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Kinetics of sequential first-order reactions occurring in a chromatographic medium is developed. A model for motion of substances of a chain 1 -> 2 -> 3 -> in an infinite chromatographic column is worked out, and a mathematical procedure…

Chemical Physics · Physics 2021-06-28 S. V. Ermolaev , A. K. Skasyrskaya

The paper gives an account of a detailed investigation of the thermodynamic branch as a path of the chemical system deviation from its isolated thermodynamic equilibrium under an external impact. For a combination of direct and reverse…

General Physics · Physics 2012-03-26 B. Zilbergleyt

The analytic solution for the kinetic description of binary reactions can be seen as the continuum version of a basic discrete iterate mapping. This fact allows a clear definition of the reaction characteristic time which takes the backward…

Mathematical Physics · Physics 2013-10-15 R. Aldrovandi

The rates of chemical reactions are not absolute but their magnitude depends upon the relative speeds of the moving observers. This has been proved by unifying theories of chemical kinetics, which are transition state theory, collision…

General Physics · Physics 2017-06-13 Mirza Wasif Baig

We consider the design criteria of a chemical mixing device based on a chaotic flow, with an emphasis on the steady-state devices. The merit of a reactor, defined as the $Q$-factor, is related to the physical dimension of the device and the…

Fluid Dynamics · Physics 2009-10-31 X. Z. Tang , A. H. Boozer

We use a recent result to show that the rate of loss of coherence of a quantum system increases with increasing system phase space structure and that a chaotic quantal system in the semiclassical limit decoheres exponentially with rate $2…

chao-dyn · Physics 2009-10-30 Arjendu K. Pattanayak , Paul Brumer

The chemical reactions are very complex, and include oscillation, condensation, catalyst and self-organization, etc. In these case changes of entropy may increase or decrease. The second law of thermodynamics is based on an isolated system…

General Physics · Physics 2008-07-03 Yi-Fang Chang

We build in this paper a numerical solution procedure to compute the flow induced by a spherical flame expanding from a point source at a constant expansion velocity, with an instantaneous chemical reaction. The solution is supposed to be…

Numerical Analysis · Mathematics 2020-10-19 D Grapsas , R Herbin , J. -C Latché , Y Nasseri

The main aim of this paper is to detect dynamical properties of the Gy\"orgyi-Field model of the Belousov-Zhabotinsky chemical reaction. The corresponding three-variable model given as a set of nonlinear ordinary differential equations…

Chaotic Dynamics · Physics 2020-05-08 Judita Nagyová , Branislav Jansík , Marek Lampart

The chaotic scattering theory is here extended to obtain escape-rate expressions for the transport coefficients appropriate for a simple classical fluid, or for a chemically reacting system. This theory allows various transport coefficients…

chao-dyn · Physics 2009-10-22 J. R. Dorfman , P. Gaspard

The predictive ability of stochastic chemical reactions is currently limited by the lack of closed form solutions to the governing chemical master equation. To overcome this limitation, this paper proposes a computational method capable of…

Quantitative Methods · Quantitative Biology 2019-01-08 Yuta Sakurai , Yutaka Hori

We introduce a fully generalized quiescent chemical reactor system in arbitrary space $\vdim =1,2$ or 3, with $n\in\mathbb{N}$ chemical constituents $\alpha_{i}$, where the character of the numerical solution is strongly determined by the…

Chemical Physics · Physics 2010-12-30 C. E. Michoski , J. A. Evans , P. G. Schmitz

Statistical aspects of the dynamics of chaotic scattering in the classical model of $\alpha$-cluster nuclei are studied. It is found that the dynamics governed by hyperbolic instabilities which results in an exponential decay of the…

Nuclear Theory · Physics 2009-09-25 S. Drożdż , J. Okołowicz , T. Srokowski , A. Budzanowski

A novel flow instability emerging during a rheometric flow of a phase change material sheared in the vicinity of the solid-fluid transition is reported. Right above the onset of the flow induced crystallisation, the presence of the crystals…

Fluid Dynamics · Physics 2021-07-01 Rawad Himo , Cathy Castelain , Teodor Burghelea

We numerically and analytically investigate the behavior of a non-equilibrium phase transition in the second Schl\"ogl autocatalytic reaction scheme. Our model incorporates both an interaction-induced phase separation and a bifurcation in…

Statistical Mechanics · Physics 2023-11-02 Reda Tiani , Uwe C. Täuber

We study phase-separating fluid mixtures as they demix in the presence of chemical reactions that maintain them away from thermodynamic equilibrium. We show that in such chemically active emulsions the interplay of chemical reactions, phase…

Fluid Dynamics · Physics 2025-09-22 Charu Datt , Jonathan Bauermann , Nazmi Burak Budanur , Frank Jülicher

We propose a concise stochastic mechanics framework for chemical reaction systems that allows to formulate evolution equations for three general types of data: the probability generating functions, the exponential moment generating…

Mathematical Physics · Physics 2018-02-23 Nicolas Behr , Gérard H. E. Duchamp , Karol A. Penson

We investigate the evolution of particle ensembles in open chaotic hydrodynamical flows. Active processes of the type A+B --> 2B and A+B --> 2C are considered in the limit of weak diffusion. As an illustrative advection dynamics we consider…

chao-dyn · Physics 2009-10-31 Gy. Karolyi , A. Pentek , Z. Toroczkai , T. Tel , C. Grebogi

The stationary-state spatial structure of reacting scalar fields, chaotically advected by a two-dimensional large-scale flow, is examined for the case for which the reaction equations contain delay terms. Previous theoretical investigations…

Fluid Dynamics · Physics 2015-05-13 Alexandra Tzella , Peter H. Haynes

Results are presented for the phase separation process of a binary mixture subject to an uniform shear flow quenched from a disordered to a homogeneous ordered phase. The kinetics of the process is described in the context of the…

Condensed Matter · Physics 2012-04-05 F. Corberi , G. Gonnella , A. Lamura