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The formalism of Kohn and Sham uses a specific (model) hamiltonian which highly simplifies the many-electron problem to that of noninteracting fermions. The theorem of Hohenberg and Kohn tells us that, for a given ground state density, this…

Materials Science · Physics 2007-07-05 Paola Gori-Giorgi , Julien Toulouse , Andreas Savin

Predictivity of the Kohn-Sham approach to dynamical problems, when regarded as an initial value problem in a time-dependent density functional framework, is analysed for a class of models for which the argument devised in the work of Maitra…

Other Condensed Matter · Physics 2015-06-16 Walter Tarantino

A general penalty method is presented for the construction of of Kohn-Sham system for given density through Levy's constrained-search. The method uses a functional $S[\rho]$ of one's choice. Different forms of $S[\rho]$ are employed to…

Atomic Physics · Physics 2020-05-22 Ashish Kumar , Manoj K. Harbola

The density functional theory is extended to account for self-bound systems. To this end the Hohenberg-Kohn theorem is formulated for the intrinsic density and a Kohn-Sham like procedure for an $N$--body system is derived using the…

Nuclear Theory · Physics 2008-11-26 Nir Barnea

The multi-component density functional theory is faced with the challenge of capturing various types of inter- and intra-particle exchange-correlation effects beyond those introduced by the conventional electronic exchange-correlation…

Atomic and Molecular Clusters · Physics 2023-12-27 Nahid Sadat Riyahi , Mohammad Goli , Shant Shahbazian

We present a numerical tool for solving the non-relativistic Kohn-Sham problem for spherically-symmetric atoms. It treats the Schr\"{o}dinger equation as an integral equation relying heavily on convolutions. The solver supports different…

Atomic and Molecular Clusters · Physics 2022-07-13 Jānis Užulis , Andris Gulans

We have obtained the solutions of linearized Shr{\"o}dinger equation for spherically and axially symmetrical electrons density oscillations in plasma in the approximation of the self-consistent field. It was shown that in the center or on…

Plasma Physics · Physics 2007-05-23 M. Dvornikov , S. Dvornikov , G. Smirnov

We present a method for the calculation of electronic structure of systems that contain tens of thousands of atoms. The method is based on the division of the system into mutually overlapping fragments and the representation of the…

Materials Science · Physics 2011-03-09 Nenad Vukmirović , Lin-Wang Wang

A complete solution to the inverse problem of Kohn-Sham (KS) density functional theory is proposed. Our method consists of two steps. First, the effective KS potential is determined from the ground state density of a given system. Then, the…

Nuclear Theory · Physics 2022-03-14 A. Liardi , F. Marino , G. Colò , X. Roca-Maza , E. Vigezzi

Simulating the unitary dynamics of a quantum system is a fundamental problem of quantum mechanics, in which quantum computers are believed to have significant advantage over their classical counterparts. One prominent such instance is the…

Quantum Physics · Physics 2024-09-04 John M. Martyn , Yuan Liu , Zachary E. Chin , Isaac L. Chuang

The starting point is the problem of finding the interaction energy of two coinciding homogeneous cubic charge distributions. The brute force method of subdividing the cube into $N^3$ sub-cubes and doing the sums results in slow convergence…

Atomic and Molecular Clusters · Physics 2007-05-23 Hanno Essen

Most treatments of electron-electron correlations in dense plasmas either ignore them entirely (random phase approximation) or neglect the role of ions (jellium approximation). In this work, we go beyond both these approximations to derive…

Plasma Physics · Physics 2020-02-05 Nathaniel R. Shaffer , Charles E. Starrett

The paper that follows describes a numerical algorithm to solve the parabolic-parabolic Keller--Segel system characterized by singular sensitivity and signal absorption in such a manner that the numerical approximations converge towards a…

Numerical Analysis · Mathematics 2026-04-01 Juan Vicente Gutiérrez-Santacreu

A fast algorithm (linear in the degrees of freedom) for the solution of linear variable-coefficient rational-order fractional integral and differential equations is described. The approach is related to the ultraspherical method for…

Numerical Analysis · Mathematics 2017-12-04 Nicholas Hale , Sheehan Olver

A linear-algebraic theory called 'multiple Arnoldi method' is presented and realizes large-scale (order-N) electronic structure calculation with generalized eigen-value equations. A set of linear equations, in the form of (zS-H) x = b, are…

Materials Science · Physics 2012-04-04 T. Hoshi , S. Yamamoto , T. Fujiwara , T. Sogabe , S. -L. Zhang

The self-consistent quantum-electrostatic (also known as Poisson-Schr\"odinger) problem is notoriously difficult in situations where the density of states varies rapidly with energy. At low temperatures, these fluctuations make the problem…

Mesoscale and Nanoscale Physics · Physics 2019-09-11 P. Armagnat , A. Lacerda-Santos , B. Rossignol , C. Groth , X. Waintal

While the treatment of chemically relevant systems containing hundreds or even thousands of electrons remains beyond the reach of quantum devices, the development of quantum-classical hybrid algorithms to resolve electronic correlation…

This paper studies the convergence rate of the Euler-Maruyama scheme for systems of interacting particles used to approximate solutions of nonlinear Fokker-Planck equations with singular interaction kernels, such as the Keller-Segel model.…

Probability · Mathematics 2025-04-09 Nicoleta Cazacu

Kohn-Sham (KS) density functional theory (DFT) is a very efficient method for calculating various properties of solids as, for instance, the total energy, the electron density, or the electronic band structure. The KS-DFT method leads to…

Materials Science · Physics 2019-09-20 Fabien Tran , Jan Doumont , Leila Kalantari , Ahmad W. Huran , Miguel A. L. Marques , Peter Blaha

We consider various iterative algorithms for solving the linear equation $ax=b$ using a quantum computer operating on the principle of quantum annealing. Assuming that the computer's output is described by the Boltzmann distribution, it is…

Quantum Physics · Physics 2023-10-25 V. Shalgin , S. Tikhomirov