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The charge and orbital ordering in Pr_{0.5} Ca_{0.5} MnO_3 is studied for the first time by ^{17}O NMR. This local probe is sensitive to spin, charge and orbital correlations. Two transitions exist in this system: the charge and orbital…

Strongly Correlated Electrons · Physics 2009-11-07 A. Yakubovskii , A. Trokiner , S. Verkhovskii , A. Gerashenko , D. Khomskii

We present the results of a systematic x-ray scattering study of the charge and orbital ordering in the manganite series Pr$_{1-x}$Ca$_x$MnO$_3$ with $x$=0.25, 0.4 and 0.5. The temperature dependence of the scattering at the charge and…

Strongly Correlated Electrons · Physics 2009-10-31 M. v. Zimmermann , C. S. Nelson , J. P. Hill , Doon Gibbs , M. Blume , D. Casa , B. Keimer , Y. Murakami , C. -C. Kao , C. Venkataraman , T. Gog , Y. Tomioka , Y. Tokura

In the manganite Nd0.5Ca0.5MnO3, charge ordering occurs at much higher temperature than the antiferromagnetic order (TCO=250K,TN=160K). The magnetic behavior of the phase TN<T<TCO is puzzling: its magnetization and susceptibility are…

Strongly Correlated Electrons · Physics 2016-08-31 F. millange , S. de Brion , G. Chouteau

The phase diagram of $Pr_{1-x}Ca_xMnO_3$ is modified x $\le$ 0.3, which suggests a reevaluation of the phase diagram of other manganites in that doping region. Rather than an orbital ordered phase reaching up to high temperatures of…

We review our recent x-ray scattering studies of charge and orbital order in doped manganites, with specific emphasis on the role of orbital correlations in Pr_1-xCa_xMnO_3. For x=0.25, we find an orbital structure indistinguishable from…

In the present work we analyze the influence of the charge-ordering on the magnetocaloric effect of Pr$_{1-x}$Ca$_x$MnO$_3$ manganites. The results for the samples with $x<$0.30 present the usual ferromagnetic behavior, peaking at the Curie…

Materials Science · Physics 2007-05-23 M. S. Reis , V. S. Amaral , J. P. Araujo , P. B. Tavares , A. M. Gomes , I. S. Oliveira

We report resonant x-ray scattering data of the orbital and magnetic ordering at low temperatures at the Mn $L_{\rm 2,3}$ edges in \lsmo. The orderings display complex energy features close to the Mn absorption edges. Systematic modeling…

To sum up, we show in the present paper that magnetic response in Nb$_2$O$_2$F$_3$ at the high-temperatures ($T>$90 K) is related to the orbital selective regime, when part of the electrons form molecular orbitals while other electrons have…

Materials Science · Physics 2017-05-24 V. V. Gapontsev , D. I. Khomskii , S. V. Streltsov

We investigated the temperature ($T=$ 15 $\sim $ 290 K) and the magnetic field ($H=$ 0 $\sim $ 17 T) dependent optical conductivity spectra of a charge/orbital ordered manganite, Nd$_{1/2}$Sr$_{1/2}$MnO$_3$. With variation of $T$ and $H$,…

Strongly Correlated Electrons · Physics 2009-10-31 J. H. Jung , H. J. Lee , T. W. Noh , E. J. Choi , Y. Moritomo , Y. J. Wang , X. Wei

We report coherent x-ray scattering studies of charge and orbital domains in manganite systems. The experiments were carried out on LaMnO_3 and Pr_{0.6}Ca_{0.4}MnO_3, with the incident photon energy tuned near the Mn K edge. At room…

Strongly Correlated Electrons · Physics 2009-11-07 C. S. Nelson , J. P. Hill , Doon Gibbs , F. Yakhou , F. Livet , Y. Tomioka , T. Kimura , Y. Tokura

