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We investigate theoretically the phase diagram of an insoluble charged surfactant monolayer in contact with a semi-dilute polyelectrolyte solution (of opposite charge). The polyelectrolytes are assumed to have long-range and attractive…

Soft Condensed Matter · Physics 2012-07-19 Adi Shafir , David Andelman

We show that charge inversion, i.e. interfacial charges attracting counterions in excess of their own nominal charge, is a general effect that takes place in most charged systems next to aqueous solutions with multivalent ions and identify…

Soft Condensed Matter · Physics 2007-05-23 J. Faraudo , A. Travesset

A model for ionic solutions with an attractive short-range pair interaction between the ions is presented. The short-range interaction is accounted for by adding a quadratic non-local term to the Poisson-Boltzmann free energy. The model is…

Soft Condensed Matter · Physics 2009-10-31 Yoram Burak , David Andelman

We investigate the thermodynamic properties of a polyelectrolyte solution in a presence of {\it multivalent} salts. The polyions are modeled as rigid cylinders with the charge distributed uniformly along the major axis. The solution,…

Condensed Matter · Physics 2015-06-25 Paulo S. Kuhn , Yan Levin , Marcia C. Barbosa

Screening of a macroion by multivalent counterions is considered. It is shown that ions form strongly correlated liquid at the macroion surface. Cohesive energy of this liquid leads to strong additional attraction of counterions to the…

Soft Condensed Matter · Physics 2009-10-31 V. I. Perel , B. I. Shklovskii

We study sedimentation equilibrium of low-salt suspensions of binary mixtures of charged colloids, both by Monte Carlo simulations of an effective colloids-only system and by Poisson-Boltzmann theory of a colloid-ion mixture. We show that…

Soft Condensed Matter · Physics 2009-11-11 M. Dijkstra , J. Zwanikken , R. van Roij

We analyze solutions of strongly charged chains bridged by linkers such as multivalent ions. The gelation induced by the strong short range electrostatic attractions is dramatically suppressed by the long range electrostatic correlations…

Condensed Matter · Physics 2009-11-07 A. V. Ermoshkin , M. Olvera de la Cruz

In solution, electrically like-charged particles can experience a strong and long-ranged attraction that leads to the formation of stable, slowly reorganizing clusters. The attractive force underpinning this spontaneous organization process…

Soft Condensed Matter · Physics 2026-01-14 Sida Wang , Angela Le , Rowan Walker-Gibbons , Madhavi Krishnan

Conditions at which a quasi-one-dimensional (1D) electron system can be considered as a quantum liquid of impenetrable charged particles are theoretically analyzed. In the presence of an inert, neutralizing background, a motion of…

Superconductivity · Physics 2024-06-21 Yu. P. Monarkha

Counterion distribution around an isolated flexible polyelectrolyte in the presence of a divalent salt is evaluated using the adsorption model [M. Muthukumar, J. Chem. Phys. {\bf 120}, 9343 (2004)] that considers Bjerrum length, salt…

Soft Condensed Matter · Physics 2008-12-29 Arindam Kundagrami , M. Muthukumar

The formation of inter-polyelectrolyte complexes from the association of oppositely charged polymers in an electrolyte is studied. The charged polymers are linear oppositely charged polyelectrolytes, with possibly a neutral block. This…

Soft Condensed Matter · Physics 2012-06-27 Vladimir A. Baulin , Emmanuel Trizac

We are interested in rationalizing the phenomenon of like-charge attraction between charged bodies, such as a pair of colloids, in the strong coupling regime. The two colloids are modelled as uniformly charged parallel plates, neutralized…

Soft Condensed Matter · Physics 2025-01-13 L. Samaj , E. Trizac , M. Trulsson

The complexation of a polyelectrolyte with an oppositely charged spherical macroion is studied for both salt free and salty solutions. When a polyelectrolyte winds around the macroion, its turns repel each other and form an almost…

Soft Condensed Matter · Physics 2009-10-31 T. T. Nguyen , B. I. Shklovskii

We explore interactions between equally charged surfaces, in the presence of simple salt and either neutral or monovalently charged polyampholytes. We consider the possibility of using these charged polymers as crude models of ion clusters.…

Soft Condensed Matter · Physics 2026-03-19 David Ribar , Clifford E Woodward , Jan Forsman

We report results from a molecular dynamics (MD) simulation on the conformations of a long flexible polyelectrolyte complexed to a charged sphere, \textit{both negatively charged}, in the presence of neutralizing counterions in the strong…

Soft Condensed Matter · Physics 2009-11-07 Rene Messina , Christian Holm , Kurt Kremer

In mixtures of colloids and nonadsorbing polyelectrolytes, a Donnan potential arises across the region between surfaces that are depleted of polyelectrolyte and the rest of the system. This Donnan potential tends to shift the…

Soft Condensed Matter · Physics 2022-10-27 Jasper Landman , Max P. M. Schelling , Remco Tuinier , Mark Vis

Experiments with polymer latex solutions show the coexistence of order-disorder structures of macroions. Because of the large macroions' sizes, this order-disorder phase coexistence imply the existence of very long-range attractive and…

Soft Condensed Matter · Physics 2019-02-20 Alfredo González-Calderón , Enrique González-Tovar , Marcelo Lozada-Cassou

Like-charge attraction, driven by ionic correlations, challenges our understanding of electrostatics both in soft and hard matter. For two charged planar surfaces confining counterions and water, we prove that even at relatively low…

Soft Condensed Matter · Physics 2023-03-15 Ivan Palaia , Abhay Goyal , Emanuela del Gado , Ladislav Šamaj , Emmanuel Trizac

A mean-field theory based on Gibbs-Bogoliubov inequality is constructed to study the interactions between two like-charged polyions. It is shown that contrary to the previously established paradigm, a properly constructed mean-field theory…

Soft Condensed Matter · Physics 2009-10-31 Jeferson J. Arenzon , Yan Levin , Juergen F. Stilck

We study a 2D system of identical mobile particles on the surface of a cylinder of finite length $d$ and circumference $W$, immersed in a medium of dielectric constant $\varepsilon$. The two end-circles of the cylinder are like-charged with…

Statistical Mechanics · Physics 2020-11-24 Ladislav Šamaj