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We stress that the so-called butterfly hysteresis curves observed in dynamical magnetization measurements on systems of low-spin magnetic molecules such as V-15 and V-6 are a signature of adiabatic Landau-Zener transitions rather than that…

Statistical Mechanics · Physics 2008-05-05 Mark Vogelsberger , D. A. Garanin , Rolf Schilling

The V_{15} polyoxovanadate molecule is made of 15 spins 1/2 with antiferromagnetic couplings. It belongs to the class of molecules with very large Hilbert space dimension (2^{15} in V_{15}, 10^8 in Mn_{12}-ac). It is a low-spin/big-molecule…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 I. Chiorescu , W. Wernsdorfer , A. Müller , H. Bögge , B. Barbara

The so-called V15 molecule is formed of 15 spins 1/2 antiferromagnetically coupled. The resultant spin is equal to 1/2. Contrary to what is expected at first sight, this half-integer spin is gapped. We show that this is a consequence of the…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 B. Barbara , I. Chiorescu , W. Wernsdorfer , H. Boegge , A. Mueller

Starting from an antiferromagnetic Heisenberg Hamiltonian for the fifteen spin-1/2 ions in V_15, we construct an effective spin Hamiltonian involving eight low-lying states (spin-1/2 and spin-3/2) coupled to a phonon bath. We numerically…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Indranil Rudra , S. Ramasesha , Diptiman Sen

(Et4N)3Fe2F9 exhibits a butterfly--shaped hysteresis below 5 K when the magnetic field is parallel to the threefold axis, in accordance with a very slow magnetization relaxation in the timescale of minutes. This is attributed to an energy…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Ralph Schenker , Michael N. Leuenberger , Gregory Chaboussant , Hans U. Guedel

The ruthenium based molecular magnet [Ru$_2$(D(3,5-Cl$_2$Ph)F)$_4$Cl(0.5H$_2$O)$\cdotp$C$_6$H$_{14}$] (hereafter Ru$_2$) behaves as a two-level system at sufficiently low temperatures. The authors performed spin detection by means of…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 L. Chen , C. M. Ramsey , N. S. Dalal , T. Ren , F. A. Cotton , W. Wernsdorfer , I. Chiorescu

A characteristic of spin reversal in the presence of phonon-bottleneck is the deviation of the magnetization cycle from a reversible function into an opened hysterezis cycle. In recent experiments on molecular magnets (e.g. V$_{15}$ and…

Mesoscale and Nanoscale Physics · Physics 2009-09-28 L. Chen , I. Chiorescu

At low temperatures, the magnetization of the molecular ferric wheel NaFe$_6$ exhibits a step at a critical field $B_c$ due to a field-induced level-crossing. By means of high-field torque magnetometry we observed a hysteretic behavior at…

Strongly Correlated Electrons · Physics 2009-11-07 O. Waldmann , R. Koch , S. Schromm , P. Müller , I. Bernt , R. W. Saalfrank

A detailed investigation of the unusual dynamics of the magnetization of (Et4N)3Fe2F9 (Fe2), containing isolated [Fe2F9]3- dimers, is presented and discussed. Fe2 possesses an S=5 ground state with an energy barrier of 2.40 K due to an…

Strongly Correlated Electrons · Physics 2009-11-11 Ralph Schenker , Michael N. Leuenberger , Gregory Chaboussant , Daniel Loss , Hans U. Gudel

Quasi-static hysteresis loops of spherical and spheroidal magnetite nanoparticles with semi-axes ratio a/b = 1.5 and 2.0 with different types of combined magnetic anisotropy are calculated using numerical simulation. For particles of each…

Mesoscale and Nanoscale Physics · Physics 2024-05-07 N. A. Usov , O. N. Serebryakova

We study the emergence of hysteresis during the process of quantum phase transition from an antiferromagnetic to a phase-separated state in a spin-1 Bose Einstein condensate of ultracold atoms. We explicitly demonstrate the appearance of a…

Quantum Gases · Physics 2018-04-04 Tomasz Swisłocki , Andrzej Zembrzuski , Michał Matuszewski , Emilia Witkowska

We have observed hysteresis loops and abrupt magnetization steps in the magnetic molecule V$_6$, where each molecule comprises a pair of identical spin triangles, in the temperature range 1-5 K for external magnetic fields $B$ with sweep…

Other Condensed Matter · Physics 2008-03-28 I. Rousochatzakis , Y. Ajiro , H. Mitamura , P. Kögerler , M. Luban

We present muon spin lattice relaxation measurements in the V15 spin 1/2 molecular nano-magnet. We find that the relaxation rate in low magnetic fields (<5 kG) is temperature independent below ~10 K, implying that the molecular spin is…

Mesoscale and Nanoscale Physics · Physics 2008-08-28 Z. Salman , R. F. Kiefl , K. H. Chow , W. A. MacFarlane , T. Keeler , T. Parolin , S. Tabbara , D. Wang

We explore the hysteretic dynamics of spinor Bose-Einstein condensates of ultracold atoms loaded in static 2D ring geometries and subjected to varying synthetic magnetic fields. Electrically neutral, pseudo-spin-$1/2$ condensates are probed…

Quantum Gases · Physics 2024-08-09 Shuji Jia , Jintao Xu , Qian Jia , Haibo Qiu , Antonio Muñoz Mateo

This article addresses a problem of micromagnetics: the reversal of magnetic moments in layered spring magnets. A one-dimensional model is used of a film consisting of several atomic layers of a soft material on top of several atomic layers…

Dynamical Systems · Mathematics 2025-10-20 J. Samuel Jiang , Hans G. Kaper , Gary K. Leaf

The spin one half molecular system V15 shows no barrier against spin reversal. This makes possible direct phonon activation between the two levels. By tuning the field sweeping rate and the thermal coupling between sample and thermal…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 I. Chiorescu , W. Wernsdorfer , A. Mueller , S. Miyashita , B. Barbara

We develop a phenomenological model to study magnetic hysteresis in two samples designed as possible perpendicular recording media. A stochastic cellular automata model captures cooperative behavior in the nucleation of magnetic domains. We…

We study the motion of a charged quantum particle, constrained on the surface of a cylinder, in the presence of a radial magnetic field. When the spin of the particle is neglected, the system essentially reduces to an infinite family of…

Quantum Physics · Physics 2007-05-23 C. Chryssomalakos , A. Franco , A. Reyes-Coronado

Formation of a magnetic hysteresis loop with respect to a bias voltage is investigated theoretically in a spin-valve device based on a single magnetic molecule. We consider a device consisting of two ferromagnetic electrodes bridged by a…

Mesoscale and Nanoscale Physics · Physics 2018-05-09 Anna Płomińska , Maciej Misiorny , Ireneusz Weymann

The magnetization reversal in a single molecular magnet (SMM) weakly coupled to an electrode with spin-dependent splitting of chemical potentials (spin bias) is theoretically investigated by means of the rate equation. A microscopic…

Mesoscale and Nanoscale Physics · Physics 2009-05-14 Hai-Zhou Lu , Bin Zhou , Shun-Qing Shen
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