Related papers: Many-Spin Effects and Tunneling Properties of Magn…
We calculate the tunneling splittings in a Mn$_{12}$ magnetic molecule taking into account its internal many-spin structure. We discuss the precision and reliability of these calculations and show that restricting the basis (limiting the…
The tunneling of a giant spin at excited levels is studied theoretically in mesoscopic magnets with a magnetic field at an arbitrary angle in the easy plane. Different structures of the tunneling barriers can be generated by the…
The tunneling splitting of the energy levels of a ferromagnetic particle in the presence of an applied magnetic field - previously derived only for the ground state with the path integral method - is obtained in a simple way from…
The phenomenon of Quantum Tunneling of Mesoscopic Spins is reviewed in the light of the behavior of the archetype of these systems: the molecular complex Mn12-ac. Most observations can be understood in the framework of the reduced Hilbert…
This thesis contains a thorough investigation of the quantum spin dynamics in Mn12-ac and Mn6 Single-molecule magnets. In particular, we have investigated the interplay between quantum tunneling of magnetization and nuclear spin dynamics in…
Quantum phase interference and spin-parity effects are studied in biaxial molecular magnets in a magnetic field at an arbitrarily directed angle. The calculations of the ground-state tunnel splitting are performed on the basis of the…
This article takes a broad view of the understanding of magnetic bistability and magnetic quantum tunneling in single-molecule magnets (SMMs), focusing on three families of relatively simple, low-nuclearity transition metal clusters: spin S…
Magnetization measurements of Mn12 molecular nanomagnets with spin ground states of S = 10 and S = 19/2 showresonance tunneling at avoided energy level crossings. The observed oscillations of the tunnel probability as a function of the…
We consider tunneling transport through a Mn$_{12}$ molecular magnet using spin density functional theory. A tractable methodology for constructing many-body wavefunctions from Kohn-Sham orbitals allows for the determination of…
We review the present state of theory and experiments on the quantum tunneling of magnetization in mesoscopic spin systems. Most attention is paid to the relaxation of magnetization in the molecular complexes Mn12 and Fe8. The role of the…
The manipulation of single magnetic molecules may enable new strategies for high-density information storage and quantum-state control. However, progress in these areas depends on developing techniques for addressing individual molecules…
The ground states of artificial molecules made of two vertically coupled quantum rings are studied within the spin density functional theory for systems containing up to 13 electrons. Quantum tunneling effects on the electronic structure of…
We study tunneling of the magnetic moment in a particle that has full rotational freedom. Exact energy levels are obtained and the ground-state magnetic moment is computed for a symmetric rotor. The effect of the mechanical freedom on spin…
The synthesis of molecular magnets has undergone rapid progress in recent years. Each of the identical molecular units can contain as few as two and up to several dozens of paramagnetic ions (spins). Although these materials appear as…
We study spin tunneling in magnetic molecules, with special reference to Fe8. The article aims to give a pedagogical discussion of what is meant by the tunneling of a spin, and how tunneling amplitudes or energy level splittings may be…
We investigate the magnetic properties of three Mn$_6$ single molecule magnets by means of inelastic neutron scattering and frequency domain magnetic resonance spectroscopy. The experimental data reveal that small structural distortions of…
Many molecular magnetic clusters, such as single-molecule magnets, are characterized by spin ground states with defined total spin S exhibiting zero-field-splittings. In this work, the spectroscopic intensities of the transitions within the…
We report spin-pair tunneling observed in Mn$_3$ single-molecule magnet, which is a crystal with 2D network of identical exchange coupling. We observed a series of extra quantum tunnelings by the ac susceptibility measurements, and…
It is shown that a single molecular magnet placed in a rapidly oscillating magnetic field displays the phenomenon of quenching of tunneling processes. The results open a way to manipulate the quantum states of molecular magnets by means of…
The level splitting formulae much discussed in the study of spin tunneling in macroscopic ferromagnetic particles and previously derived only by complicated pseudoparticle methods for the ground state, are derived from those of eigenvalues…