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First-principles calculations reveal large zone-center spin-phonon coupling and magnetically-driven phonon anisotropy in cubic perovskites Sr$M$O$_3$ ($M$=V,Cr,Mn,Fe,Co). In particular, the frequency and splitting of the polar Slater mode…

Strongly Correlated Electrons · Physics 2012-09-10 Jun Hee Lee , Karin M. Rabe

We report on the structural evolution, spin phonon interactions, and magnetoelastic effects in bulk LaFeO3 perovskite across its antiferromagnetic transition. We found that while the lattice constants exhibit slight deviations at the Neel…

Phonon-derived behaviors are important indicators of novel phenomena in transition metal trihalides, including spin liquid behavior, two-dimensional magnetism, and spin-lattice coupling. However, phonons and their dependence on spin…

The spin-lattice coupling plays an important role in strongly frustrated magnets. In ZnCr$_2$O$_4$, an excellent realization of the Heisenberg antiferromagnet on the ``pyrochlore'' network, a lattice distortion relieves the geometrical…

Strongly Correlated Electrons · Physics 2009-11-10 A. B. Sushkov , H. D. Drew , O. Tchernyshyov , W. Ratcliff , S. W. Cheong

We have carried out an extensive phonon study on multiferroic GaFeO3 to elucidate its dynamical behavior. Inelastic neutron scattering measurements are performed over a wide temperature range, 150 to 1198 K. First principles lattice…

Materials Science · Physics 2015-06-19 M. K. Gupta , R. Mittal , M. Zbiri , Ripandeep Singh , S. Rols , H. Schober , S. L. Chaplot

We experimentally study the tunability of the cooperativity in coupled spin--cavity systems by changing the magnetic state of the spin system via an external control parameter. As model system, we use the skyrmion host material…

The magneto-electric (ME) coupling on spin-wave resonances in single-crystal Cu2OSeO3 was studied by a novel technique using electron spin resonance combined with electric field modulation. An external electric field E induces a magnetic…

Strongly Correlated Electrons · Physics 2015-06-04 A. Maisuradze , A. Shengelaya , H. Berger , D. M. Djokić , H. Keller

We introduce a one-dimensional model for a CuO chain, with holes and $S=1/2$ spins localized in $3d_{x^2-y^2}$ orbitals, and $p_\sigma$ oxygen orbitals without holes in the ground state. We consider a single hole doped at an oxygen site and…

Strongly Correlated Electrons · Physics 2015-03-30 Krzysztof Bieniasz , Andrzej M. Oleś

The spin-phonon interaction is the dominant process for spin relaxation in Si, and as thermal transport in Si is dominated by phonons, one would expect spin polarization to influence Si's thermal conductivity. Here we report the…

Mesoscale and Nanoscale Physics · Physics 2018-09-07 Paul Lou , Laura de Sousa Oliveira , Chi Tang , Alex Greaney , Sandeep Kumar

We perform a low temperature Raman scattering study of phononic and collective spin excitations in the orthogonal dimers compound SrCu_2(BO_3)_2, focussing on the symmetry and the effects of external fields on the magnetic modes. The zero…

Strongly Correlated Electrons · Physics 2009-11-11 A. Gozar , B. S. Dennis , H. Kageyama , G. Blumberg

Manipulating magnetism at the THz timescale in atomically thin ferromagnets by exploiting the interactions of spins with optical phonon modes presents an innovative idea for THz spintronics and magnonics. Utilizing the coupling of phonon…

The spin-boson model with quadratic coupling is studied using the bosonic numerical renormalization group method. We focus on the dynamical auto-correlation functions $C_{O}(\omega)$, with the operator $\hat{O}$ taken as $\hat{\sigma}_x$,…

Mesoscale and Nanoscale Physics · Physics 2018-11-19 Da-Chuan Zheng , Ning-Hua Tong

We study the magnetically-induced phonon splitting in cubic ACr$_2$O$_4$ (A=Mg, Zn, Cd, Hg) spinels from first principles, and demonstrate that the sign of the splitting, which is experimentally observed to be opposite in CdCr$_2$O$_4$…

Materials Science · Physics 2016-05-04 Aleksander L. Wysocki , Turan Birol

The vibrational properties of ferrimagnetic $\mathrm{Mn_3Si_{2}Te_6}$ single crystals are investigated using Raman spectroscopy and density functional theory calculations. Eighteen Raman-active modes are identified, fourteen of which are…

Strong electron-electron interactions are known to significantly modify the electron-phonon coupling relative to the predictions of density functional theory, but this effect is challenging to calculate with realistic theories of strongly…

Strongly Correlated Electrons · Physics 2025-07-21 David J. Abramovitch , Jennifer Coulter , Sophie Beck , Andrew Millis

While 3$d$-containing materials display strong electron correlations, narrow band widths, and robust magnetism, 5$d$ systems are recognized for strong spin-orbit coupling, increased hybridization, and more diffuse orbitals. Combining these…

Single crystals of the spin-gap system $\rm (VO)_2P_2O_7$ have been investigated by means of Raman scattering. At temperatures below T=75 K~$\approx 2\Delta_{01}({\bf k}=0)$, with $\Delta_{01}$ the singlet-triplet gap, a shoulder appears at…

Superconductivity · Physics 2009-10-31 M. Grove , P. Lemmens , G. Güntherodt , B. C. Sales , F. Büllesfeld , W. Assmus

Effects of coupling between phonon distortions and stripe-like spin waves in the CuO plane of HgBa$_2$CuO$_4$ are studied by band calculations. Local exchange enhancements depend sensitively on the local structure around Cu sites.…

Superconductivity · Physics 2009-11-07 T. Jarlborg

Using Raman scattering we studied the effect of substitutions on 1D spin fluctuations in CuGeO_3 observed as a spinon continuum in frustration induced exchange scattering. For temperatures below the spin-Peierls transition (T_{SP}=14K) the…

Strongly Correlated Electrons · Physics 2016-08-31 M. Fischer , P. Lemmens , G. Güntherodt , M. Weiden , W. Richter , C. Geibel , F. Steglich

CuCrO2 is a manifestation of a two-dimensional triangular antiferromagnet which exhibits an incommensurate noncollinear magnetic structure similar to a classical 120 degree ordering. Using the inelastic neutron scattering technique, direct…

Strongly Correlated Electrons · Physics 2016-09-21 Kisoo Park , Joosung Oh , Jonathan C. Leiner , Jaehong Jeong , Kirrily C. Rule , Manh Duc Le , Je-Geun Park