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The Landau Zener model has recently been used to measure very small tunnel splittings in molecular clusters of Fe8, which at low temperature behaves like a nanomagnet with a spin ground state of S = 10. The observed oscillations of the…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 W. Wernsdorfer , I. Chiorescu , R. Sessoli , D. Gatteschi , D. Mailly

The Landau Zener method allows to measure very small tunnel splittings \Delta in molecular clusters Fe_8. The observed oscillations of \Delta as a function of the magnetic field applied along the hard anisotropy axis are explained in terms…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 W. Wernsdorfer , R. Sessoli , A. Caneschi , D. Gatteschi , A. Cornia

Ramsey et al. [Nature Phys. 4, 277-281 (2008)] report the observation of quantum interference associated with tunnelling trajectories between states of different total spin length in a dimeric molecular nanomagnet. They argue that the…

Mesoscale and Nanoscale Physics · Physics 2008-07-07 W. Wernsdorfer

A Mn4 single-molecule magnet (SMM), with a well isolated spin ground state of S = 9/2, is used as a model system to study Landau-Zener (LZ) tunneling in the presence of weak intermolecular dipolar and exchange interactions. The anisotropy…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 W. Wernsdorfer , S. Bhaduri , A. Vinslava , G. Christou

The tunnel splitting in biaxial antiferromagnetic particles is studied with a magnetic field applied along the hard anisotropy axis. We observe the oscillation of tunnel splitting as a function of the magnetic field due to the quantum phase…

Condensed Matter · Physics 2019-08-17 Yi-Hang Nie , Yan-Hong Jin , J. -Q. Liang , H. J. W. Müller-Kirsten , D. K. Park , F. -C. Pu

Magnetization measurements of Mn12 molecular nanomagnets with spin ground states of S = 10 and S = 19/2 showresonance tunneling at avoided energy level crossings. The observed oscillations of the tunnel probability as a function of the…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 W. Wernsdorfer , N. E. Chakov , G. Christou

Quantum phase interference and spin-parity effects are studied in biaxial molecular magnets in a magnetic field at an arbitrarily directed angle. The calculations of the ground-state tunnel splitting are performed on the basis of the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Hui Hu , Jia-Lin Zhu , Rong Lu , Jia-Jiong Xiong

We study spin tunneling in magnetic molecules, with special reference to Fe8. The article aims to give a pedagogical discussion of what is meant by the tunneling of a spin, and how tunneling amplitudes or energy level splittings may be…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Anupam Garg

Renormalized tunnel splitting with a finite distribution in the biaxial spin model for molecular magnets is obtained by taking into account the dipolar interaction of enviromental spins. Oscillation of the resonant tunnel splitting with a…

Strongly Correlated Electrons · Physics 2009-11-07 Zhi-De Chen , J. -Q. Liang , Shun-Qing Shen

Two antiferromagnetically coupled tunneling systems is a minimal model exhibiting the effect of quantum-mechanical phase in the Landau-Zener effect. It is shown that the averaged staying probability oscillates vs resonance shift between the…

Statistical Mechanics · Physics 2007-05-23 D. A. Garanin

Magnetization measurements of a molecular clusters Mn12 with a spin ground state of S = 10 show resonance tunneling at avoided energy level crossings. The observed oscillations of the tunnel probability as a function of the magnetic field…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 W. Wernsdorfer , M. Soler , G. Christou , D. N. Hendrickson

The tunneling splitting in biaxial ferrimagnetic particles at excited states with an explicit calculation of the prefactor of exponent is obtained in terms of periodic instantons which are responsible for tunneling at excited states and is…

Condensed Matter · Physics 2019-08-17 Yi-Hang Nie , Yan-Hong Jin , J. -Q Liang , F. -C Pu

Single-molecule magnets facilitate the study of quantum tunneling of magnetization at the mesoscopic level. The spin-parity effect is among the fundamental predictions that have yet to be clearly observed. It is predicted that quantum…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 W. Wernsdorfer , S. Bhaduri , C. Boskovic , G. Christou , D. N. Hendrickson

Quantum-mechanical systems having two discrete energy levels are ubiquitous in nature. For crossing energy levels, depending on how fast they approach each other, there is a possibility of a transition between them. This phenomenon is known…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 Mika Sillanpaa , Teijo Lehtinen , Antti Paila , Yuriy Makhlin , Pertti Hakonen

We generalize the Landau-Zener theory of coherent tunneling transitions by taking thermal relaxation into account. The evaluation of a new generalized master equation containing a dynamic tunneling rate that includes the interaction between…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Michael N. Leuenberger , Daniel Loss

Magnetic relaxation in molecular magnets under a sweeping field is studied by taking into account local stray fields. It is found that the randomness of local stray field leads to a distribution of the relaxation rate which subsequently…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Z. D. Chen , S. Q. Shen

A multi-terminal device based on a carbon nanotube quantum dot was used at very low tem- perature to probe a single electronic and nuclear spin embedded in a bis-phthalocyanine Terbium (III) complex (TbPc2). A spin-valve signature with…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 Matias Urdampilleta , Svetlana Klyatskaya , Mario Ruben , Wolfgang Wernsdorfer

We study Landau-Zener macroscopic quantum transitions in ferromagnetic metal nanoparticles containing on the order of 100 atoms. The model that we consider is described by an effective giant-spin Hamiltonian, with a coupling to a random…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 V. G. Benza , C. M. Canali , G. Strini

A Landau-Zener multi-crossing method has been used to investigate the tunnel splittings in high quality Mn$_{12}$-acetate single crystals in the pure quantum relaxation regime and for fields applied parallel to the magnetic easy axis. With…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 E. del Barco , A. D. Kent , E. M. Rumberger , D. N. Hendrickson , G. Christou

A quantum Hall system which is divided into two laterally coupled subsystems by means of a tunneling barrier exhibits a complex Landau level dispersion. Magnetotunneling spectroscopy is employed to investigate the small energy gaps which…

Mesoscale and Nanoscale Physics · Physics 2008-02-05 Matthias Habl , Werner Wegscheider
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