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The ultrafast dynamics of the antiferrodistortive (AFD) phase transition in perovskite SrTiO3 is monitored via time-domain Brillouin scattering. Using femtosecond optical pulses, we induce a thermally driven tetragonal-to-cubic structural…

Materials Science · Physics 2023-09-07 Saqeeb Adnan , Amey Khanolkar , Shuxiang Zhou , David H. Hurley , Marat Khafizov

The effect of ferroelectric fluctuations on the temperature dependent dielectric constant of SrTiO$_3\,$(STO) has been long studied. Those fluctuations have been shown in recent years to be quantum critical and STO demonstrated to form the…

Strongly Correlated Electrons · Physics 2019-12-18 M. J. Coak , C. R. S. Haines , C. Liu , G. G. Guzmán-Verri , S. S. Saxena

Perovskite structured materials contain myriad tunable ordered phases of electronic and magnetic origin with proven technological importance and strong promise for a variety of energy solutions. An always-contributing influence beneath…

Zero-temperature or quantum phase transitions in itinerant electronic systems both with and without quenched disordered are discussed. Phase transitions considered include, the ferromagnetic transition, the antiferromagnetic transition, the…

Statistical Mechanics · Physics 2008-02-03 T. R. Kirkpatrick , D. Belitz

Motivated by recent experiments reporting superconductivity only at very low temperature in a class of heavy fermion compounds, we study the impact of energy fluctuations with small momentum transfer on the pairing instability near an…

Superconductivity · Physics 2018-12-31 Jian Kang , Rafael M. Fernandes , Elihu Abrahams , Peter Wölfle

Dielectric spectroscopy of $SrTiO_3$ single crystal over a broad range of microwave frequency using quasi $TE_{m,1,1}$ and quasi $TM_{m,1,1}$ modes reveals crystal asymmetry from typical measurement of $Q$-factor, transmission or frequency…

Materials Science · Physics 2025-05-22 M. A. Hosain , J-M. Le Floch , J. F. Bourhill , J. Krupka , M. E. Tobar

Composites of ferroelectric and paraelectric perovskites have attracted a lot of attention due to their application potential in energy storage as well as novel computing and memory devices. So far the main focus of research has been on…

Materials Science · Physics 2025-07-23 Sheng-Han Teng , Chinwendu Anabaraonye , Anna Grünebohm

The temperature dependence of static dielectric susceptibility of a system with strongly coupled fluctuating dipoles is calculated within a self consistent mean fluctuation field approximation. Results are qualitatively in good agreement…

Materials Science · Physics 2015-05-13 Nabyendu Das , Suresh G. Mishra

It has been known for a long time that the low temperature behavior shown by the dielectric constant of quantum paraelectric $SrTiO_{3}$ can not be fitted properly by Barrett's formula using a single zero point energy or saturation…

Materials Science · Physics 2009-11-11 Manuel I. Marques , Carmen Arago , Julio A. Gonzalo

Quantum fluctuations (QFs) caused by zero-point phonon vibrations (ZPPVs) are known to prevent the occurrence of polar phases in bulk incipient ferroelectrics down to 0K1-3. On the other hand, little is known about the effects of QFs on the…

Materials Science · Physics 2023-10-27 W. Luo , A. Akbarzadeh , Y. Nahas , S. Prokhorenko , L. Bellaiche

We demonstrate an approach for calculating temperature-dependent quantum and anharmonic effects with beyond density-functional theory accuracy. By combining machine-learned potentials and the stochastic self-consistent harmonic…

Materials Science · Physics 2023-03-03 Carla Verdi , Luigi Ranalli , Cesare Franchini , Georg Kresse

Molecular dynamics simulations predict a giant electrocaloric effect at the ferroelectric-antiferroelectric phase boundary in PZT (PbTiO$_3$-PbZrO$_3$). These large-scale simulations also give insights into the atomistic mechanisms of the…

Materials Science · Physics 2019-07-24 A. V. Kimmel , O. T. Gindele , D. M. Duffy , R. E. Cohen

We investigate the structural and thermodynamic properties of high-pressure ice by incorporating quantum anharmonicity at a non-perturbative level. Quantum fluctuations reduce the critical pressure of the phase transition between phase VIII…

Other Condensed Matter · Physics 2024-03-15 Marco Cherubini , Lorenzo Monacelli , Bingjia Yang , Roberto Car , Michele Casula , Francesco Mauri

The interpretation of the magnetic phase diagrams of strongly correlated electron systems remains controversial. In particular, the physics of quantum phase transitions, which occur at zero temperature, is still enigmatic. Heavy-fermion…

Strongly Correlated Electrons · Physics 2012-11-08 W. Knafo , S. Raymond , P. Lejay , J. Flouquet

We determine the effects of quantum fluctuations about the T=0 mean field solution of the BCS-BEC crossover in a dilute Fermi gas using the functional integral method. These fluctuations are described in terms of the zero point motion of…

Other Condensed Matter · Physics 2008-03-20 Roberto B. Diener , Rajdeep Sensarma , Mohit Randeria

In one-dimension, quantum fluctuations prevent the appearance of long-range order in a supersolid, and only quasi long-range order can survive. We derive this quantum critical behavior and study its influence on the superfluid response and…

Quantum Gases · Physics 2023-08-11 Chris Bühler , Tobias Ilg , Hans Peter Büchler

We present an inexpensive first-principles approach for describing quantum paraelectricity that combines density functional theory (DFT) treatment of the electronic subsystem with quantum mechanical treatment of the ions through solution of…

Materials Science · Physics 2022-07-27 Tobias Esswein , Nicola A. Spaldin

A semiclassical approach that incorporates quantum mechanical behavior of heat capacity in direct caloric effect simulations is proposed. Application of this methodology to study electrocaloric effect in prototypical ferroelectrics ${ \rm…

Computational Physics · Physics 2017-12-27 P. Jouzdani , S. Cuozzo , S. Lisenkov , I. Ponomareva

SrTiO$_{3}$ undergoes a cubic-to-tetragonal phase transition at 105K. This antiferrodistortive transition is believed to be in competition with incipient ferroelectricity. Substituting strontium by isovalent calcium induces a ferroelectric…

The machine learning potential (MLP) based molecular dynamics (MD) method was applied for constructing the pressure-temperature phase diagram in the barium titanate (BaTiO3) crystals. The nuclear quantum effects (NQEs) on the phase…

Materials Science · Physics 2024-11-19 Kansei Kanayama , Kazuaki Toyoura