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Two-photon absorption is theoretically analyzed within the semiclassical formalism of radiation-matter interaction. We consider an ensemble of inhomogeneously broadened three-level atoms subjected to the action of two counterpropagating…

Quantum Physics · Physics 2007-05-23 I. Perez-Arjona , G. J. de Valcarcel , Eugenio Roldan

For dissipation-free photon-photon interaction at the single photon level, we analyze one-photon transition and two-photon transition induced by photon pairs in three-level atoms using two-photon wavefunctions. We show that the two-photon…

Quantum Physics · Physics 2011-06-16 Toshihiro Nakanishi , Hirokazu Kobayashi , Kazuhiko Sugiyama , Masao Kitano

It is well known that energy-time entanglement can enhance two photon absorption (TPA) by simultaneously optimizing the two photon resonance and the coincidence rate of photons at the absorber. However, the precise relation between…

Quantum Physics · Physics 2021-08-31 Baihong Li , Holger F. Hofmann

Based on quantum electrodynamics, we reexamine the two-photon decay of one-electron atoms. Special attention is paid to the calculation of the (two-photon) total decay rates which can be viewed as the imaginary part of the two-loop…

Atomic Physics · Physics 2008-07-08 Ulrich D. Jentschura , Andrey Surzhykov

We calculate the rate of two-photon absorption for frequency entangled photons in a tapered optical fiber whose diameter is comparable to the wavelength of the light. The confinement of the electric field in the transverse direction…

Quantum Physics · Physics 2010-04-12 Hao You , S. M. Hendrickson , J. D. Franson

We present a theoretical analysis of two-photon absorption of classical and squeezed light valid when one-photon absorption to an intermediate state is either resonant or far-detuned from resonance, and in both the low and high intensity…

Quantum Physics · Physics 2022-09-14 Christian Drago , John Sipe

We present a quantum sensing protocol for three-dimensional estimation of the difference between the momenta of two photons based on spatially resolved interferometric sampling measurements. The protocol attains ultimate quantum precision…

Quantum Physics · Physics 2026-03-10 Luca Maggio , Vincenzo Tamma

We have expressed the nonlinear optical absorption of a semiconductor in terms of its linear spectrum. We determined that the two-photon absorption coefficient in a strong DC-electric field of a direct gap semiconductor can be expressed as…

Optics · Physics 2009-11-13 Hernando Garcia , Ramki Kalyanaraman

In this paper, we analyze how multi-photon subtraction operations in a feedback-assisted interferometer can enhance measurement precision for single-parameter and two-parameter estimation under both ideal and photon-loss conditions. We…

Quantum Physics · Physics 2025-06-09 Qingqian Kang , Zekun Zhao , Qisi Zhou , Teng Zhao , Cunjin Liu , Xin Su , Liyun Hu , Sanqiu Liu

In this paper, two-photon absorption resonance has been investigated . We studied this phenomenon in three-level system with common upper level, two lower long-life levels and two quasi-resonant laser fields with different frequency…

Atomic Physics · Physics 2014-07-23 Tara Ahmadi , Sergei. A Pulkin

Accurate predictions of inclusive scattering cross sections in the linear response regime require efficient and controllable methods to calculate the spectral density in a strongly-correlated many-body system. In this work we reformulate…

Quantum Physics · Physics 2023-03-29 Jeremy Hartse , Alessandro Roggero

The absorption of broadband photons in atomic ensembles requires either an effective broadening of the atomic transition linewidth, or an off-resonance Raman interaction. Here we propose a scheme for a quantum memory capable of storing and…

Quantum Physics · Physics 2017-01-18 G. S. Thekkadath , K. Heshami , D. G. England , P. J. Bustard , B. J. Sussman , M. Spanner

The rapid advancement of quantum information technology has increased the demand for precise testing and calibration of quantum modules, especially in optical quantum circuits where module reliability directly impacts system performance. To…

Quantum Physics · Physics 2025-01-10 Xiaoqian Zhang , Maolin Luo , Xiaoqi Zhou

Two-photon absorption in indirect gap semiconductors is an frequently encountered, but not well-understood phenomenon. To address this, the Real Density Matrix Approach is applied to describe two-photon absorption in silicon through the…

Ultrafast optical spectroscopy is a powerful technique for studying the dynamic processes of molecular systems in condensed phases. However, in molecular systems containing many dye molecules, the spectra can become crowded and difficult to…

Chemical Physics · Physics 2025-02-05 Yuta Fujihashi , Akihito Ishizaki , Ryosuke Shimizu

We demonstrate the ultimate sensitivity allowed by quantum physics in the estimation of the time delay between two photons by measuring their interference at a beam-splitter through frequency-resolving sampling measurements. This…

Quantum Physics · Physics 2023-04-25 Danilo Triggiani , Giorgos Psaroudis , Vincenzo Tamma

Joint spectral measurements are a powerful tool for characterising biphoton spectral correlation, which is crucial for quantum information and communication technologies. In these applications, highly pure biphoton states are essential in…

When a low flux of time-frequency-entangled photon pairs (EPP) illuminates a two-photon transition, the rate of two-photon absorption (TPA) can be enhanced considerably by the quantum nature of photon number correlations and frequency…

We formulate a computationally efficient time-independent method based on the multi-electron molecular R-matrix formalism. This method is used to calculate transition matrix elements for the multi-photon ionization of atoms and molecules…

Atomic Physics · Physics 2022-05-10 Jakub Benda , Zdeněk Mašín

Within the well-established optical response function formalism, a new strategy with the central idea of employing the forward-backward stochastic Schr\"{o}dinger equations in a segmented way to accurately obtain the two-dimensional (2D)…

Chemical Physics · Physics 2018-08-08 Yaling Ke , Yi Zhao
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