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The thermoelectric properties of La-filled skutterudites are discussed from the point of view of their electronic structures. These are calculated from first principles within the local density approximation. The electronic structure is in…

Materials Science · Physics 2009-10-30 D. J. Singh , I. I. Mazin

First principles calculations are used to investigate the band structure and the transport related properties of unfilled and filled 4d skutterudite antimonides. The calculations show that, while RhSb3 and p-type La(Rh,Ru)4Sb12 are…

Materials Science · Physics 2009-10-31 Marco Fornari , David J. Singh

This work presents theoretical calculations of the electrical transport properties of the Ag, Au, and La fractionally filled bulk skutterudites: CoSb3, CoAs3, and CoP3. Density functional theory (DFT), along with projector augmented wave…

Materials Science · Physics 2015-04-28 Maria Stoica , Cynthia S. Lo

Phosphide skutterudites primarily show promise for thermoelectric applications due to their chemical stability at high temperatures and relatively low cost. Ion doping and band gap engineering have been used to enhance their typically poor…

We report ab-initio calculations of the stability, lattice dynamics, electronic and thermoelectric properties of cubic La3-yX4 (X=S,Se,Te) materials in view of analyzing their potential for thermoelectric applications. The lanthanum motions…

Materials Science · Physics 2013-12-16 Romain Viennois , Kinga Niedziolka , Philippe Jund

Tetrahedrite (copper antimony sulfosalt) is promising p-type themoeletric material due to very low intrinsic thermal conductivity and moderately-high power factor, with one of the limitations being lack of n-type variant to create…

Materials Science · Physics 2024-08-02 Krzysztof Kapera , Andrzej Kolezynski

We report LDA calculated band structure, densities of states and Fermi surfaces for recently discovered Pt-pnictide superconductors APt3P (A=Ca,Sr,La), confirming their multiple band nature. Electronic structure is essentially three…

Superconductivity · Physics 2015-03-20 I. A. Nekrasov , M. V. Sadovskii

High entropy materials offer a promising avenue for thermoelectric materials discovery, design, and optimization. However, the large chemical spaces that need to be explored hamper their development. In this work, a large family of…

Filling the large voids in the crystal structure of the skutterudite CoSb$_3$ with rattler atoms $R$ provides an avenue for both increasing carrier concentration and disrupting lattice heat transport, leading to impressive thermoelectric…

Materials Science · Physics 2020-07-17 Eric B. Isaacs , Chris Wolverton

The structural, elastic, thermodynamic and thermoelectric characteristics of the $\textrm{CeIr}_\textrm{4} \textrm{P}_\textrm{12}$ skutterudite have been predicted for the first time by applying density functional theory and the…

Materials Science · Physics 2025-04-01 M. Bouchenaki , L. I. Karaouzène , B. N. Brahmi , M. Kaid Slimane

LaOBiPbS$_3$ is a kind of pnictogen-dichalcogenide layered compounds, which have recently been experimentally investigated as thermoelectric materials owing to their low thermal conductivity and high controllability of constituent elements.…

Materials Science · Physics 2020-01-15 Keiya Kurematsu , Masayuki Ochi , Hidetomo Usui , Kazuhiko Kuroki

The electronic structure and thermopower ($\alpha$) behavior of LaFeO$_{3}$ compound were investigated by combining the ab-initio electronic structures and Boltzmann transport calculations. LSDA plus Hubbard U (U = 5 eV) calculation on…

Strongly Correlated Electrons · Physics 2018-05-09 Saurabh Singh , Shivprasad S. Shastri , Sudhir K. Pandey

The microscopic knowledge of the structural, energetic, and electronic properties of scandium fluoride is still incomplete, despite the relevance of this material as an intermediate for the manufacturing of Al-Sc alloys. In a work based on…

We present an angle-resolved photoemission spectroscopy study of the electronic structure of SnTe, and compare the experimental results to ab initio band structure calculations as well as a simplified tight-binding model of the p-bands. Our…

Cu$_3$SbSe$_4$ is a promising thermoelectric material due to high thermopower ($>400\ \mu$V/K) at 300K and higher. Although it has a simple crystal structure derived from zinc blende structure, previous work has shown that the physics of…

Materials Science · Physics 2014-09-17 Dat T. Do , S. D. Manhanti

The large variety of complex electronic structure materials and their alloys, offer highly promising directions for improvements in thermoelectric (TE) power factors (PF). Their electronic structure contains rich features, referred to as…

Materials Science · Physics 2023-11-08 Patrizio Graziosi , Neophytos Neophytou

Using first-principles electronic structure calculations, we studied the electronic and thermoelectric properties of SrTiO3 based oxide materials and their nanostructures identifying those nanostructures which possess highly anisotropic…

We report a comparison study of LaOFeP and LaOFeAs, two parent compounds of recently discovered iron-pnictide superconductors, using angle-resolved photoemission spectroscopy. Both systems exhibit some common features that are very…

The optical conductivity [$\sigma(\omega)$] spectra of alkaline-earth-filled skutterudites with the chemical formula $A^{2+}M_{4}$Sb$_{12}$ ($A$ = Sr, Ba, $M$ = Fe, Ru, Os) and a reference material La$^{3+}$Fe$_{4}$Sb$_{12}$ were obtained…

Strongly Correlated Electrons · Physics 2009-11-13 Shin-ichi Kimura , Hojun Im , Takafumi Mizuno , Shota Narazu , Eiichi Matsuoka , Toshiro Takabatake

The electronic band structure of correlated Ca3Ru2O7 featuring an antiferromagnetic as well as a structural transition has been determined theoretically at high temperatures, which has led to the understanding of the remarkable properties…

Strongly Correlated Electrons · Physics 2018-01-30 Hui Xing , Libin Wen , Chenyi Shen , Jiaming He , Xinxin Cai , Jin Peng , Shun Wang , Mingliang Tian , Zhu-An Xu , Wei Ku , Zhiqiang Mao , Ying Liu
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