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Thermodynamic properties of charge-stabilised colloidal suspensions depend sensitively on the effective charge of the macroions, which can be substantially lower than the bare charge in the case of strong counterion-macroion association. A…

Soft Condensed Matter · Physics 2011-06-28 Alan R. Denton

The influence of a chemically or electrically heterogeneous distribution of interaction sites at a planar substrate on the number density of an adjacent fluid is studied by means of classical density functional theory (DFT). In the case of…

Soft Condensed Matter · Physics 2018-05-25 Maximilian Mußotter , Markus Bier , S. Dietrich

We present a new analytical approach to the strong electrostatic coupling regime (SC), that can be achieved equivalently at low temperatures, high charges, low dielectric permittivity etc. Two geometries are analyzed in detail: one charged…

Statistical Mechanics · Physics 2015-06-03 L. Šamaj , E. Trizac

The effective interaction between two classical nonrelativistic electrons (positrons) in the presence of intense electromagnetic radiation (one and two waves) is theoretically studied. Small relativistic corrections are taking into account…

Plasma Physics · Physics 2020-01-08 S. S. Starodub , S. P. Roshchupkin , V. V. Dubov

The equilibrium phase behavior of a binary mixture of charged colloids and neutral, non-adsorbing polymers is studied within free-volume theory. A model mixture of charged hard-sphere macroions and ideal, coarse-grained, effective-sphere…

Soft Condensed Matter · Physics 2009-11-11 Alan R. Denton , Matthias Schmidt

While the important role of electrostatic interactions in aqueous colloidal suspensions is widely known and reasonably well-understood, the relevance of charge in nonpolar suspensions remains mysterious. We demonstrate that particles can…

Soft Condensed Matter · Physics 2007-05-23 Ming F. Hsu , Eric R. Dufresne , David A. Weitz

Using integral equation theory of liquids to a binary mixed fluid lipid membrane, we study the membrane-mediated interactions between the macroions and the redistribution of neutral and charged lipids due to binding macroions. We find that…

Soft Condensed Matter · Physics 2015-06-25 Xia-qing Shi , Yu-qiang Ma

We present an analytical approach to the strong coupling regime of similarly and highly charged plates in the presence of counter-ions. The procedure is physically transparent and based on an exact expansion around the ground state formed…

Statistical Mechanics · Physics 2011-02-23 L. Samaj , E. Trizac

Realistic charged macromolecules are characterized by discrete (rather than homogeneous) charge distributions. We investigate the effects of surface charge discretization on the counterion distribution at the level of mean-field theory…

Soft Condensed Matter · Physics 2007-05-23 Mark L. Henle , Christian D. Santangelo , Deena M. Patel , Philip A. Pincus

The electrostatic double layer force is key to determining the stability and self-assembly of charged colloids and many other soft matter systems. Fully understanding the attractive force between two like-charged surfaces remains a great…

Soft Condensed Matter · Physics 2024-02-27 Nikhil R. Agrawal , Ravtej Kaur , Carlo Carraro , Rui Wang

Like-charge attraction, driven by ionic correlations, challenges our understanding of electrostatics both in soft and hard matter. For two charged planar surfaces confining counterions and water, we prove that even at relatively low…

Soft Condensed Matter · Physics 2023-03-15 Ivan Palaia , Abhay Goyal , Emanuela del Gado , Ladislav Šamaj , Emmanuel Trizac

Brownian Dynamics simulations are carried out to understand the effect of temperature and dielectric constant of the medium on microphase separation of charged-neutral diblock copolymer systems. For different dielectric media, we focus on…

Soft Condensed Matter · Physics 2011-07-20 Monojoy Goswami , Rajeev Kumar , Bobby G. Sumpter , Jimmy Mays

We investigate the complexation of a highly charged sphere with a long flexible polyelectrolyte, \textit{both negatively charged} in salt free environment. Electroneutrality is insured by the presence of divalent counterions. Using…

Soft Condensed Matter · Physics 2007-05-23 Rene Messina , Christian Holm , Kurt Kremer

From cement cohesion to DNA condensation, a proper statistical physics treatment of systems with long range forces is important for a number of applications in physics, chemistry, and biology. We compute here the effective force between…

Soft Condensed Matter · Physics 2018-03-14 E. Trizac , G. Téllez

The equilibrium properties of hard rod monolayers are investigated in a lattice model (where position and orientation of a rod are restricted to discrete values) as well as in an off--lattice model featuring spherocylinders with continuous…

Soft Condensed Matter · Physics 2016-09-21 M. Oettel , M. Klopotek , M. Dixit , E. Empting , T. Schilling , H. Hansen--Goos

Neutral or charged polymers that are densely end-grafted to surfaces form brush-like structures and are highly stretched under good-solvent conditions. We discuss and compare relevant results from scaling models, self-consistent-field…

Soft Condensed Matter · Physics 2007-05-23 Ali Naji , Christian Seidel , Roland R. Netz

The effects of discrete macroion surface charge distribution and valences of these surface charges and counterions on charge reversal have been studied for macroions of three different geometries and compared with those of continuous…

Biological Physics · Physics 2008-07-25 Arup K. Mukherjee

In this paper, we theoretically study the electrostatic interaction between a pair of identical colloids with constant surface potentials sitting in close vicinity of each other at a fluid interface. By employing a simplified yet reasonable…

Soft Condensed Matter · Physics 2020-07-29 Rick Bebon , Arghya Majee

The transport of polyelectrolytes confined by oppositely charged surfaces and driven by a constant electric field is of interest in studies of DNA separation according to size. Using molecular dynamics simulations that include surface…

Soft Condensed Matter · Physics 2020-09-15 Debarshee Bagchi , Monica Olvera de la Cruz

The phase behavior of charge-stabilized colloidal suspensions is modeled by a combination of response theory for electrostatic interparticle interactions and variational theory for free energies. Integrating out degrees of freedom of the…

Soft Condensed Matter · Physics 2009-11-11 Alan R. Denton