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We propose a mean-field analytical model to account for the observed asymmetry in the ability to form long-range attraction by the negatively charged colloidal particles and not their equivalently charged positive counterpart. We conjecture…

Soft Condensed Matter · Physics 2009-11-13 William Kung , Monica Olvera de la Cruz

In classical density functional theory (DFT) the part of the Helmholtz free energy functional arising from attractive inter-particle interactions is often treated in a mean-field or van der Waals approximation. On the face of it, this is a…

Soft Condensed Matter · Physics 2017-07-25 Andrew J. Archer , Blesson Chacko , Robert Evans

Simulation of warm dense matter requires computational methods that capture both quantum and classical behavior efficiently under high-temperature, high-density conditions. Currently, density functional theory molecular dynamics is used to…

Chemical Physics · Physics 2015-10-21 Attila Cangi , Aurora Pribram-Jones

The Fermi surface is an abstract object in the reciprocal space of a crystal lattice, enclosing the set of all those electronic band states that are filled according to the Pauli principle. Its topology is dictated by the underlying lattice…

Strongly Correlated Electrons · Physics 2016-07-20 Mukunda P. Das , Frederick Green

The contact value of the charge profile for nonsymmetrical electrolytes is presented as the sum of three contributions. One of them is the normal component of the Maxwell electrostatic stress tensor. The second one is the surface…

Statistical Mechanics · Physics 2009-11-13 M. Holovko , D. di Caprio

We present an investigation of the combined effects of the Debye-Huckel (DH) repulsive and overlaping Debye spheres (ODS) attractive interaction potentials around charged dust particles on collective modes, phase separation and ordered dust…

Plasma Physics · Physics 2013-05-31 Zoltan Donko , Peter Hartmann , Padma K. Shukla

Non-covalent interactions are essential in the description of soft matter, including materials of technological importance and biological molecules. In density-functional theory, common approaches fail to describe dispersion forces, an…

Chemical Physics · Physics 2014-12-30 Gino A. DiLabio , Alberto Otero-de-la-Roza

Studies of the structural, electronic, and optical characteristics of the interfaces between graphene and ZnO polar surfaces is carried out using first-principles simulations. At the interface, a strong van der Waals force is present, and…

Materials Science · Physics 2023-05-23 H. D. Etea , K. N. Nigussa

We investigate the equilibrium properties of a colloidal solution in contact with a soft interface. As a result of symmetry breaking, surface effects are generally prevailing in confined colloidal systems. In this Letter, particular…

Statistical Mechanics · Physics 2015-06-24 Hamid Kaidi , Thomas Bickel , Mabrouk Benhamou

When two macromolecules come very near in a fluid, the surrounding molecules, having finite volume, are less likely to get in between. This leads to a pressure difference manifesting as an entropic attraction, called depletion force. Here…

Soft Condensed Matter · Physics 2020-02-26 Nathaniel Rupprecht , Dervis Can Vural

Based on fundamental measure theory, a Helmholtz free energy density functional for three-component mixtures of hard spheres with general, non-additive interaction distances is constructed. The functional constitutes a generalization of the…

Soft Condensed Matter · Physics 2011-09-28 Matthias Schmidt

Mesoscopic theory for soft-matter systems that combines density functional and statistical field theory is derived from the microscopic theory by a systematic coarse-graining procedure. Within the framework of this theory we obtain the…

Soft Condensed Matter · Physics 2013-05-29 A. Ciach

We present a continuum theory of electrolytes composed of a waterlike solvent and univalent ions. First, we start with a density functional $\cal F$ for the coarse-grained solvent, cation, and anion densities, including the Debye-H\"uckel…

Soft Condensed Matter · Physics 2020-08-20 Ryuichi Okamoto , Kenichiro Koga , Akira Onuki

Effective potential of a charged dusty particle moving in homogeneous plasma has a negative part that provides attraction between similarly charged dusty particles. A depth of this potential well is great enough to ensure both stability of…

Plasma Physics · Physics 2009-11-10 Andrei G. Bashkirov

The principles of density-functional theory are studied for finite lattice systems represented by graphs. Surprisingly, the fundamental Hohenberg-Kohn theorem is found void in general, while many insights into the topological structure of…

Quantum Physics · Physics 2022-01-13 Markus Penz , Robert van Leeuwen

We investigate effective interactions between a colloidal particle, immersed in a binary mixture of smaller spheres, and a semipermeable membrane. The colloid is modeled as a big hard sphere and the membrane is represented as an infinitely…

Soft Condensed Matter · Physics 2007-05-23 Pawel Bryk

We derive a connection between the intrinsic tribological properties and the electronic properties of a solid interface. In particular, we show that the adhesion and frictional forces are dictated by the electronic charge redistribution…

Other Condensed Matter · Physics 2018-07-17 M. Wolloch , G. Levita , P. Restuccia , M. C. Righi

We perform the analysis of predictions of a classical density functional theory for associating fluids with different association strength concerned with wetting of solid surfaces. The four associating sites water-like models with…

Soft Condensed Matter · Physics 2024-04-01 A. Kozina , M. Aguilar , O. Pizio , S. Sokołowski

The physics of an electron solid, held on a cryogenic liquid surface by a pressing electric field, is examined in a low-density regime that has not been explored before. We consider the effect of the pressing field in distorting the surface…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Masudul Haque , Indranil Paul , Sergey Pankov

We prove by means of a renormalization group method that in weakly interacting many-electron systems at half-filling on a periodic hyper-cubic lattice, the free energy density uniformly converges to an analytic function of the coupling…

Mathematical Physics · Physics 2016-12-19 Yohei Kashima