Related papers: Quantum Coherence in Fe8 Molecular Nanomagnets
The magnetization of Zn1-xCoxO (0.0055 < x < 0.073) nanoparticles has been measured as a function of temperature T (1.7 K < T , 10 K) and for magnetic field up to 65 kOe using a SQUID magnetometer. Samples were synthesized by three…
Magnetic resonance detection is one of the most important tools used in life-sciences today. However, as the technique detects the magnetization of large ensembles of spins it is fundamentally limited in spatial resolution to mesoscopic…
In this article, we report on inelastic neutron scattering measurements on a quasi-1D antiferromagnet BaCo$_2$V$_2$O$_8$ under a transverse magnetic field applied along the (0,1,0) direction. Combining results of inelastic neutron…
A major challenge in quantum metrology is the generation of entangled states with macroscopic atom number. Here, we demonstrate experimentally that atomic squeezing generated via non-linear dynamics in Bose Einstein condensates, combined…
The spin-reversal in dilute Li$_2$(Li$_{1-x}$Fe$_{x}$)N with $x < 1$ % is dominated by resonant quantum tunneling of spatially well-separated states. We report on the effect of finite couplings between those states that give rise to…
Molecular magnets are attractive as spin qubits due to their chemical tunability, addressability through electron-spin resonance techniques, and long coherence times. Clock transitions (CTs), for which the system is immune to the effect of…
We report $^{115}$In nuclear magnetic resonance (NMR) measurements in CeCoIn$_5$ at low temperature ($T \approx 70$ mK) as a function of magnetic field ($H_0$) from 2 T to 13.5 T applied perpendicular to the $\hat c$-axis. NMR line shift…
Close to the quantum critical point of the transverse-field Ising spin-chain model, an exotic dynamic spectrum was predicted to emerge upon a perturbative longitudinal field. The dynamic spectrum consists of eight particles and is governed…
The excellent sensitivities of quantum sensors are a double-edged sword: minuscule quantities can be observed, but any undesired signal acts as noise. This is challenging when detecting quantities that are obscured by such noise. Decoupling…
We calculate from first principles the electronic structure, relaxation and magnetic moments in small Fe particles, applying the numerical local orbitals method in combination with norm-conserving pseudopotentials. The accuracy of the…
Quantum oscillations in the binary antiferromagnetic metal FeAs are presented and compared to theoretical predictions for the electronic band structure in the anomalous spin density wave state of this material. Demonstrating a new method…
We review the present state of theory and experiments on the quantum tunneling of magnetization in mesoscopic spin systems. Most attention is paid to the relaxation of magnetization in the molecular complexes Mn12 and Fe8. The role of the…
The concept of entanglement, in which coherent quantum states become inextricably correlated, has evolved from one of the most startling and controversial outcomes of quantum mechanics to the enabling principle of emerging technologies such…
The assemblies of either quantum dots or magnetic nanoclusters are studied. It is shown that such assemblies can produce coherent radiation. A method is developed for solving the systems of nonlinear equations describing the dynamics of…
High-frequency ($f$ = 190 GHz) electron paramagnetic resonance (EPR) at magnetic fields up to 12 T as well as Q-band ($f$ = 34.1 GHz) EPR were performed on single crystals of the molecular wheel CsFe$_8$. In this molecule, eight Fe(III)…
We report zero-field inelastic neutron scattering experiments on a deuterated powder sample of Mn12-Acetate consisting of a large number of nominally identical spin-10 magnetic clusters. Our resolution enables us to see a series of peaks…
In zero magnetic field, the famous neutron spin resonance in the f-electron superconductor CeCoIn5 is similar to the recently discovered exciton peak in the non-superconducting CeB6. Magnetic field splits the resonance in CeCoIn5 into two…
The inhomogeneous magnetic stray field of micromagnets has been extensively used to manipulate electron spin qubits. By means of micromagnetic simulations and scanning superconducting quantum interference device microscopy, we show that the…
Similar to atoms and nuclei, semiconductor quantum dots exhibit formation of shells. Predictions of magnetic behavior of the dots are often based on the shell occupancies. Thus, closed-shell quantum dots are assumed to be inherently…
High energy resolution spectroscopic studies of quantum magnets have proven to be extremely valuable in directly accessing magnetodynamics quantities, such as energy barriers, magnetic interactions, lifetime of excited states and…