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We present a total energy study as a function of volume in the cubic phase of LaMnO$_{3}$. A charge disproportionated state into planes of Mn$^{3+}$O$_{2}$/Mn$^{4+}$O$_{2}$ was found. It is argued that the pressure driven…

Strongly Correlated Electrons · Physics 2009-11-10 G. Banach , W. M. Temmerman

External pressure driven phase transitions of FeSe are predicted using \textit{ab initio} calculations. The calculations reveal that $\alpha$-FeSe takes transitions to NiAs-type, MnP-type, and CsCl-type FeSe. Transitions from NiAs-type to…

Materials Science · Physics 2015-06-03 Gul Rahman , In Gee Kim , Arthur J. Freeman

We report a facile `metric' for the identification of structurally and dynamically (positive definite phonon structure) stable inorganic compounds. The metric considers charge-imbalance within the local substructures in crystalline…

Materials Science · Physics 2020-11-19 R. Villarreal , P. Singh , R. Arroyave

We have performed systematic first principles study of the electronic structure and band topology properties of $LnPn$ compounds ($Ln$=Ce, Pr, Gd, Sm, Yb; $Pn$=Sb, Bi). Assuming the $f$-electrons are well localized in these materials, both…

Strongly Correlated Electrons · Physics 2018-11-09 Xu Duan , Fan Wu , Jia Chen , Peiran Zhang , Yang Liu , Huiqiu Yuan , Chao Cao

We search for new superhard B-N-O compounds with an iterative machine learning (ML) procedure, where ML models are trained using sample crystal structures from evolutionary algorithm. We first use cohesive energy to evaluate the…

Materials Science · Physics 2022-06-22 Wei-Chih Chen , Yogesh K. Vohra , Cheng-Chien Chen

We report first principles calculations of the structural, electronic, elastic and vibrational properties of the semiconducting orthorhombic ZnSb compound. We study also the intrinsic point defects in order to eventually improve the…

Materials Science · Physics 2012-07-09 Philippe Jund , Romain Viennois , Xiaoma Tao , Kinga Niedziolka , Jean-Claude Tedenac

We give a general thermodynamical argument showing that in neutron stars, the Coulomb structured mixed phase is always favored for any first order phase transition involving systems in equilibrium with baryon number and electric charge as…

Astrophysics · Physics 2007-05-23 Michael B. Christiansen , Norman K. Glendenning

First Principles calculations are performed on the cubic bulk and its (001) surface of CsPbBr3 to reveal its electronic and optoelectronic properties. Various calculation schemes like GGA, GGA+SOC and the highly accurate modified Becke…

Materials Science · Physics 2021-08-03 H. Joshi , R. K. Thapa , Lalrinthara Pachuau , Lalmuanpuia Vanchhawng , D. P. Rai

The structure of Nd$_{1-x}$Pb$_{x}$MnO$_{3}$ crystals is determined by single crystal X-ray diffraction. Substitution of Pb at the Nd site results in structural phase change from tetragonal (x = 0.25) to cubic (x = 0.37). These changes are…

Strongly Correlated Electrons · Physics 2007-05-23 Nilotpal Ghosh , Suja Elizabeth , H. L. Bhat , G. Nalini , B. Muktha , T. N. Guru Row

Brittle topologically close-packed precipitates form in many advanced alloys. Due to their complex structures little is known about their plasticity. Here, we present a strategy to understand and tailor the deformability of these complex…

The structural misfit compound (PbSe)1.16(TiSe2)2 is reported. It is a superconductor with a Tc of 2.3 K. (PbSe)1.16(TiSe2)2 derives from a parent compound, TiSe2, which shows a charge density wave transition and no superconductivity. The…

Superconductivity · Physics 2015-05-19 N. Giang , Q. Xu , Y. S. Hor , A. J. Williams , S. E. Dutton , H. W. Zandbergen , R. J. Cava

Over the past two decades, unconventional superconductivity with gap symmetry other than s-wave has been found in several classes of materials, including heavy fermion (HF), high-T_c, and organic superconductors. Unconventional…

Superconductivity · Physics 2009-11-11 Y. Matsuda , K. Izawa , I. Vekhter

Monte Carlo simulations, supplemented by ab initio calculations, shed light into the energetics and thermodynamic stability of nanostructured amorphous carbon. The interaction of the embedded nanocrystals with the host amorphous matrix is…

Materials Science · Physics 2009-11-11 Maria G. Fyta , Pantelis C. Kelires

We have studied structural phase transition in BaNi2As2 superconductor with the application of Phosphorous doping based on first principles calculations. Our results reproduce experimental findings and explain some of the experimental…

Superconductivity · Physics 2012-08-03 Wasim Raja Mondal , Swapan K. Pati

A series of MnO2 unique nanostructures were synthesized by a facile hydrothermal method with microwave-assisted procedures. A novel nanostructure formation mechanism has been proposed, that MnO6 octahedral nuclei and molecular layers can be…

Mesoscale and Nanoscale Physics · Physics 2012-07-16 R. Zeng , J. Q. Wang , G. D. Du , W. X. Li , Z. X. Chen , S. Li , S. X. Dou

Possible crystalline modifications of chemical compounds at low temperatures correspond to local minima of the energy landscape. Determining these minima via simulated annealing is one method for the prediction of crystal structures, where…

Materials Science · Physics 2008-10-31 K. Doll , J. C. Schoen , M. Jansen

The temperature ($T$) as a function of pressure ($P$) phase diagram is reported for the cubic Laves phase compound Au$_2$Pb, which was recently proposed to support linearly dispersing "topological" bands, together with conventional…

Materials Science · Physics 2016-01-25 K. W. Chen , D. Graf , T. Besara , A. Gallagher , N. Kikugawa , L. Balicas , T. Siegrist , A. Shekhter , R. E. Baumbach

Ordinary band structure calculations of quantum materials often incorrectly predicted metallic, instead of insulating electronic structure, motivating Mott-Hubbard strong electron correlation as a gapping mechanism. More recently, allowing…

Materials Science · Physics 2024-08-02 Jia-Xin Xiong , Xiuwen Zhang , Alex Zunger

X-ray photoelectron spectroscopy and diffraction (XPS, XPD) and scanning tunneling microscopy (STM) have been used for study of NbOx-structures on the Nb(110) surface. It is shown that niobium atoms are ordered to form a two-dimensional…

Materials Science · Physics 2008-11-11 A. S. Razinkin , E. V. Shalaeva , M. V. Kuznetsov

We present an ab-initio study of boron nitride as well as carbon allotropes. Their relative thermodynamic stabilities and structural phase transitions from low- to high-density phases are investigated. Pressure-temperature phase diagrams…

Materials Science · Physics 2019-02-22 Thomas Gruber , Andreas Grüneis