Related papers: Oscillatory Tunnel Splittings in Spin Systems: A D…
A discrete version of the WKB method is developed and applied to calculate the tunnel splittings between classically degenerate states of spin Hamiltonians. The results for particular model problems are in complete accord with those…
We study spin tunneling in magnetic molecules, with special reference to Fe8. The article aims to give a pedagogical discussion of what is meant by the tunneling of a spin, and how tunneling amplitudes or energy level splittings may be…
Spin tunneling in the particular case of the magnetic molecular cluster octanuclear iron(III), Fe8, is treated by an effective Hamiltonian that allows for an angle-based description of the process. The presence of an external magnetic field…
We study spin tunnelling in molecular magnets as an instance of a mesoscopic phenomenon, with special emphasis on the molecule Fe8. We show that the tunnel splitting between various pairs of Zeeman levels in this molecule oscillates as a…
The spin Hamiltonian that describes the molecular magnet Fe$_8$ has biaxial symmetry with mutually perpendicular easy, medium, and hard magnetic axes. Previous calculations of the ground state tunnel splittings in the presence of a magnetic…
The perfect quenching of spin tunneling that has previously been discussed in terms of interfering instantons, and has recently been observed in the magnetic molecule \Fe8, is treated using a discrete phase integral (or…
The ground state tunnel splitting for the biaxial spin model in the magnetic field, H = -D S_{x}^2 + E S_{z}^2 - g \mu_B S_z H_z, has been investigated using an instanton approach. We find a new type of spin instanton and a new quantum…
We have investigated analytically quantum tunneling of large spin in the biaxial spin system with the magnetic field applied along the hard and medium anisotropy axes by using a purely quantum-mechanical approach. When the magnetic field…
Quantum phase interference and spin-parity effects are studied in biaxial molecular magnets in a magnetic field at an arbitrarily directed angle. The calculations of the ground-state tunnel splitting are performed on the basis of the…
The double-well potential is a good example, where we can compute the splitting in the bound state energy of the system due to the tunneling effect with various methods, namely WKB or instanton calculations. All these methods are…
The study of tunneling splitting is fundamental to get insight into the dynamics of a multitude of molecular systems. In this paper, a novel approach to the analysis of the ground-state tunneling splitting is presented and explicitly…
The perfect quenching of spin tunneling first predicted for a model with biaxial symmetry, and recently observed in the magnetic molecule Fe_8, is further studied using the discrete phase integral (or Wentzel-Kramers-Brillouin) method. The…
The oscillation of tunnel splitting in the biaxial spin system within magnetic field along the anisotropy axis is analyzed within the particle mapping approach, rather than in the (\theta-\phi) spin coherent-state representation. In our…
Spin coherent state path integrals with discontinuous semiclassical paths are investigated with special reference to a realistic model for the magnetic degrees of freedom in the Fe8 molecular solid. It is shown that such paths are essential…
A formalism is developed to study certain five-term recursion relations by discrete phase integral (or Wentzel-Kramers-Brillouin) methods. Such recursion relations arise naturally in the study of the Schrodinger equation for certain spin…
Starting from a phenomenological Hamiltonian originally written in terms of angular momentum operators we derive a new quantum angle-based Hamiltonian that allows for a discussion on the quantum spin tunneling. The study of the…
Discrete quantum phase space formalism is used to discuss some basic aspects of the spin tunneling occurring in Fe8 magnetic cluster by means of Wigner functions as well as Husimi distributions. Those functions were obtained for sharp angle…
The tunneling splitting in biaxial ferrimagnetic particles at excited states with an explicit calculation of the prefactor of exponent is obtained in terms of periodic instantons which are responsible for tunneling at excited states and is…
A discrete WKB method is developed for calculating tunnel splittings in spin problems. The method is then applied to the issue of how nuclear spins affect the macroscopic quantum coherence of the total magnetic moment in small magnetic…
We use an instanton approximation to the continuous-time spin coherent-state path integral to obtain the tunnel splitting of classically degenerate ground states. We show that provided the fluctuation determinant is carefully evaluated, the…