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We demonstrate that the half-doped bilayer manganite La_{1}Sr_{2}Mn_{2}O_{7} exhibits CE-type charge-ordered and spin-ordered states below $T_{N, CO}^A = 210$ K and below $T_{N}^{CE} \sim 145$ K, respectively. However, the volume fraction…

Strongly Correlated Electrons · Physics 2009-10-31 M. Kubota , H. Yoshizawa , Y. Moritomo , H. Fujioka , K. Hirota , Y. Endoh

By calculating the electronic, orbital, magnetic and lattice structure of half-doped manganites we establish the central role of oxygen buckling caused by the tilting of the MnO$_6$ octahedra -- in essence a steric effect. The buckling…

Strongly Correlated Electrons · Physics 2015-05-27 Paolo Barone , Silvia Picozzi , Jeroen van den Brink

This review will deal with several types of free charge localisation in oxides and their consequences on the effective dielectric spectra of such materials. The first one is the polaronic localisation at the unit cell scale on residual…

Materials Science · Physics 2010-06-21 Mario Maglione

A new method for analyzing second-order phase transitions is presented and applied to the polaronic system La$_{0.7}$Ca$_{0.3}$MnO$_{3}$. It utilizes heat capacity and thermal expansion data simultaneously to correctly predict the critical…

Strongly Correlated Electrons · Physics 2007-05-23 A. Souza , Yi-Kuo Yu , J. J. Neumeier , H. Terashita , R. F. Jardim

We report an inelastic neutron scattering study of acoustic phonons in the charge and orbitally ordered bilayer manganite LaSr$_2$Mn$_2$O$_7$. For excitation energies less than $15\,\rm{meV}$, we observe an abrupt increase (decrease) of the…

Strongly Correlated Electrons · Physics 2011-12-14 F. Weber , S. Rosenkranz , J. -P. Castellan , R. Osborn , H. Zheng , J. F. Mitchell , Y. Chen , Songxue Chi , J. W. Lynn , D. Reznik

Single crystalline (Bi,Ca)MnO3 (74< %Ca <82) were studied with neutron scattering, electron diffraction and bulk magnetic measurement. We discovered dynamic ferromagnetic spin correlations at high temperatures, which are replaced by…

Strongly Correlated Electrons · Physics 2009-10-28 Wei Bao , J. D. Axe , C. H. Chen , S-W. Cheong

Taking the orbital degeneracy of $e_g$ conduction bands and the Coulomb interaction into account in a double-exchange model, we investigate charge dynamics of perovskite Mn oxides by the Lancz$\ddot{\rm o}$s diagonalization method. In the…

Strongly Correlated Electrons · Physics 2009-10-31 Hiroki Nakano , Yukitoshi Motome , Masatoshi Imada

We present a femtosecond optical pump-probe study of the multiferroic manganite Eu$_{0.75}$Y$_{0.25}$MnO$_3$. The optical response of the material at pump energies of 1.55 and 3.1 eV is dominated by the $d$-$d$ and $p$-$d$ transitions of…

We use the density functional theory and lattice dynamics calculations to investigate the properties of potassium superoxide KO$_2$ in which spin, orbital, and lattice degrees of freedom are interrelated and determine the low-temperature…

The spin correlations of the bilayer manganite $La_{1.2}Sr_{1.8}Mn_{2}O_{7}$ have been studied using neutron scattering. On cooling within the paramagnetic state, we observe purely two-dimensional behavior with a crossover to…

Strongly Correlated Electrons · Physics 2007-05-23 S. Rosenkranz , R. Osborn , L. Vasiliu-Doloc , J. W. Lynn , S. K. Sinha , J. F. Mitchell

The double exchange (DE) model is systematically applied for studying the coupling between ferroelectric (FE) and magnetic orders in several prototypical types of multiferroic manganites. The model was constructed for the magnetically…

Strongly Correlated Electrons · Physics 2014-11-26 I. V. Solovyev , S. A. Nikolaev

We investigate the structural, magnetic and spin-state transitions, and magnetocaloric properties of Sr$_{2-x}$La$_x$CoNbO$_6$ ($x=$ 0--1) double perovskites. The structural transition from tetragonal to monoclinic phase at $x$ $\geqslant$…

Materials Science · Physics 2020-04-21 Ajay Kumar , R. S. Dhaka

Understanding the coexistence of ferromagnetism and insulating behavior in manganites is an unsolved problem. We propose a localized-band model involving effective intermediate-range electron-electron (electron-hole) repulsion (attraction)…

Strongly Correlated Electrons · Physics 2018-05-15 Sanjukta Paul , Sudhakar Yarlagadda

In correlated electron materials, electrons often self-organize and form a variety of patterns with potential ordering of charges, spins, and orbitals, which are believed to be closely connected to many novel properties of these materials…

Strongly Correlated Electrons · Physics 2009-10-31 Z. Sun , Q. Wang , A. V. Fedorov , H. Zheng , J. F. Mitchell , D. S. Dessau

We discuss the origin of the reentrant behaviors of insulating states above the Curie temperature of the colossal magnetoresistance manganites. We consider a system where charge ordering and ferromagnetism compete with each other. In the…

Strongly Correlated Electrons · Physics 2007-05-23 Nobuo Furukawa , Yukitoshi Motome , Naoto Nagaosa

The optical properties of the charge-ordering ($CO$) phase of the one-dimensional (1D) half-filled spinless Holstein model are derived at zero temperature within a well-known variational approach improved including second-order lattice…

Strongly Correlated Electrons · Physics 2009-11-10 C. A. Perroni , V. Cataudella , G. De Filippis , G. Iadonisi , V. Marigliano Ramaglia , F. Ventriglia

We study the spin polarised tunnelling mechanism through magnetisation and magnetoresistance in the granular polycrystalline colossal magnetoresistive manganite, La0.55Ho0.15Sr0.3MnO3. This system has a ferromagnetic transition temperature…

Strongly Correlated Electrons · Physics 2019-08-17 P. Raychaudhuri , A. K. Nigam , R. Pinto , Sujeet Chaudhary , S. B. Roy

Spin-crossover compounds, which are characterized by magnetic ions showing low-spin and high-spin states at thermally accessible energies, are ubiquitous in nature. We here focus on the effect of an exchange interaction on the collective…

Statistical Mechanics · Physics 2009-11-13 Carsten Timm , Charles J. Pye

Using ab initio dynamical mean-field theory we explore the electronic and magnetic states of layered Li$_x$MnO$_2$ as a function of $x$, the state of charge. Constructing real-space Wannier projections of Kohn-Sham orbitals based on the…

Strongly Correlated Electrons · Physics 2023-10-18 Hrishit Banerjee , Clare P. Grey , Andrew J. Morris

Neutron diffraction measurements on multiferroic LuFe2O4 show changes in the antiferromagnetic (AFM) structure characterized by wavevector q = (1/3 1/3 1/2) as a function of electric field cooling procedures. The increase of intensity from…

Strongly Correlated Electrons · Physics 2011-11-09 A. M. Mulders , M. Bartkowiak , J. R. Hester , E. Pomjakushina , K. Conder