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The role of surface collective excitations in the electron relaxation in small metal particles is studied. It is shown that the dynamically screened electron-electron interaction in a nanoparticle contains a size-dependent correction…

Condensed Matter · Physics 2009-10-31 T. V. Shahbazyan , I. E. Perakis

We study the effect of Coulomb correlations on the ultrafast optical dynamics of small metal particles. We demonstrate that a surface-induced dynamical screening of the electron-electron interactions leads to quasiparticle scattering with…

Condensed Matter · Physics 2009-10-31 T. V. Shahbazyan , I. E. Perakis , J. -Y. Bigot

We study the linewidth of the surface plasmon resonance in the optical absorption spectrum of metallic nanoparticles, when the decay into electron-hole pairs is the dominant channel. Within a semiclassical approach, we find that the…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Rafael A. Molina , Dietmar Weinmann , Rodolfo A. Jalabert

The electronic environment causes decoherence and dissipation of the collective surface plasmon excitation in metallic nanoparticles. We show that the coupling to the electronic environment influences the width and the position of the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Guillaume Weick , Gert-Ludwig Ingold , Rodolfo A. Jalabert , Dietmar Weinmann

In this paper we analyse the importance of a detailed description of the electronic transitions in ultra-small nanoparticles through the optical response to very small changes of size in systems, whose dimensions are in the subnanometric…

Mesoscale and Nanoscale Physics · Physics 2014-04-29 Mario Zapata-Herrera , Angela S. Camacho

Multipolar plasmon oscillation frequencies and corresponding damping rates for nanospheres formed of the simplest free-electron metals are studied. The possibility of controlling plasmon features by choosing the size and dielectric…

Optics · Physics 2008-04-15 A. Derkachova , K. Kolwas

Two possible mechanisms of surface plasmon (SP) oscillations damping in metallic nanoparticles (MNPs), not connected with electron-phonon interaction are investigated theoretically: a) the radiation damping of SP, b) resonant coupling of SP…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Armen Melikyan , Hayk Minassian

Surface and volume plasmons excited in a metal cluster by moving electron and corresponding inelastic scattering spectra are studied based on the hydrodynamic approach. Along with the bulk losses traditionally taken into account, the…

Plasma Physics · Physics 2016-04-20 V. B. Gildenburg , V. A. Kostin , I. A. Pavlichenko

We show that the dynamics of the surface plasmon in metallic nanoparticles damped by its interaction with particle-hole excitations can be modelled by a single degree of freedom coupled to an environment. In this approach, the fast decrease…

Mesoscale and Nanoscale Physics · Physics 2011-11-09 Cesar Seoanez , Guillaume Weick , Rodolfo A. Jalabert , D. Weinmann

Optical manipulation of Mie-resonant dielectric nanoparticles is strongly influenced by their enhanced scattering and multipolar response, which fundamentally modifiesthe balance of optical forces. In this work, we study the optical forces…

Optics · Physics 2026-05-19 Semyon Borodulin , Natalia Kostina , Mihail Petrov

We study the thermal response of a single spherical metal nanoparticle to continuous wave illumination as a function of its size. We show that the particle temperature increases non-monotonically as the particle size increases, indicating…

Optics · Physics 2020-01-08 Ieng-Wai Un , Yonatan Sivan

We investigate theoretically the formation of collective excitations in atomic scale quasi-one dimensional metallic nanostructures. The response of the system is calculated within the linear response theory and random phase approximation.…

Mesoscale and Nanoscale Physics · Physics 2008-04-17 Amy Cassidy , Ilya Grigorenko , Stephan Haas

Damping rates of multipolar, localized surface plasmons (SP) of gold and silver nanospheres of radii up to $1000nm$ were found with the tools of classical electrodynamics. The significant increase in damping rates followed by noteworthy…

Optics · Physics 2012-11-21 Krystyna Kolwas , Anastasiya Derkachova

We study the role of strong electron confinement in surface-enhanced Raman scattering from molecules adsorbed on small noble-metal particles. We describe a new source of Raman signal enhancement which originates from different behavior of…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Vitaliy N. Pustovit , Tigran V. Shahbazyan

The fact that surface-induced damping rate of surface plasmon polaritons (SPPs) in metal nanoparticles increases with the decrease of particle size is well known. We show that this rate also increases with the degree of the mode…

Optics · Physics 2016-01-20 Jacob B Khurgin , Greg Sun

Theoretical description of oscillations of electron liquid in large metallic nanospheres (with radius of few tens nm) is formulated within random-phase-approximation semiclassical scheme. Spectrum of plasmons is determined including both…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 W. Jacak , J. Krasnyj , J. Jacak , R. Gonczarek , A. Chepok , L. Jacak , D. Z. Hu , D. Schaadt

Assemblies of closely separated gold nanoparticles exhibit a strong collective plasmonic response due to coupling of the plasmon modes of the individual nanostructures. In the context of self-assembly of nanoparticles, closed packed 2D…

Materials Science · Physics 2021-08-05 Rituraj Borah , Sammy W. Verbruggen

We report the studies of ultrafast electron nanocrystallography on size-selected Au nanoparticles (2-20 nm) supported on a molecular interface. Reversible surface melting, melting, and recrystallization were investigated with dynamical…

Materials Science · Physics 2015-05-13 Chong-Yu Ruan , Yoshie Murooka , Ramani K. Raman , Ryan A. Murdick

We report size-dependent melting of spherical copper nanoparticles embedded into silica matrix. Based on the temperature dependence of the surface plasmon resonance energy and its width we observe two distinct melting regimes. For particles…

Materials Science · Physics 2007-05-23 Oleg A. Yeshchenko , Igor M. Dmytruk , Alexandr A. Alexeenko , Andriy M. Dmytruk

We study the spin-dependent electronic excitations in alkali-metal nanoparticles. Using numerical and analytical approaches, we focus on the resonances in the response to spin-dependent dipole fields. In the spin-dipole absorption spectrum…

Mesoscale and Nanoscale Physics · Physics 2009-09-18 Yue Yin , Paul-Antoine Hervieux , Rodolfo A. Jalabert , Giovanni Manfredi , Emmanuel Maurat , Dietmar Weinmann
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