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Text-book concepts of diffusion- versus kinetic-control are well-defined for reaction-kinetics involving macroscopic concentrations of diffusive reactants that are adequately described by rate-constants -- the inverse of the…

Chemical Physics · Physics 2019-11-05 Denis S. Grebenkov , Ralf Metzler , Gleb Oshanin

We study a hierarchy of directed percolation (DP) processes for particle species A, B, ..., unidirectionally coupled via the reactions A -> B, ... When the DP critical points at all levels coincide, multicritical behavior emerges, with…

Statistical Mechanics · Physics 2009-10-30 Uwe C. Täuber , Martin J. Howard , Haye Hinrichsen

Steric or attractive interactions among reactants or between reactants and inert crowders can substantially influence the total rate of a diffusion-influenced reaction in the liquid phase. However, the role of the product species, that has…

Chemical Physics · Physics 2018-04-19 Rafael Roa , Toni Siegl , Won Kyu Kim , Joachim Dzubiella

We consider a $4\times4$ nonlinear reaction-diffusion system posed on a smooth domain $\Omega$ of $\mathbb{R}^N$ ($N \geq 1$) with controls localized in some arbitrary nonempty open subset $\omega$ of the domain $\Omega$. This system is a…

Optimization and Control · Mathematics 2018-08-09 Kévin Le Balc'h

We report an experimental approach to control the position of molecular aggregates on surfaces by vacuum deposition. The control is accomplished by regulating the molecular density on the surface in a confined area. The diffusing molecules…

Chemical Physics · Physics 2016-05-13 Hong Wang , Oleg Buller , Wenchong Wang , Andreas Heuer , Dequin Zhang , Harald Fuchs , Lifeng Chi

We review the milestones in the century-long development of the theory of diffusion-controlled reactions. Starting from the seminal work by von Smoluchowski who recognized the importance of diffusion in chemical reactions, we discuss…

Chemical Physics · Physics 2025-07-15 Denis S. Grebenkov

We report on the linear viscoelastic properties of mixtures comprising multiarm star (as model soft colloids) and long linear chain homopolymers in a good solvent. In contrast to earlier works, we investigated symmetric mixtures (with a…

Soft Condensed Matter · Physics 2020-07-01 Daniele Parisi , Domenico Truzzolillo , Vishnu D. Deepak , Mario Gauthier , Dimitris Vlassopoulos

Adsorption of dimers is modelled using random sequential adsorption algorithm. The interaction between molecules is given by screened electrostatic potential. The paper focuses on the properties of adsorbed monolayers as well as the…

Materials Science · Physics 2013-05-14 Michal Ciesla , Jakub Barbasz

Stochastic chemical systems with diffusion are modeled with a reaction-diffusion master equation. On a macroscopic level, the governing equation is a reaction-diffusion equation for the averages of the chemical species. On a mesoscopic…

Numerical Analysis · Mathematics 2009-03-06 Stefan Engblom , Lars Ferm , Andreas Hellander , Per Lötstedt

Diffusion is often accompanied by a reaction or sorption which can induce temperature inhomogeneities. Monte Carlo simulations of Lennard-Jones atoms in zeolite NaCaA are reported with a hot zone presumed to be created by a reaction. Our…

Statistical Mechanics · Physics 2019-05-15 A. V. Anil Kumar , S. Yashonath , G. Ananthakrishna

We consider the stability of position control of traveling waves in reaction-diffusion system as proposed in {[}J. L\"ober, H. Engel, arXiv:1304.2327{]}. Instead of analyzing the controlled reaction-diffusion system, stability is studied on…

Pattern Formation and Solitons · Physics 2014-06-16 Jakob Löber

Diffusion mediated reaction models are particularly ubiquitous in the description of physical, chemical or biological processes. The random walk schema is a useful tool for formulating these models. Recently, evanescent random walk models…

Data Analysis, Statistics and Probability · Physics 2015-10-08 Miguel A. Ré , Natalia C. Bustos

Diffusion-limited association reactions are ubiquitous in nature. They are particularly important for biological reactions, where the reaction rates are often determined by the diffusive transport of the molecules on two-dimensional…

Soft Condensed Matter · Physics 2020-10-06 Sumantra Sarkar

The statistics of equally weighted random paths (ideal polymer) is studied in $2$ and $3$ dimensional percolating clusters. This is equivalent to diffusion in the presence of a trapping environment. The number of $N$ step walks follows a…

Condensed Matter · Physics 2009-10-22 Achille Giacometti , Amos Maritan

We study a model for unimolecular reaction on a supported catalyst including reactant diffusion and desorption, using analytical methods and scaling concepts. For rapid reactions, enhancing surface diffusion or increasing particle size…

Statistical Mechanics · Physics 2009-06-18 T. G. Mattos , Fabio D. A. Aarao Reis

The reversible A <-> B reaction-diffusion process, when species A and B are initially mixed and diffuse with different diffusion coefficients, is investigated using the boundary layer function method. It is assumed that the ratio of the…

Statistical Mechanics · Physics 2008-10-22 M. Sinder , V. Sokolovsky , J. Pelleg

The effect of turbulence on the heterogeneous (solid-fluid) reactions of solid particles is studied numerically with Direct Numerical Simulations (DNS). A simplified reaction system is used, where the solid-fluid reaction is represented by…

Fluid Dynamics · Physics 2016-07-14 Jonas Krüger , Nils E. L. Haugen , Dhrubaditya Mitra , Terese Løvås

We show that, for any spatially discretized system of reaction-diffusion, the approximate solution given by the explicit Euler time-discretization scheme converges to the exact time-continuous solution, provided that diffusion coefficient…

Optimization and Control · Mathematics 2019-12-12 Adrien Le Coënt , Laurent Fribourg

We study the dynamics of an ideal polymer chain in a crowded, viscoelastic medium and in the presence of active forces. The motion of the centre of mass and of individual monomers is calculated. On time scales that are comparable to the…

Soft Condensed Matter · Physics 2015-12-23 Hans Vandebroek , Carlo Vanderzande

We analyze the statistics of loops formation in $f$-branched star polymers in an environment with structural defects, correlated at large distances $r$ according to a power law $\sim r^{-a}$. Applying the direct polymer renormalization…

Soft Condensed Matter · Physics 2017-10-04 K. Haydukivska , V. Blavatska