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The properties of amorphous solid water at and near the calorimetric glass transition temperature, $T_{g}$, of 136 K have been debated for years. One hypothesis is that water turns into a "true" liquid at $T_{g}$ (i.e., it becomes ergodic)…

Soft Condensed Matter · Physics 2025-03-03 Greg A. Kimmel , Megan K. Dunlap , Kirill Gurdumov , R. Scott Smith , Loni Kringle , Bruce D. Kay

We report the results of a density-functional study of the diffusion of Pt dimers on the (111) surface of Pt. The calculated activation energy of 0.37 eV is in {\em exact} agreement with the recent experiment of Kyuno {\em et al.}…

Materials Science · Physics 2009-10-31 Ghyslain Boisvert , Laurent J. Lewis

We propose a theoretical approach for predicting thermodynamics and kinetics of guest molecules in nanoporous materials. This statistical mechanical-based method requires a minimal set of physical parameters that may originate from…

The charge transfer (ionization) of hydrogen Rydberg atoms (principal quantum number $n=25-34$) incident at a Cu(100) surface is investigated. Unlike fully metallic surfaces, where the Rydberg electron energy is degenerate with the…

Chemical Physics · Physics 2016-06-22 J. A. Gibbard , M. Dethlefsen , M. Kohlhoff , C. J. Rennick , E. So , M. Ford , T. P. Softley

Under strong electric fields, an arc of strong current flowing through plasma can link two metal surfaces even in ultra high vacuum. Despite decades of research, the chain of events leading to vacuum arc breakdowns is hitherto unknown.…

Materials Science · Physics 2022-09-30 Jyri Kimari , Ye Wang , Andreas Kyritsakis , Veronika Zadin , Flyura Djurabekova

Using numerical simulations, we perform an extensive finite-size analysis of the transverse diffusion coefficient in a sheared 2D amorphous solid, over a broad range of strain rates, at temperatures up to the supercooled liquid regime. We…

Materials Science · Physics 2015-05-27 Joyjit Chattoraj , Christiane Caroli , Anaël Lemaître

Recently developed quantum mechanical theory of inelastic He atom scattering (HAS) from solid surfaces is employed to analyze the energy transfer between projectile particles (thermal energy He-atoms) and vibrational degrees of freedom…

Statistical Mechanics · Physics 2007-05-23 A. Siber , B. Gumhalter , J. P. Toennies

Based on the phenomenological theory of heat diffusion, we show that the generated peak temperature $T_{\text{max}}$ after absorption of a laser pulse strongly depends on the pulse duration. We identify three different heat conduction…

Applied Physics · Physics 2020-02-26 Roman Shayduk , Peter Gaal

An investigation of the effect of surface diffusion in random deposition model is made by analytical methods and reasoning. For any given site, the extent to which a particle can diffuse is decided by the morphology in the immediate…

Soft Condensed Matter · Physics 2011-12-14 Baisakhi Mal , Subhankar Ray , J. Shamanna

We propose to revisit the diffusion of atoms in the Knudsen regime in terms of a complex dynamical reflection process. By means of molecular dynamics simulation we emphasize the asymptotic nature of the cosine law of reflection at the…

Statistical Mechanics · Physics 2009-11-13 Franck Celestini , Fabrice Mortessagne

The effects of thermal diffuse scattering on the transmission and eventual diffraction of highly accelerated electrons are investigated with a method that incorporates the frozen phonon approximation to the exact numerical solution of the…

Computational Physics · Physics 2018-01-22 S. Rudinsky , A. S. Sanz , R. Gauvin

Molecular dynamics simulation is employed to understand the thermodynamic behavior of cuboctahedron (cub) and icosahedron (ico) nanoparticles with 2-20 number of shells (55-28741 atoms). The embedded atom method was used to describe the…

Materials Science · Physics 2019-08-13 Maryam Azadeh , Movaffaq Kateb , Pirooz Marashi

It is common practice to discuss the temperature effect on molecular dynamics of glass formers above the melting temperature in terms of the Arrhenius law. Using dielectric spectroscopy measurements of dc-conductivity and structural…

Materials Science · Physics 2018-04-26 Erik Thoms , Andrzej Grzybowski , Sebastian Pawlus , Marian Paluch

We have used the indium/copper surface alloy to study the dynamics of surface vacancies on the Cu(001) surface. Individual indium atoms that are embedded within the first layer of the crystal, are used as probes to detect the rapid…

Materials Science · Physics 2007-05-23 R. van Gastel , E. Somfai , S. B. van Albada , W. van Saarloos , J. W. M. Frenken

Time-resolved vibrational spectroscopy constitutes an invaluable experimental tool for monitoring hot-carrier induced surface reactions. However, the absence of a full understanding on the precise microscopic mechanisms causing the…

Materials Science · Physics 2019-01-14 D. Novko , J. C. Tremblay , M. Alducin , J. I. Juaristi

Overdamped motion of Brownian particles in tilted piecewise linear periodic potentials is considered. Explicit algebraic expressions for the diffusion coefficient, current, and coherence level of Brownian transport are derived. Their…

Soft Condensed Matter · Physics 2009-11-10 Els Heinsalu , Risto Tammelo , Teet Ord

We present energy- and charge-resolved measurements of low and hyperthermal energy Na+ ions scattered from a Ag(001) surface. With the primary ion beam oriented along the [110] crystal direction, distinct peaks in the energy distributions…

Mesoscale and Nanoscale Physics · Physics 2015-04-02 M. P. Ray , R. E. Lake , J. B. Marston , C. E. Sosolik

Diffusion processes are fundamental in modelling stochastic dynamics in natural sciences. Recently, simulating such processes on complicated geometries has found applications for example in biology, where toroidal data arises naturally when…

Probability · Mathematics 2019-06-25 Mathias Højgaard Jensen , Anton Mallasto , Stefan Sommer

Event-by-event hydrodynamics is applied to Cu-Au collisions at 200GeV. Predictions for charged particle distributions in pseudorapidity, transverse momentum spectra, femtoscopy radii are given. The triangular and elliptic flow coefficients…

Nuclear Theory · Physics 2012-10-09 Piotr Bozek

To control and utilize quantum features in small scale for practical applications such as quantum transport, it is crucial to gain deep understanding of quantum characteristics of states such as coherence. Here by introducing a technique…

Quantum Physics · Physics 2018-01-03 Laleh Memarzadeh , Azam Mani