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We present a theory for analyzing residence times of single molecules in a fixed detection area of a scanning tunneling microscope (STM). The approach is developed for one-dimensional molecule diffusion and can be extended to two dimensions…

Mesoscale and Nanoscale Physics · Physics 2022-08-23 Christoph Schiel , Philipp Rahe , Philipp Maass

Molecular dynamics simulations are utilized to study the melting transition in pentane (C5H12) and heptane (C7H16), physisorbed onto the basal plane of graphite at near-monolayer coverages. Through use of the newest, optimized version of…

Materials Science · Physics 2009-11-11 Cary L. Pint

Local deformation of atomically thin van der Waals materials provides a powerful approach to create site-controlled chip-compatible single-photon emitters (SPEs). However, the microscopic mechanisms underlying the formation of such…

Machine learning (ML) methods are extraordinarily successful at denoising photographic images. The application of such denoising methods to scientific images is, however, often complicated by the difficulty in experimentally obtaining a…

Smectic liquid crystals are materials formed by stacking deformable, fluid layers. Though smectics prefer to have flat, uniformly-spaced layers, boundary conditions can impose curvature on the layers. Since the layer spacing and curvature…

Differential Geometry · Mathematics 2007-05-23 Randall D. Kamien , Christian D. Santangelo

Organic molecules are widely present in the dense interstellar medium, and many have been synthesized in the laboratory on Earth under the conditions typical for an interstellar environment. Until now, however, only relatively small…

Biological Physics · Physics 2022-02-25 S. A. Krasnokutski , K. -J. Chuang , C. Jäger , N. Ueberschaar , Th. Henning

A method is proposed for generating and discriminating Bell states of high fidelity from consecutive single-photons generated in a semiconductor quantum dot. The use of a non-symmetric beam splitter is found to be essential and sufficient,…

Quantum Physics · Physics 2012-09-17 Partha Ghose

The recently developed two-stage growth model of synthesis of monodispersed polycrystalline colloidal particles is utilized and improved to explain growth of uniform cadmium sulfide spheres. The model accounts for the coupled processes of…

Soft Condensed Matter · Physics 2010-09-22 Sergiy Libert , Vyacheslav Gorshkov , Dan Goia , Egon Matijevic , Vladimir Privman

Alkylsilane self-assembled monolayers (SAMs) are often used as model substrates for their ease of preparation and hydrophobic properties. We have observed that these atomically smooth monolayers also provide a slip boundary condition for…

In complex plasmas, the behavior of freely floating micrometer sized particles is studied. The particles can be directly visualized and recorded by digital video cameras. To analyze the dynamics of single particles, reliable algorithms are…

Plasma Physics · Physics 2018-02-14 Daniel P. Mohr , Christina A. Knapek , Peter Huber , Erich Zaehringer

We report on a novel scheme to perform efficient simulations of Scanning Tunneling Microscopy (STM) of molecules weakly bonded to surfaces. Calculations are based on a tight binding (TB) technique including self-consistency for the molecule…

Materials Science · Physics 2009-11-11 M. Dubois , S. Latil , L. Scifo , B. Grevin , A. Rubio

We calculate bending moduli along the principal directions for thirty-two select atomic monolayers using ab initio Density Functional Theory (DFT). Specifically, considering representative materials from each of Groups IV, V, III-V…

Materials Science · Physics 2020-06-11 Shashikant Kumar , Phanish Suryanarayana

Planar, disordered assemblies of small particles incorporated in layered media -- sometimes called ``disordered metasurfaces'' in the recent literature -- are becoming widespread in optics and photonics. Their ability to scatter light with…

Optics · Physics 2023-08-08 Kevin Vynck , Armel Pitelet , Louis Bellando , Philippe Lalanne

When thin films are grown on a substrate by chemical vapor deposition, the evolution of the first deposited layers may be described, on mesoscopic scales, by dynamical models of the reaction-diffusion type. For monoatomic layers, such…

Mesoscale and Nanoscale Physics · Physics 2015-06-16 Daniel Walgraef

We study the self-assembly on a spherical surface of a model for a binary mixture of amphiphilic dimers in the presence of guest particles via Monte Carlo (MC) computer simulation. All particles have a hard core, but one monomer of the…

Soft Condensed Matter · Physics 2021-06-11 Nkosinathi Dlamini , Santi Prestipino , Giuseppe Pellicane

Macromolecules can form regular structures on inert surfaces. We have developed a combined empirical and modeling approach to derive the bonding. From experimental scanning tunneling microscopy (STM) images of structures formed on Au(111)…

A microscopic theory of the transport in a scanning tunnelling microscope (STM) set-up is introduced for \pi-conjugated molecules on insulating films, based on the density matrix formalism. A key role is played in the theory by the energy…

Mesoscale and Nanoscale Physics · Physics 2012-05-23 Sandra Sobczyk , Andrea Donarini , Milena Grifoni

We present a newly developed facility, comprised of a combinatorial laser molecular beam epitaxy system and an in-situ scanning tunneling microscopy (STM). This facility aims at accelerating the materials research in a highly efficient way,…

Applied Physics · Physics 2020-03-26 Ge He , Zhongxu Wei , Zhongpei Feng , Xiaodong Yu , Beiyi Zhu , Li Liu , Kui Jin , Jie Yuan , Qing Huan

A mean field rate theory description of the homo- and co-polymerization of $f$-functional molecules is developed, which contains the formation of short cyclic structures inside the network. The predictions of this model are compared with…

Soft Condensed Matter · Physics 2021-03-31 Michael Lang , Konrad Schwenke , Jens-Uwe Sommer

Polarized atomic beam sources have been in operation since many years to produce either nuclear polarized atomic hydrogen or deuterium beams. In recent experiments such a source was used to polarize both isotopes independently at the same…

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