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Ring torsion effects on optical excitation properties in poly(para-phenylene) (PPP) and polyaniline (PAN) are investigated by the intermediate exciton formalism. Long-range excitons are characterized, and the long-range component of the…

Soft Condensed Matter · Physics 2008-02-03 Kikuo Harigaya

Component of photoexcited states with large spatial extent is investigated for optical absorption spectra of the electroluminescent conjugated polymers by using the intermediate exciton theory. We calculate the ratio of oscillator strengths…

Soft Condensed Matter · Physics 2008-02-03 Kikuo Harigaya

The component of photoexcited states with large spatial extent is investigated for poly(para-phenylenevinylene) using the intermediate exciton theory. We find a peak due to long-range excitons at the higher-energy side of the lowest main…

Condensed Matter · Physics 2008-02-03 Kikuo Harigaya

The two state molecular orbital (2-MO) model of the phenyl based semiconductors is used to calculate the low-lying spectra of the Ag and Bu states of poly(para-phenylene) (PPP). The model parameters are determined by fitting its predictions…

Condensed Matter · Physics 2009-10-31 W. Barford , R. J. Bursill , M. Yu. Lavrentiev

We perform ab initio calculations of optical properties for a typical semiconductor conjugated polymer, poly-para-phenylenevinylene, in both isolated chain and crystalline packing. In order to obtain results for excitonic energies and…

Materials Science · Physics 2009-11-07 Alice Ruini , Marilia J. Caldas , Giovanni Bussi , Elisa Molinari

We investigate the effects of disorder on Frenkel excitons in disordered conjugated polymers with allowed rotations about single bonds. In these materials, the principal effect of the disorder is to modify the transfer integrals appearing…

Disordered Systems and Neural Networks · Physics 2007-05-23 I. Avgin , D. L. Huber

Electronic structures and optical excitations in Moebius conjugated polymers are studied theoretically. Periodic and Moebius boundary conditions are applied to the tight binding model of poly(para-phenylene), taking exciton effects into…

Materials Science · Physics 2007-05-23 Kikuo Harigaya

A phenomenological coupled exciton model is proposed in order to characterize optical excitations in extended dendrimers. An onsite exciton state is assigned at each phenyl rings and a nearest neighbor hopping integral which obeys the…

Materials Science · Physics 2016-08-31 Kikuo Harigaya

A phenomenological coupled exciton model is proposed in order to characterize optical excitations in extended dendrimers. An onsite exciton state is assigned at each phenyl rings and a nearest neighbor hopping integral which obeys the…

Condensed Matter · Physics 2017-09-13 Kikuo Harigaya

We study the effect of magnetic field and geometric confinement on excitons confined to a quantum ring. We use analytical matrix elements of the Coulomb interaction and diagonalize numerically the effective-mass Hamiltonian of the problem.…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Jakyoung Song , Sergio E. Ulloa

Exciton effects on conjugated polymers are investigated in the soliton lattice system. We use the Su-Schrieffer-Heeger model with long-range Coulomb interactions treated by the single-excitation configuration-interaction method. The soliton…

Condensed Matter · Physics 2008-02-03 Kikuo Harigaya , Yukihiro Shimoi , Shuji Abe

Electronic structures and optical excitations in Moebius conjugated polymers are studied theoretically. Periodic and Moebius boundary conditions are applied to the tight binding model of poly(para-phenylene), taking into account of the…

Materials Science · Physics 2007-05-23 Kikuo Harigaya

The effects of the electron-phonon interaction on optical excitations can be understood in terms of exciton-phonon coupling, and require a careful treatment in low-dimensional materials with strongly bound excitons or strong electron-hole…

Materials Science · Physics 2022-02-17 Gabriel Antonius , Steven G. Louie

The problem of long-range correlations of particles produced in high- energy collisions is discussed. Long-range correlations involve large groups of particles. Among them are, e.g., those correlations which lead to ring-like and elliptic…

High Energy Physics - Phenomenology · Physics 2016-09-06 I. M. Dremin

We study theoretically the optical properties of an exciton in a two-dimensional ring threaded by a magnetic flux. We model the quantum ring by a confining potential that can be continuously tuned from strictly one-dimensional to truly…

Mesoscale and Nanoscale Physics · Physics 2011-12-05 C. González-Santander , F. Domínguez-Adame , R. A. Römer

Structural relaxations in electronically excited poly(para-phenylene) are studied using many-body perturbation theory and density-functional-theory methods. A sophisticated description of the electron-hole interaction is required to…

Materials Science · Physics 2009-11-10 Emilio Artacho , M. Rohlfing , M. Cote , P. D. Haynes , R. J. Needs , C. Molteni

In this paper we present results of large-scale correlated calculations of triplet photoinduced absorption (PA) spectrum of oligomers of poly-(para)phenylenevinylene (PPV) containing up to five phenyl rings. In particular, the high-energy…

Condensed Matter · Physics 2010-01-14 Alok Shukla

This is a review of exciton dynamics in conjugated polymers. Exciton dynamics encompass multiple time and length scales. Ultrafast femtosecond processes are intrachain and involve a quantum mechanical correlation of the exciton and nuclear…

Chemical Physics · Physics 2021-02-15 William Barford

Exciton-phonon dynamics on a 1D lattice with long-range exciton-exciton interaction have been introduced and elaborated. Long-range interaction leads to a nonlocal integral term in the motion equation of the exciton subsystem if we go from…

Mathematical Physics · Physics 2011-04-08 Nick Laskin

The exciton relaxation dynamics of photoexcited electronic states in poly($p$-phenylenevinylene) (PPV) are theoretically investigated within a coarse-grained model, in which both the exciton and nuclear degrees of freedom are treated…

Chemical Physics · Physics 2018-02-14 Jonathan R. Mannouch , William Barford , Sarah Al-Assam
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