Related papers: Quantum Fluctuations in Large-Spin Molecules
The majority of nuclei available for study in solid state Nuclear Magnetic Resonance have half-integer spin $I > 1/2 $, with corresponding electric quadrupole moment. As such, they may couple with a surrounding electric field gradient. This…
Due to quantum fluctuations, a black hole of mass $M$ represents an average over an ensemble of black hole geometries with angular momentum. This observation is apparently at odds with the fact that the curvature singularity inside a…
Magnetization measurements of Mn12 molecular nanomagnets with spin ground states of S = 10 and S = 19/2 showresonance tunneling at avoided energy level crossings. The observed oscillations of the tunnel probability as a function of the…
We investigate the dynamics of a large anisotropic spin whose easy-axis component is coupled to a bosonic bath with a spectral function $J(\w)\propto \omega^s$. Such a spin complex might be realized in a single-molecular magnet. Using the…
We theoretically investigate the role of spin fluctuations in charge transport through a magnetic junction. Motivated by recent experiments that measure a nonlinear dependence of the current on electrical bias, we develop a systematic…
Current theories still fail to give a satisfactory explanation of the observed quantum phenomena in the relaxation of the magnetisation of the molecular cluster Mn12 acetate. In the very low temperature regime, Prokof'ev and Stamp recently…
We address the issue of accurately treating interaction effects in the mesoscopic regime by investigating the ground state properties of isolated irregular quantum dots. Quantum Monte Carlo techniques are used to calculate the distributions…
We study electronic transport through a magnetic molecule with an intrinsic spin $S$ coupled to two magnetic electrodes, in the incoherent regime. The molecule is modeled as a single resonant level with large Coulomb repulsion (no double…
In this work, the many-spin interactions taking place in Mn12 large-spin clusters are extensively studied using the 8-spin model Hamiltonian, for which we determine the possible parameters based on experimental data. Account of the…
Currently under active study in condensed matter physics, both theoretically and experimentally, are quantum spin liquid (QSL) states, in which no long-range magnetic ordering appears at low temperatures due to strong quantum fluctuations…
We report on a complex nontrivial behavior of the optical anisotropy of quantum dots that is induced by a magnetic field in the plane of the sample. We find that the optical axis either rotates in the opposite direction to that of the…
This article takes a broad view of the understanding of magnetic bistability and magnetic quantum tunneling in single-molecule magnets (SMMs), focusing on three families of relatively simple, low-nuclearity transition metal clusters: spin S…
Quantum nanomagnets can show a field dependence of the relaxation time very different from their classical counterparts, due to resonant tunneling via excited states (near the anisotropy barrier top). The relaxation time then shows minima…
We use the high sensitivity to magnetic flux of mesoscopic conductance fluctuations in large quantum dots to investigate changes in the two-dimensional electron dispersion caused by an in-plane magnetic field. In particular, changes in…
When probing nuclear spins in materials on the nanometer scale, random fluctuations of the spin polarization will exceed the mean Boltzmann polarization for sample volumes below about (100nm)^3. In this work, we use magnetic resonance force…
Few examples of magnetic systems displaying a transition to pure dipolar magnetic order are known to date, and single-molecule magnets can provide an interesting example. The molecular cluster spins and thus their dipolar interaction energy…
We investigate the interplay of quantum fluctuations and magnetic anisotropies in metallic ferromagnets. Our central result is that fluctuations close to a quantum critical point can drive the moments to point along a magnetic hard axis. As…
It is shown, by considering the case of the harmonic oscillator, that quantum fluctuations may be the most significant contribution to the random walk of a single molecule. From this point, the controversy on the existence of a standard…
We study the effects of quantum fluctuations and the excitation spectrum for the antiferromagnetic Heisenberg model on a two-dimensional quasicrystal, by numerically solving linear spin-wave theory on finite approximants of the octagonal…
We present the results of a comprehensive magneto-optical characterization of single CdTe quantum dots containing a few Mn2+ ions. We find that some quantum dots exhibit an unexpected evolution of excitonic photoluminescence spectrum with…