The nature of the cooperative Jahn-Teller (JT) transition accompanied by orbital order-disorder in Nd1-xCaxMnO3 has been studied by high temperature (300 - 1200K) synchrotron and laboratory X-ray powder diffraction in the low doping region…

Materials Science · Physics 2009-11-13 C. V. Colin , A. J. C. Buurma , M. v. Zimmermann , T. T. M. Palstra

We describe neutron scattering experiments performed to investigate the magnetic order and dynamics of half-doped La1.5Sr0.5CoO4. This layered perovskite exhibits a near-ideal checkerboard pattern of Co2+/Co3+ charge order at temperatures…

Strongly Correlated Electrons · Physics 2009-10-19 L. M. Helme , A. T. Boothroyd , R. Coldea , D. Prabhakaran , C. D. Frost , D. A. Keen , L. P. Regnault , P. G. Freeman , M. Enderle , J. Kulda

The melting process of the orbital order in Pr0.5Ca0.5MnO3 single crystal has been studied in detail as a function of temperature by neutron diffraction. It is demonstrated that a commensurate-incommensurate (C-IC) transition of the orbital…

Strongly Correlated Electrons · Physics 2016-08-31 R. Kajimoto , H. Yoshizawa , Y. Tomioka , Y. Tokura

We report an x-ray scattering study of octahedral tilt ordering in the manganite series Pr$_{1-x}$Ca$_x$MnO$_3$ with x=0.4 and 0.25 and in LaMnO$_3$. The sensitivity to tilt ordering is achieved by tuning the incident x-ray energy to the…

We report low temperature specific heat measurements of Pr$_{1-x}$Ca$_{x}$MnO$_{3}$ ($0.3\leq x \leq 0.5$) and La$_{0.5}$Ca$_{0.5}$MnO$_{3}$ with and without applied magnetic field. An excess specific heat, $C^{\prime}(T)$, of non-magnetic…

Strongly Correlated Electrons · Physics 2009-10-31 V. N. Smolyaninova , Amlan Biswas , X. Zhang , K. H. Kim , Bog-Gi Kim , S-W. Cheong , R. L. Greene

Motivated by the recent ARPES measurements (Evtushinsky et. al., PRL {\bf 105}, 147201 (2010)) and evidence for the density-wave state for the charge and orbital ordering (Garc\'{i}a et al., PRL {\bf 109}, 107202 (2012)) in…

Strongly Correlated Electrons · Physics 2017-06-29 Dheeraj Kumar Singh , Tetsuya Takimoto

We report Electron Paramagnetic Resonance measurements on single crystalline and powder samples of Nd_0.5Ca_0.5MnO_3 across the charge-ordering transition at T_co=240 K down to the antiferromagnetic ordering transition at T_N = 140 K. The…

Strongly Correlated Electrons · Physics 2021-05-26 Janhavi P. Joshi , Rajeev Gupta , A. K. Sood , S. V. Bhat , A. R. Raju , C. N. R. Rao

We investigate the evolution of spin and orbital order in undoped LaMnO$_3$ under increasing temperature with a model including both superexchange and Jahn-Teller interactions. We used several cluster mean field calculation schemes and find…

Strongly Correlated Electrons · Physics 2016-12-26 Mateusz Snamina , Andrzej M. Oleś

It is argued that both transitions observed in 50%-doped manganites, at the N\'{e}el temperature ($T_{\rm N}$) and the so-called charge ordering temperature ($T_{\rm CO}$), are magnetic. $T_{\rm N}$ corresponds to the order-disorder…

Strongly Correlated Electrons · Physics 2007-05-23 I. V. Solovyev

In a recent published paper [Phys. Rev. B 64, 195133 (2001)], Zimmermann et al. present a systematic x-ray scattering study of charge and orbital ordering phenomena in the Pr1-xCaxMnO3 series with x= 0.25, 0.4 and 0.5. They propose that for…

Strongly Correlated Electrons · Physics 2009-11-10 Joaquin Garcia , Gloria Subias
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