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Model calculations that include the effects of irreversible, environmental couplings on top of a coupled-channels dynamical description of the collision of two complex nuclei are presented. The Liouville-von Neumann equation for the…

Nuclear Theory · Physics 2009-11-13 Alexis Diaz-Torres , David Hinde , Mahananda Dasgupta , Gerard Milburn , Jeff Tostevin

Stochastic evolution underpins several approaches to the dynamics of open quantum systems, such as random modulation of Hamiltonian parameters, the stochastic Schrodinger equation (SSE), and the stochastic Liouville equation (SLE). These…

Quantum Physics · Physics 2026-01-22 Pietro De Checchi , Federico Gallina , Barbara Fresch , Giulio G. Giusteri

The Driven Liouville von Neumann approach [J. Chem. Theory Comput. 10, 2927-2941 (2014)] is a computationally efficient simulation method for modeling electron dynamics in molecular electronics junctions. Previous numerical simulations have…

Chemical Physics · Physics 2016-06-08 Oded Hod , César A. Rodríguez-Rosario , Tamar Zelovich , Thomas Frauenheim

We present an application of the Extended Stochastic Liouville-von Neumann equations (ESLN) method introduced earlier [PRB 95, 125124 (2017); PRB 97, 224310 (2018)] which describes the dynamics of an exactly thermalised open quantum system…

Quantum Physics · Physics 2020-07-01 M. A. Lane , D. Matos , I. J. Ford , L. Kantorovich

The Fokker-Planck equations for stochastic dynamical systems, with non-Gaussian $\alpha-$stable symmetric L\'evy motions, have a nonlocal or fractional Laplacian term. This nonlocality is the manifestation of the effect of non-Gaussian…

Numerical Analysis · Mathematics 2013-10-30 Ting Gao , Jinqiao Duan , Xiaofan Li

The standard weak-coupling approximations associated to open quantum systems have been extensively used in the description of a two-level quantum system, qubit, subjected to relatively weak dissipation compared with the qubit frequency.…

Quantum Physics · Physics 2022-02-15 Wallace S. Teixeira , Fernando L. Semião , Jani Tuorila , Mikko Möttönen

A numerically exact Monte Carlo scheme for calculation of open quantum system dynamics is proposed and implemented. The method consists of a Monte-Carlo summation of a perturbation expansion in terms of trajectories in Liouville phase-space…

Chemical Physics · Physics 2014-11-10 Jan Olsina , Tobias Kramer , Christoph Kreisbeck , Tomas Mancal

In the dynamics of driven impurity models, there is a fundamental asymmetry between the processes of emission and absorption of environment excitations: most of the emitted excitations are rapidly and irreversibly scattered away, and only a…

Strongly Correlated Electrons · Physics 2017-12-13 Evgeny A. Polyakov , Alexey N. Rubtsov

Quantum computers can be used to simulate nonlinear non-Hamiltonian classical dynamics on phase space by using the generalized Koopman-von Neumann formulation of classical mechanics. The Koopman-von Neumann formulation implies that the…

Quantum Physics · Physics 2020-10-27 Ilon Joseph

A systematic procedure for optimising the friction coefficient in underdamped Langevin dynamics as a sampling tool is given by taking the gradient of the associated asymptotic variance with respect to friction. We give an expression for…

Computation · Statistics 2023-11-01 Martin Chak , Nikolas Kantas , Tony Lelièvre , Grigorios A. Pavliotis

The stochastic differential equations for a model of dissipative particle dynamics, with both total energy and total momentum conservation at every time-step, are presented. The algorithm satisfies detailed balance as well as the…

Statistical Mechanics · Physics 2007-05-23 Allan D. Mackie , Josep Bonet Avalos

We discuss two methods of an exact stochastic representation of the non-Markovian quantum dynamics of open systems. The first method employs a pair of stochastic product vectors in the total system's state space, while the second method…

Quantum Physics · Physics 2007-07-13 Heinz-Peter Breuer , Francesco Petruccione

A recent proposal for practical calculation of vibrational mode lifetimes is tested on simple, low-dimensional anharmonic models. The proposed scheme approximates the mode lifetime in terms of ensemble averages of specific functions in…

Statistical Mechanics · Physics 2013-04-26 Yang Gao , Doyl Dickel , David Harrison , Murray S. Daw

Quantum dynamics for arbitrary system are traditionally realized by time evolutions of wave functions in Hilbert space and/or density operators in Liouville space. However, the traditional simulations may occasionally turn out to be…

Quantum Physics · Physics 2023-04-20 Gombojav O. Ariunbold

We propose a highly efficient mixed quantum-classical molecular dynamics scheme based on a solution of the quantum-classical Liouville equation (QCLE). By casting the equations of motion for the quantum subsystem and classical bath degrees…

Chemical Physics · Physics 2018-07-06 Junjie Liu , Gabriel Hanna

We point out that the quantum dynamical map of an open quantum system can be generated by an effective Liouville operator. The effective Liouville shows the dynamical breaking of time reversibility. This breaking of reversibility is…

Quantum Physics · Physics 2017-08-01 Martin Janßen

A recently proposed method for computer simulations in the isothermal-isobaric (NPT) ensemble, based on Langevin-type equations of motion for the particle coordinates and the ``piston'' degree of freedom, is re-derived by straightforward…

Soft Condensed Matter · Physics 2016-08-31 A. Kolb , B. Duenweg

A Gaussian operator basis provides a means to formulate phase-space simulations of the real- and imaginary-time evolution of quantum systems. Such simulations are guaranteed to be exact while the underlying distribution remains…

Computational Physics · Physics 2012-04-04 M. Ogren , K. V. Kheruntsyan , J. F. Corney

Exact and nonperturbative quantum master equation can be constructed via the calculus on path integral. It results in hierarchical equations of motion for the reduced density operator. Involved are also a set of well--defined auxiliary…

Statistical Mechanics · Physics 2015-05-13 Jian Xu , Rui-Xue Xu , YiJing Yan

It has been recently realized that dissipative processes can be harnessed and exploited to the end of coherent quantum control and information processing. In this spirit we consider strongly dissipative quantum systems admitting a…

Quantum Physics · Physics 2014-12-18 Paolo Zanardi , Lorenzo Campos Venuti