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Buckingham expansion is important for understanding molecular multipoles and (hyper)polarizabilities. In this study, we give a complete derivation of Buckingham expansion in the traced form using successive Taylor series. Based on such…

Chemical Physics · Physics 2020-08-26 Houxian Chen , Menglin Liu , Tianying Yan

By judicious use of extrapolations to the 1-particle basis set limit and $n$-particle calibration techniques, total atomization energies of molecules with up to four heavy atoms can be obtained with calibration accuracy (1 kJ/mol or better,…

Chemical Physics · Physics 2007-05-23 Jan M. L. Martin

Shell-model calculations in a large model space are performed for _{\Lambda}^{16}O and_{\Lambda}^{17}O. Effective interactions with degrees of freedom of \Sigma in addition to \Lambda and nucleons are derived from hyperon-nucleon and…

Nuclear Theory · Physics 2009-11-07 S. Fujii , R. Okamoto , K. Suzuki

Almost every numerical task can be cast as extrapolation with respect to the fidelity or tolerance parameters of a consistent numerical method. This perspective enables probabilistic uncertainty quantification and optimal experimental…

Methodology · Statistics 2026-04-03 Chris. J. Oates , Richard Howey , Toni Karvonen

High-precision predictions of nuclear properties are a central objective of ab initio nuclear structure theory. However, state-of-the-art many-body methods rely on truncated model spaces to render the nuclear many-body problem tractable,…

Nuclear Theory · Physics 2026-04-10 Marco Knöll

Quantum Monte Carlo methods find fruitful application in large shell model problems. These methods reduce the imaginary-time many-body evolution operator to a coherent superposition of one-body evolutions in a fluctuating one-body field;…

Nuclear Theory · Physics 2008-02-03 S. E. Koonin

The configuration-interaction shell model approach provides an attractive framework for the calculation of nuclear level densities in the presence of correlations, but the large dimensionality of the model space has hindered its application…

Nuclear Theory · Physics 2016-01-05 Y. Alhassid , G. F. Bertsch , C. N. Gilbreth , H. Nakada , C. Özen

The shell model is the standard tool for addressing the canonical nuclear many-body problem of nonrelativistic nucleons interacting through a static potential. We discuss several of the uncontrolled approximations that are made in this…

Nuclear Theory · Physics 2007-05-23 W. C. Haxton , C. -L. Song

The accuracy of the Heller's derivative rule to calculate the numerical weights associated with discretized energy spectrum is enhanced by Broad's extension which adds (N-1) more interpolating points to the original N points. The extension…

Mathematical Physics · Physics 2017-10-03 Hashim A. Yamani , Abdulaziz D. Alhaidari

Direct numerical simulation of dynamical systems is of fundamental importance in studying a wide range of complex physical phenomena. However, the ever-increasing need for accuracy leads to extremely large-scale dynamical systems whose…

Dynamical Systems · Mathematics 2015-03-04 Jeff T. Borggaard , Serkan Gugercin

A novel approach to obtain the excitation spectrum of nuclei is presented as well as its proof-of-principle. The Monte Carlo Shell Model is extended so that the excitation spectrum can be calculated from its ground state with full of…

Nuclear Theory · Physics 2018-07-02 Takaharu Otsuka , Tomoaki Togashi , Noritaka Shimizu , Yutaka Utsuno , Toshio Suzuki

The purpose of the paper is to present a new pricing method for clean spread options, and to illustrate its main features on a set of numerical examples produced by a dedicated computer code. The novelty of the approach is embedded in the…

Pricing of Securities · Quantitative Finance 2015-05-27 Rene Carmona , Michael Coulon , Daniel Schwarz

The shell model Monte Carlo (SMMC) method enables calculations in model spaces that are many orders of magnitude larger than those that can be treated by conventional methods, and is particularly suitable for the calculation of level…

Nuclear Theory · Physics 2015-06-18 Y. Alhassid , M. Bonett-Matiz , S. Liu , A. Mukherjee , H. Nakada

We obtain an expansion of the implicit weak discretization error for the target of stochastic approximation algorithms introduced and studied in [Frikha2013]. This allows us to extend and develop the Richardson-Romberg extrapolation method…

Probability · Mathematics 2015-03-10 Noufel Frikha , Lorick Huang

The shell model Monte Carlo (SMMC) approach provides a powerful method for the microscopic calculation of statistical and collective nuclear properties in model spaces that are many orders of magnitude larger than those that can be treated…

Nuclear Theory · Physics 2015-06-11 Y. Alhassid , A. Mukherjee , H. Nakada , C. Özen

We introduce a particle-number reprojection method in the shell model Monte Carlo that enables the calculation of observables for a series of nuclei using a Monte Carlo sampling for a single nucleus. The method is used to calculate nuclear…

Nuclear Theory · Physics 2009-10-31 Y. Alhassid , S. Liu , H. Nakada

The performance of numerical micromagnetic models is limited by the demagnetizing field computation, which typically accounts for the majority of the computation time. For magnetization dynamics simulations explicit evaluation methods are…

Computational Physics · Physics 2022-06-15 Serban Lepadatu

In this contribution, a new framework for H2-optimal reduction of multiple-input, multiple- output linear dynamical systems by tangential interpolation is presented. The framework is motivated by the local nature of both tangential…

Numerical Analysis · Mathematics 2017-09-22 Alessandro Castagnotto , Boris Lohmann

Calculating relative free energies is a topic of substantial interest and has many applications including solvation and binding free energies, which are used in computational drug discovery. However, there remain the challenges of accuracy,…

Chemical Physics · Physics 2016-09-28 Asaf Farhi , Bipin Singh

We construct a reference benchmark set for atomic and molecular random-phase-approximation (RPA) correlation energies in a density functional theory (DFT) framework at the complete basis set limit. This set is used to evaluate the accuracy…

Chemical Physics · Physics 2013-02-22 E. Fabiano , F. Della Sala