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We present the Raman scattering results on layered 2D semiconducting ferromagnetic compound CrSiTe$_3$. Four Raman active modes, predicted by symmetry, have been observed and assigned. The experimental results are supported by DFT…

Materials Science · Physics 2018-10-16 A. Milosavljević , A. Šolajić , J. Pešić , Yu Liu , C. Petrovic , N. Lazarević , Z. V. Popović

The magnetic field--driven transition in the spin-Peierls system CuGeO_3 associated with the closing of the spin gap is investigated numerically. The field dependence of the spin dynamical structure factor (seen by inelastic neutron…

Strongly Correlated Electrons · Physics 2009-10-30 D. Poilblanc , J. Riera , C. A. Hayward , C. Berthier , M. Horvatic

A spin and phonon excitations spectrum are studied using quantum Monte Carlo method in antiferromagnetic chain with spins $S=1/2$ coupled nonadiabaticity with acoustic phonons . It is found the critical coupling exists to open gap in the…

Soft Condensed Matter · Physics 2007-05-23 S. S. Aplesnin

The thermal conductivity of the Spin-Peierls (SP) compound CuGeO_3 was measured in magnetic fields up to 16 T. Above the SP transition, the heat transport due to spin excitations causes a peak at around 22 K, while below the transition the…

Strongly Correlated Electrons · Physics 2009-10-31 Yoichi Ando , J. Takeya , D. L. Sisson , S. G. Doettinger , I. Tanaka , R. S. Feigelson , A. Kapitulnik

The mechanism of spin-phonon coupling in high-T$_C$ copper oxides is explored from band calculations on La$_{(2-x)}$Sr$_x$CuO$_4$ and HgBa$_2$CuO$_4$ systems. The LMTO band calculations, based on the local density approximation, are made…

Materials Science · Physics 2015-06-25 T. Jarlborg

We report on infrared, Raman, magnetic susceptibility, and specific heat measurements on CdCr2O4 and ZnCr2O4 single crystals. We estimate the nearest-neighbor and next-nearest neighbor exchange constants from the magnetic susceptibility and…

Strongly Correlated Electrons · Physics 2010-02-03 Ch. Kant , J. Deisenhofer , T. Rudolf , F. Mayr , F. Schrettle , A. Loidl , V. Gnezdilov , D. Wulferding , P. Lemmens , V. Tsurkan

Direct experimental evidence of spin-phonon coupling in CrSBr is provided by the temperature dependent Cr L-edge resonant inelastic x-ray scattering (RIXS) spectra. Zone-center optical phonons are observed exclusively in the low-temperature…

The infrared phonon spectrum of the spinel CdCr2O4 is measured as a function temperature from 6 K to 300K. The triply degenerate Cr phonons soften in the paramagnetic phase as temperature is lowered below 100 K and then split into a singlet…

Materials Science · Physics 2009-11-13 R. Valdés Aguilar , A. B. Sushkov , Y. J. Choi , S-W. Cheong , H. D. Drew

By applying Wannier-based extended Kugel-Khomskii model, we carry out first-principles calculations and electronic structure analysis to understand the spin-phonon coupling effect in transition-metal perovskites. We demonstrate the…

Materials Science · Physics 2017-08-17 Hongwei Wang , Lixin He , Hong Jiang , Cameron Steele , Xifan Wu

Spin-orbit interaction is an important vehicle for spin relaxation. At finite temperature lattice vibrations modulate the spin-orbit interaction and thus generate a mechanism for spin-phonon coupling, which needs to be incorporated in any…

Materials Science · Physics 2018-09-26 Subhayan Roychoudhury , Stefano Sanvito

Band calculations on HgBa$_2$CuO$_4$ and La$_{(2-x)}$Sr$_x$CuO$_4$ with phonon and spin-waves within the CuO planes show that partial gaps are created at various energies depending on wavelengths. Spin and phonon gaps appear at different…

Superconductivity · Physics 2009-11-11 T. Jarlborg

The heat transport in a system of $S=1/2$ large-$J$ Heisenberg spin chains, describing closely Sr$_2$CuO$_3$ and SrCuO$_2$ cuprates, is studied theoretically at $T\ll J$ by considering interactions of the bosonized spin excitations with…

Strongly Correlated Electrons · Physics 2016-01-11 A. L. Chernyshev , A. V. Rozhkov

The microscopic description of the spin-Peierls transition in pure and doped CuGeO_3 is developed taking into account realistic details of crystal structure. It it shown that the presence of side-groups (here Ge) strongly influences…

Condensed Matter · Physics 2009-10-28 D. Khomskii , W. Geertsma , M. Mostovoy

Raman study on a select few orthochromites, RCrO$_3$ (R = Y, Lu, Gd, Eu and Sm) shows that the phonon behavior at TN in compounds with magnetic R-ion (Gd and Sm) is remarkably different from that of non-magnetic R-ion (Y, Lu and Eu). While…

Materials Science · Physics 2013-06-11 Venkata Srinu Bhadram , B. Rajeswaran , A. Sundaresan , Chandrabhas Narayana

Polarization- and temperature-dependent Raman data along with theoretical simulations are presented for the Kagome ferromagnet Fe_3Sn_2. Eight out of nine expected phonon modes were identified. The experimental energies compare well with…

The optical conductivity of the CuO$_3$-chains, a subsystem of the 1-2-3 materials, is dominated by a broad peak in the mid-infrared ($\omega \approx 0.2$eV), and a slowly falling high-frequency tail. The 1D $t$-$J$-model is proposed as the…

Condensed Matter · Physics 2009-10-22 Roland Fehrenbacher

Materials having strong coupling between different degrees of freedom such as spin, lattice, orbital, and charge are of immense interest due to their potential device applications. Here, we have stabilized the 9R phase of BaMnO3, by Sr (Ti)…

Materials Science · Physics 2021-10-27 Bommareddy Poojitha , Anjali Rathore , Surajit Saha

Band calculations show that a stripe-like anti-ferromagnetic spin wave is enforced by a 'half-breathing' phonon distortion within the CuO plane of HgBa_2CuO_4. This spin-phonon coupling is increased further by shear distortion and by…

Superconductivity · Physics 2009-11-10 T. Jarlborg

Raman scattering measurements on BiFeO3 single crystals show an important coupling between the magnetic order and lattice vibrations. The temperature evolution of phonons shows that the lowest energy E and A1 phonon modes are coupled to the…

Strongly Correlated Electrons · Physics 2010-10-12 P. Rovillain , M. Cazayous , Y. Gallais , A. Sacuto , R. P. S. M. Lobo , D. Lebeugle , D. Colson

MnV$_2$O$_4$ in the spinel structure is known to exhibit coupled orbital and spin ordering, and its Raman spectra show interesting anomalies in its low-temperature phase. With a goal to explain this behavior involving coupled spins and…

Materials Science · Physics 2020-05-27 Dibyendu Dey , T. Maitra , U. V. Waghmare , A. Taraphder