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Related papers: Dynamics of Highly Supercooled Liquids

200 papers

We have investigated dynamical heterogeneity in a highly supercooled liquid using molecular-dynamics simulations in three dimensions. Dynamical heterogeneity can be characterized by three quantities: correlation length $\xi_4$, intensity…

Soft Condensed Matter · Physics 2012-04-25 Hideyuki Mizuno , Ryoichi Yamamoto

We study the transport properties of a system of active particles moving at constant speed in an heterogeneous two-dimensional space. The spatial heterogeneity is modeled by a random distribution of obstacles, which the active particles…

Biological Physics · Physics 2013-10-23 Oleksandr Chepizhko , Fernando Peruani

The microscopic dynamics and aging of a soft thermosensitive suspension was investigated by looking at the thermal fluctuations of tracers in the suspension. Below and above the glass transition, the dense microgel particles suspension was…

Soft Condensed Matter · Physics 2014-02-05 Rémy Colin , Ahmed M. Alsayed , Jean-Christophe Castaing , Rajesh Goyal , Larry Hough , Bérengère Abou

We study a highly supercooled two-dimensional fluid mixture via molecular dynamics simulation. We follow bond breakage events among particle pairs, which occur on the scale of the $\alpha$ relaxation time $\tau_{\alpha}$. Large scale…

Soft Condensed Matter · Physics 2015-06-25 Ryoichi Yamamoto , Akira Onuki

Spatial distributions of heavy particles suspended in an incompressible isotropic and homogeneous turbulent flow are investigated by means of high resolution direct numerical simulations. In the dissipative range, it is shown that particles…

Chaotic Dynamics · Physics 2007-05-23 J. Bec , L. Biferale , M. Cencini , A. Lanotte , S. Musacchio , F. Toschi

We use computer simulations to explore the manner in which the particle displacements on intermediate time scales in supercooled fluids correlate to their dynamic structural environment. The fluid we study, a binary mixture of hard spheres,…

Soft Condensed Matter · Physics 2010-05-11 William P. Krekelberg , Venkat Ganesan , Thomas M. Truskett

Diffusion-coagulation can be simply described by a dynamic where particles perform a random walk on a lattice and coalesce with probability unity when meeting on the same site. Such processes display non-equilibrium properties with strong…

Statistical Mechanics · Physics 2018-03-13 L. Turban , J. -Y. Fortin

We simulate a model of repulsively interacting colloids on a commensurate two-dimensional triangular pinning substrate where the amount of heterogeneous motion that appears at melting can be controlled systematically by turning off a…

Soft Condensed Matter · Physics 2009-11-11 J. -X. Lin , C. Reichhardt , Z. Nussinov , Leonid P. Pryadko , C. J. Olson Reichhardt

Molecular dynamics simulations are performed to study spatially heterogeneous dynamics in a model of viscous silica above and below the critical temperature of the mode coupling theory, $T_{MCT}$. Specifically, we follow the evolution of…

Soft Condensed Matter · Physics 2009-11-10 M. Vogel , S. C. Glotzer

It is widely believed that the breakdown of the Stokes-Einstein (SE) relation between the translational diffusivity and the shear viscosity in supercooled liquids is due to the development of dynamic heterogeneity i.e. the presence of both…

Statistical Mechanics · Physics 2015-06-12 Shiladitya Sengupta , Smarajit Karmakar

In this paper the phenomenon of dynamic heterogeneity in supercooled liquid systems is considered in terms of the recently proposed gauge theory of glass transition. The physical interpretation of the dynamic scaling is considered. It is…

Statistical Mechanics · Physics 2015-06-23 Mikhail Vasin

Dynamical heterogeneity, in which transitory local fluctuations occur in the conformation and dynamics of constituent particles, is widely hypothesized to be essential to evolution of supercooled liquids into the structural glass state. Yet…

Supercooled liquids exhibit complicated dynamical behaviors: At the microscopic level, the dynamics is heterogeneous spatially, known as dynamic heterogeneity. At the macroscopic level, the shear viscosity $\eta$ decreases as shear rate…

Soft Condensed Matter · Physics 2025-09-01 Ke-Qi Zeng , Dong-Xu Yu , Zhe Wang

Non-Gaussian displacement distributions are universal predictors of dynamic heterogeneity in slowly varying environments. Here, we explore heterogeneous dynamics in supercooled liquid using molecular dynamics simulations and show the…

Soft Condensed Matter · Physics 2023-08-29 Vinay Vaibhav , Suman Dutta

Recent experiments and computer simulations show that supercooled liquids around the glass transition temperature are "dynamically heterogeneous" [1]. Such heterogeneity is expected from the random first order transition theory of the glass…

Disordered Systems and Neural Networks · Physics 2009-10-31 Xiaoyu Xia , Peter G. Wolynes

We discuss the relaxation dynamics of a simple lattice gas model for glass-forming systems and show that with increasing density of particles this dynamics slows down very quickly. By monitoring the trajectory of tagged particles we find…

Soft Condensed Matter · Physics 2010-05-07 Pinaki Chaudhuri , Ludovic Berthier , Srikanth Sastry , Walter Kob

We investigate the single-file dynamics of a tagged particle in a system consisting of N hardcore interacting particles (the particles cannot pass each other) which are diffusing in a one-dimensional system where the particles have…

Statistical Mechanics · Physics 2009-11-13 Tobias Ambjornsson , Ludvig Lizana , Michael A. Lomholt , Robert J. Silbey

We examine the structure of the distribution of single particle displacements (van-Hove function) in a broad class of materials close to glass and jamming transitions. In a wide time window comprising structural relaxation, van-Hove…

Statistical Mechanics · Physics 2009-11-13 Pinaki Chaudhuri , Ludovic Berthier , Walter Kob

The mechanism of diffusion in supercooled liquids is investigated from the potential energy landscape point of view, with emphasis on the crossover from high- to low-T dynamics. Molecular dynamics simulations with a time dependent mapping…

Statistical Mechanics · Physics 2009-11-07 T. Keyes , J. Chowdhary

State-of-the-art techniques for simulating deeply supercooled liquids require a high degree of size polydispersity to be effective. While these techniques have enabled great insight into the microscopic dynamics near the glass transition,…

Soft Condensed Matter · Physics 2023-08-10 Ilian Pihlajamaa , Corentin C. L. Laudicina , Liesbeth M. C. Janssen