , E Weinan

An interesting fundamental problem in density-functional theory of electronic structure of matter is to construct the exact Kohn-Sham (KS) potential for a given density. The exact potential can then be used to assess the accuracy of…

Atomic and Molecular Clusters · Physics 2019-05-22 Ashish Kumar , Rabeet Singh , Manoj K. Harbola

A system of electrons in a local or nonlocal external potential can be studied with 1-matrix functional theory (1MFT), which is similar to density functional theory (DFT) but takes the one-particle reduced density matrix (1-matrix) instead…

Strongly Correlated Electrons · Physics 2008-07-23 Ryan Requist , Oleg Pankratov

Density functional theory is currently the most widely applied method in electronic structure theory. The Kohn-Sham method, based on a fictitious system of non-interacting particles, is the work horse of the theory. The particular form of…

Chemical Physics · Physics 2016-06-01 Hubertus J J van Dam

One of the potential applications of a quantum computer is solving quantum chemical systems. It is known that one of the fastest ways to obtain somewhat accurate solutions classically is to use approximations of density functional theory.…

Quantum Physics · Physics 2020-11-18 Thomas E. Baker , David Poulin

We introduce a general, variational scheme applied to Kohn-Sham density functional theory that allows for partitioning of the ground-state density matrix into distinct spectral domains, each of which spanned by an independent diagonal…

Plasma Physics · Physics 2023-08-29 Babak Sadigh , Daniel Aberg , John Pask

Density-functional theory for superfluid systems is developed in the framework of the functional renormalization group based on the effective action formalism. We introduce the effective action for the particle-number and nonlocal pairing…

Nuclear Theory · Physics 2021-05-11 Takeru Yokota , Haruki Kasuya , Kenichi Yoshida , Teiji Kunihiro

Developing a reliable kinetic energy density functional within orbital-free density functional theory remains a long-standing challenge, particularly for atomic and molecular systems. A major difficulty lies in the absence of a systematic…

Chemical Physics · Physics 2025-10-22 Priya Priya , Anuvab Panda , Saswata Basu , Mainak Sadhukhan

A Skyrme-like effective interaction is built up from the equation of state of nuclear matter. The latter is calculated in the framework of the Brueckner-Hartree-Fock approximation with two and three body forces. A complete Skyrme…

Nuclear Theory · Physics 2009-11-11 L. G. Cao , U. Lombardo , C. W. Shen , Nguyen Van Giai

It has recently been observed [Phys. Rev. Lett. 113, 113002 (2014)] that the ground-state energy may be obtained directly as a simple sum of augmented Kohn-Sham orbital energies, where it was ascertained that the corresponding one-body…

Chemical Physics · Physics 2016-05-04 Mel Levy , Federico Zahariev

Relativistic mean field theory is formulated with the Green's function method in coordinate space to investigate the single-particle bound states and resonant states on the same footing. Taking the density of states for free particle as a…

Nuclear Theory · Physics 2015-06-23 T. T. Sun , S. Q. Zhang , Y. Zhang , J. N. Hu , J. Meng

We consider the extension of the standard single-determinant Kohn-Sham method to the case of a multiconfiguration trial wavefunction. By applying the rigorous Kohn-Sham method to this case, we construct the proper interacting and…

Strongly Correlated Electrons · Physics 2008-12-08 Yair Kurzweil , M. Head-Gordon

We introduce a functional of the local spectral electron density which can be used to to compute the total energy and the local spectral function of strongly-correlated materials. We illustrate the applicability of the method by using as an…

Strongly Correlated Electrons · Physics 2007-05-23 S. Y. Savrasov , G. Kotliar

The LSDA+U approach to density functional theory is carefully reanalyzed. Its possible link to single-particle Green's function theory is occasionally discussed. A simple and elegant derivation of the important sum rules for the on-site…

Strongly Correlated Electrons · Physics 2009-11-10 H. Eschrig , K. Koepernik , I. Chaplygin

The Green's function method in the \emph{Quasiparticle Time Blocking Approximation} is applied to nuclear excitations in $^{132}$Sn and $^{208}$Pb. The calculations are performed self-consistently using a Skyrme interaction. The method…

Nuclear Theory · Physics 2008-11-26 N. Lyutorovich , J. Speth , A. Avdeenkov , F. Gruemmer , S. Kamerdzhiev , S. Krewald , V. I. Tselyaev

The single-particle spectral functions in asymmetric nuclear matter are computed using the ladder approximation within the theory of finite temperature Green's functions. The internal energy and the momentum distributions of protons and…

Nuclear Theory · Physics 2009-11-10 T. Frick , H. Müther , A. Rios , A. Polls , A. Ramos