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The controlled assembly of twisted 2D structures requires precise determination of the crystal orientation of their component layers. In the established procedure, the second-harmonic generation (SHG) intensity of a noncentrosymmetric layer…

The generation of harmonics by atoms interacting with two circularly polarized and frequency related laser fields is addressed through ab initio numerical simulations. A detailed charaterization of a few specific harmonics is given. In…

Atomic Physics · Physics 2009-11-10 F. Ceccherini , N. Davini , D. Bauer , F. Cornolti

Optical response of free-electron gas leads to inherent nonlinear optical behaviour of nanostructured plasmonic materials enabled via both strong local field enhancements and inherent complex electron dynamics. We present a comprehensive…

High-strain piezoelectric materials are often ceramics with a complicated constitution. In particular, PZT is used with compositions near to a so-called morphotropic phase boundary, where not only different variants of the same phase…

Materials Science · Physics 2009-11-11 Johannes Rödel

We generate high-order harmonics in gaseous medium with tunable photon energy using time domain interferometry of double pulses in a non-collinear generation geometry. The method is based on the fact that the generated harmonics inherit…

Second-harmonic generation (SHG) is a powerful surface-specific probe for centrosymmetric materials, with broad relevance to energy and biological interfaces. Plasmonic nanomaterials have been extensively utilized to amplify this nonlinear…

Nonlinear crystals are widely used to efficiently generate second or third harmonics, and also for frequency mixing. Generation of multiple cascaded harmonics simultaneously, however, appears much less studied, although supported by the…

Optics · Physics 2026-03-16 J. Seres , E. Seres , T. Schumm

Nonlinear optical processes in whispering gallery mode (WGM) microresonators have attracted much attention. Owing to the strong confinement of light in a small volume, a WGM microresonator can dramatically boost the strength of light field,…

Optics · Physics 2015-12-29 Jintian Lin , Yingxin Xu , Jielei Ni , Min Wang , Zhiwei Fang , Lingling Qiao , Wei Fang , Ya Cheng

The recently discovered ferroelectric nematic liquids incorporate to the functional combination of fluidity, processability and anisotropic optical properties of nematic liquids, an astonishing range of physical properties derived from the…

Second-harmonic generation (SHG) is a fundamental tool in modern laser technology, enabling coherent frequency conversion to remote optical bands, serving as the basis for self-referenced femtosecond lasers and quadrature-squeezed light…

Optics · Physics 2025-12-10 Nikolai Kuznetsov , Zihan Li , Tobias J. Kippenberg

The enhanced electric field at plasmonic resonances in nanoscale antennas can lead to efficient harmonic generation, especially when the plasmonic geometry is asymmetric on either inter-particle or intra-particle levels. The planar…

The generation of high-order harmonics in bulk solids subjected to intense ultrashort laser pulses has opened up new avenues for research in extreme nonlinear optics and light-matter interaction on sub-cycle timescales. Despite significant…

On the basis of the Edward-Kornfeld formulation, we study the effective susceptibility of secondharmonic generation (SHG) in colloidal crystals, which are made of graded metallodielectric nanoparticles with an intrinsic SHG susceptibility…

Optics · Physics 2008-03-24 J. P. Huang , Y. C. Jian , C. Z. Fan , K. W. Yu

High-harmonic generation by a highly non-linear interaction of infrared laser fields with matter allows for the generation of attosecond pulses in the XUV spectral regime. This process, well established for atoms, has been recently extended…

We study parametric interactions in a new type of nonlinear photonic structures, which is realized in the vicinity of a pair of nonlinear crystals. In this kind of structure, which we call binary, multiple nonlinear optical processes can be…

Optics · Physics 2016-12-21 M. Yu. Saygin , A. S. Chirkin

Parametric nonlinear optical processes are instrumental in optical quantum technology for generating entangled light. However, the range of materials conventionally used for producing entangled photons is limited. Metal-organic frameworks…

Optics · Physics 2023-11-30 Simón Paiva , Ruben A. Fritz , Sanoj Raj , Yamil J. Colón , Felipe Herrera

We show that the divergence of extreme ultraviolet pulses from high harmonic generation, which is directly linked to the shape and size of the refocused beam, can be controlled by the relative delay between the fundamental and its intense…

The ferroelectric nematic phase (N$_{\text{F}}$) has quickly become the most studied system in liquid crystal research. In this work, we investigate the origin of such polar structure by studying a compound for which the N$_{\text{F}}$…

Soft Condensed Matter · Physics 2024-11-14 Aitor Erkoreka , Nerea Sebastián , Alenka Mertelj , Josu Martinez-Perdiguero

We study nonlinear effects in two-dimensional photonic metasurfaces supporting topologically-protected helical edge states at the nanoscale. We observe strong third-harmonic generation mediated by optical nonlinearities boosted by…

We theoretically and experimentally investigate type II second harmonic generation in III-V-on-insulator wire waveguides. We show that the propagation direction plays a crucial role and that longitudinal field components can be leveraged…