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We propose an ab-initio molecular dynamics method, capable to reduce dramatically the autocorrelation time required for the simulation of classical and quantum particles at finite temperature. The method is based on an efficient…

Strongly Correlated Electrons · Physics 2017-01-11 Sandro Sorella , Guglielmo Mazzola

Molecular dynamics simulation is used to study the time-scales involved in the homogeneous melting of a superheated crystal. The interaction model used is an embedded-atom model for Fe developed in previous work, and the melting process is…

Statistical Mechanics · Physics 2015-05-27 D. Alfè , C. Cazorla , M. J. Gillan

The results of the molecular dynamics simulation of the radiation influence on the structure and thermophysical properties of water are presented. The changes in the radial distribution functions, momentum distribution function and the…

Statistical Mechanics · Physics 2017-01-25 L. A. Bulavin , K. V. Cherevko , D. A. Gavryushenko , V. M. Sysoev , T. S. Vlasenko

This paper presents an $ab$ $initio$ study of hydrogen dynamics inside nanometer-size voids in $a$-Si within the framework of the density-functional theory for a varying hydrogen load of 10 to 30 H atoms/void at the low and high temperature…

Materials Science · Physics 2021-10-04 Parthapratim Biswas , Dil Limbu

Tight binding molecular dynamics simulations, with a non orthogonal basis set, are performed to study the fragmentation of carbon fullerenes doped with up to six silicon atoms. Both substitutional and adsorbed cases are considered. The…

Materials Science · Physics 2009-11-07 Chu-Chun Fu , Javier Fava , Ruben Weht , M. Weissmann

We use extensive classical molecular dynamics simulations to calculate the thermal conductivity of a model silica glass. Apart from the potential parameters, this is done with no other adjustable quantity and the standard equations of heat…

Disordered Systems and Neural Networks · Physics 2009-10-31 Philippe Jund , Remi Jullien

The changing thermal conductivity of an irradiated material is among the principal design considerations for any nuclear reactor, but at present few models are capable of predicting these changes starting from an arbitrary atomistic model.…

Materials Science · Physics 2021-11-25 Daniel R Mason , Abdallah Reza , Fredric Granberg , Felix Hofmann

Aqueous mixtures of 1-propanol have been investigated by high-energy synchrotron X-ray diffraction upon cooling. X-ray weighted total scattering structure factors of 6 mixtures, from 8 mol% to 89 mol% alcohol content, as well as that of…

Chemical Physics · Physics 2021-08-25 Ildikó Pethes , László Pusztai , Koji Ohara , László Temleitner

Cadmium selenide (CdSe) is an inorganic semiconductor with unique optical and electronic properties that made it useful in various applications, including solar cells, light-emitting diodes, and biofluorescent tagging. In order to…

Materials Science · Physics 2023-05-30 Linshuang Zhang , Manyi Yang , Shiwei Zhang , Haiyang Niu

Ab initio molecular dynamics is used to study deformations of sodium clusters at temperatures $500\cdots 1100$ K. Open-shell Na$_{14}$ cluster has two shape isomers, prolate and oblate, in the liquid state. The deformation is stabilized by…

mtrl-th · Physics 2016-09-07 H. Hakkinen , M. Manninen

The vibrational entropy of a solid at finite temperature is investigated from the perspective of information theory. Ab initio molecular dynamics (AIMD) simulations generate ensembles of atomic configurations at finite temperature from…

Statistical Mechanics · Physics 2022-05-11 Yang Huang , Michael Widom

We report a new approach to simulate amorphous networks of covalently bonded materials that leads to excellent radial distribution functions and realistic atomic arrangements. We apply it to generate the first ab initio structures of…

Materials Science · Physics 2007-05-23 Fernando Alvarez , Ariel A. Valladares

For the first time primary hot isotope distributions are experimentally reconstructed in intermediate heavy ion collisions and used with antisymmetrized molecular dynamics (AMD) calculations to determine density, temperature and symmetry…

Computational modelling of passage of high-energy electrons through crystalline media is carried out by means of the relativistic molecular dynamics. The results obtained are compared with the experimental data for 855 MeV electron beam…

Accelerator Physics · Physics 2023-09-19 V. V. Haurylavets , V. K. Ivanov , A. V. Korol , A. V. Solov'yov

An ab initio molecular dynamics study of femtosecond laser processing of germanium is presented in this paper. The method based on the finite temperature density functional theory is adopted to probe the structural change, thermal motion of…

Computational Physics · Physics 2016-02-02 Pengfei Ji , Yuwen Zhang

Using a realistic flexible molecule model of the fragile glass former orthoterphenyl, we calculate via molecular dynamics simulation the collective dynamic structure factor, recently measured in this system by Inelastic X-ray Scattering.…

Soft Condensed Matter · Physics 2009-11-07 S. Mossa , G. Monaco , G. Ruocco , M. Sampoli , F. Sette

A molecular dynamics simulation of sublimation of silicene and silicon films of different thikness is performed. It is shown that thiner films sublimate at lower temperatures. The sublimation temperature comes to a saturated value of…

Materials Science · Physics 2023-09-06 Yu. D. Fomin , E. N. Tsiok , V. N. Ryzhov

The performance of amorphous selenium (a-Se) as a cryogenic photodetector material is evaluated through a series of experiments using laterally structured devices operated in a custom optical test stand. These studies investigate the…

Instrumentation and Detectors · Physics 2025-11-03 M. Rooks , S. Abbaszadeh , J. Asaadi , V. A. Chirayath , M. Febbraro , M. Á. García-Peris , E. Gramellini , K. Hellier , B. Sudarsan , I. Tzoka

Since the discovery of high-temperature superconductivity in the thin-film FeSe/SrTiO$_3$ system, iron selenide and its derivates have been intensively scrutinized. Using ab initio density functional theory calculations we review the…

Superconductivity · Physics 2017-09-07 Daniel Guterding , Harald O. Jeschke , Roser Valenti

Methanol-water liquid mixtures have been investigated by high-energy synchrotron X-ray and neutron diffraction at low temperatures. We are thus able to report the first complete sets of both X-ray and neutron weighted total scattering…