Related papers: Quantum Fluctuations in Large-Spin Molecules
Molecular nanomagnets, besides promising to open new frontiers in technology, have attracted huge interest in the scientific community because they can exhibit the phenomenon known as quantum tunnelling of the magnetization, i.e. coherent…
A single-molecule magnet placed in a magnetic field perpendicular to its anisotropy axis can be truncated to an effective two-level system, with easily tunable energy splitting. The quantum coherence of the molecular spin is largely…
The nonlinear dynamical response of Mn$_{12}$ single-molecule magnets is experimentally found to be very large, quite insensitive to the spin-lattice coupling constant, and displaying peaks reversed with respect to classical…
Molecular spin clusters are mesoscopic systems whose structural and physical features can be tailored at the synthetic level. Besides, their quantum behavior is directly accessible in laboratory and their magnetic properties can be…
Recent experimental results point to the existence of coherent quantum phenomena in systems made of a large number of particles, despite the fact that for many-body systems the presence of decoherence is hardly negligible and emerging…
One way to look for complex behaviours in many-body quantum systems is to let the number $N$ of degrees of freedom become large and focus upon collective observables. Mean-field quantities scaling as $1/N$ tend to commute, whence complexity…
The thermal activation of magnetization reversal in magnetic nanoparticles is controlled by the anisotropy-energy barrier. Using perturbation theory, exact diagonalization and stability analysis of the ferromagnetic spin-s Heisenberg model…
The variation with microwave frequency and temperature of previously reported anomalous peaks in the EPR spectra of Mn12-acetate, under large transverse fields, reveals that the molecular easy magnetization axes are tilted with respect to…
We review the present state of theory and experiments on the quantum tunneling of magnetization in mesoscopic spin systems. Most attention is paid to the relaxation of magnetization in the molecular complexes Mn12 and Fe8. The role of the…
This thesis contains a thorough investigation of the quantum spin dynamics in Mn12-ac and Mn6 Single-molecule magnets. In particular, we have investigated the interplay between quantum tunneling of magnetization and nuclear spin dynamics in…
We summarize the present status of the theories of spin fluctuations in dealing with the anomalous or non-Fermi liquid behavior and unconventional superconductivity in strongly correlated electron systems around their magnetic instabilities…
We calculate the mesoscopic fluctuations of the magnetic anisotropy of ferromagnetic nanoparticles. A microscopic spin-orbit Hamiltonian considered as a perturbation of the much stronger exchange interaction first yields an explicit…
Starting from a phenomenological Hamiltonian originally written in terms of angular momentum operators we derive a new quantum angle-based Hamiltonian that allows for a discussion on the quantum spin tunneling. The study of the…
The spin relaxation in the molecular magnet \Mn12 is investigated by a novel type of high-frequency magnetic spectroscopy. By reversing the external magnetic field the intensities of the $|\pm 10>\to |\pm 9>$ transitions within the ground…
We show that the nuclear spin dynamics in the single-molecule magnet Mn12-ac below 1 K is governed by quantum tunneling fluctuations of the cluster spins, combined with intercluster nuclear spin diffusion. We also obtain the first…
The phenomenon of Quantum Tunneling of Mesoscopic Spins is reviewed in the light of the behavior of the archetype of these systems: the molecular complex Mn12-ac. Most observations can be understood in the framework of the reduced Hilbert…
Investigations of spin squeezing in ensembles of quantum particles have been limited primarily to a subspace of spin fluctuations and a single spatial mode in high-spin and spatially extended ensembles. Here, we show that a wider range of…
Quantum spin fluctuations provide a unique way to study spin dynamics without system perturbation. Here we put forward an optical resonance shift spin noise spectroscopy as a powerful tool to measure the spin noise of various systems from…
For quantum fluids, the role of quantum fluctuations may be significant in several regimes such as when the dimensionality is low, the density is high, the interactions are strong, or for low particle numbers. In this paper we propose a…
Spin currents may be generated by applying bias voltages V to the nanostructures even in the absence of spin-active ferromagnetic interfaces. Most theoretical proposals concentrate on a concrete spin-orbit interaction and on the…