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The ionic composition and pair correlations in fluid phases of realistically salt-free charged colloidal sphere suspensions are calculated in the primitive model. We obtain the number densities of all ionic species in suspension, including…

Soft Condensed Matter · Physics 2014-03-28 Marco Heinen , Thomas Palberg , Hartmut Löwen

Recent experiments show a strong rotational-diffusion enhancement for self-propelled microrheological probes in colloidal glasses. Here, we provide microscopic understanding using simulations with a frictional probe-medium coupling that…

Soft Condensed Matter · Physics 2020-12-22 Clara Abaurrea-Velasco , Celia Lozano , Clemens Bechinger , Joost de Graaf

Monte Carlo simulations have been performed for aqueous charged colloidal suspensions as a function of charge density on the particles and salt concentration. We vary the charge density in our simulations over a range where a reentrant…

Soft Condensed Matter · Physics 2007-05-23 P. S. Mohanty , B. V. R. Tata

This paper adopts a previously developed activation model of shear thickening, published by the authors, to sterically stabilized colloidal suspensions. When particles arranged along the compression axis of a sheared suspension, they may…

Soft Condensed Matter · Physics 2012-07-12 Joachim Kaldasch , Bernhard Senge

We propose a numerical method to simulate electrohydrodynamic phenomena in charged colloidal dispersions. This method enables us to compute the time evolutions of colloidal particles, ions, and host fluids simultaneously by solving Newton,…

Soft Condensed Matter · Physics 2007-05-23 Kang Kim , Yasuya Nakayama , Ryoichi Yamamoto

Using Brownian dynamics computer simulations we show that a two-dimensional suspension of self-propelled ("active") colloidal particles crystallizes at sufficiently high densities. Compared to the equilibrium freezing of passive particles…

Soft Condensed Matter · Physics 2012-06-12 Julian Bialké , Thomas Speck , Hartmut Löwen

We report experimental and computational observations of dynamic contact networks for colloidal suspensions undergoing shear thickening. The dense suspensions are comprised of sterically stabilized poly(methyl methacrylate) hard sphere…

Soft Condensed Matter · Physics 2021-10-13 Shravan Pradeep , Mohamad Nabizadeh , Alan R. Jacob , Safa Jamali , Lilian C. Hsiao

Charged soft-matter systems--such as colloidal dispersions and charged polymers--are dominated by attractive forces between constituent like-charged particles when neutralizing counterions of high charge valency are introduced. Such…

Soft Condensed Matter · Physics 2009-11-11 Ali Naji , Swetlana Jungblut , Andre G. Moreira , Roland R. Netz

In this paper, some equations are derived to describe the out-of-equilibrium thermodynamics of colloidal suspensions. These results are obtained assuming that the properties of the colloids essentially come from their surfaces which are…

Soft Condensed Matter · Physics 2013-03-29 Pierre de Thier

The present review summarizes and assesses recent theoretical and experimental advances, with special emphasis on the effective interaction between charge-stabilized colloids, in the bulk or in confined geometries, and on the ambiguities of…

Soft Condensed Matter · Physics 2015-06-24 J. -P. Hansen , H. Lowen

We explore the effects of counterion condensation on fluid-fluid phase separation in charged colloidal suspensions. It is found that formation of double layers around the colloidal particles stabilizes suspensions against phase separation.…

Soft Condensed Matter · Physics 2009-10-31 Alexandre Diehl , Marcia C. Barbosa , Yan Levin

We study the hydrodynamic interactions between colloids suspended in a compressible fluid inside a rigid channel. Using lattice-Boltzmann simulations and a simplified hydrodynamic theory, we find that the diffusive dynamics of density…

Soft Condensed Matter · Physics 2013-02-13 Derek Frydel , Haim Diamant

We present a computer simulation study on the crystal nucleation process in suspensions of hard spheres, fully taking into account the solvent hydrodynamics. If the dynamics of collodial crystallization were purely diffusive, the crystal…

Soft Condensed Matter · Physics 2015-06-12 Marc Radu , Tanja Schilling

We studied the self-diffusion of colloidal ellipsoids in a monolayer near a flat wall by video microscopy. The image processing algorithm can track the positions and orientations of ellipsoids with sub-pixel resolution. The translational…

Soft Condensed Matter · Physics 2015-05-19 Zhongyu Zheng , Yilong Han

We employ a novel Monte Carlo simulation scheme to elucidate the stabilization of neutral colloidal microspheres by means of highly-charged nanoparticles [V. Tohver et al., Proc. Natl. Acad. Sci. U.S.A. 98, 8950 (2001)]. In accordance with…

Soft Condensed Matter · Physics 2009-11-10 Jiwen Liu , Erik Luijten

Thermally induced particle flow in a charged colloidal suspension is studied in a fluid-mechanical approach. The force density acting on the charged boundary layer is derived in detail. From Stokes' equation with no-slip boundary conditions…

Soft Condensed Matter · Physics 2014-01-31 S. Fayolle , T. Bickel , A. Würger

A Rayleigh-Taylor-like instability of a dense colloidal layer under gravity in a capillary of microfluidic dimensions is considered. We access all relevant lengthscales with particle-level microscopy and computer simulations which…

Experimental studies of the variation of the mean square displacement (MSD) of a particle in a confined colloid suspension that exhibits density variations on the scale length of the particle diameter are not in agreement with the…

Soft Condensed Matter · Physics 2018-06-13 Molly Wolfson , Christopher Liepold , Binhua Lin , Stuart A. Rice

The emergence of particle irreversibility in periodically driven colloidal suspensions has been interpreted as resulting either from a nonequilibrium phase transition to an absorbing state or from the chaotic nature of particle…

Statistical Mechanics · Physics 2015-04-10 Elsen Tjhung , Ludovic Berthier

The particle diffusion in a fluid is a classical topic that dates back to more than one century ago. However, a full solution to this issue still lacks. In this work the velocity autocorrelation function and the diffusion constant are…

Fluid Dynamics · Physics 2016-08-03 Hanqing Zhao , Hong Zhao