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A variational approach, based on a discrete representation of the chain, is used to calculate free energy and conformational properties in polyelectrolytes. The true bond and Coulomb potentials are approximated by a trial isotropic harmonic…

chem-ph · Physics 2016-08-15 B. Jönsson , C. Peterson , B. Söderberg

A normal ordered exponential parametrization is used to obtain equations for thermal one-and two-particle reduced density matrices, as well as free energies, partition functions and entropy for both Fermionic (electronic) and Bosonic…

Quantum Physics · Physics 2022-01-12 Marcel Nooijen , Songhao Bao

We propose a pair-condensate variational approach (PCV) to determine a set of the most important collective pairs in the description of low-lying states in atomic nuclei. Having available the precise details on these key collective pairs --…

Nuclear Theory · Physics 2020-08-19 Y. Lei , H. Jiang , S. Pittel

Quantitative estimates are derived, on the whole space, for the relative entropy between the joint law of random interacting particles and the tensorized law at the limiting systeme. The developed method combines the relative entropy method…

Probability · Mathematics 2024-01-18 Paul Nikolaev , David J. Prömel

We introduce a computational method to discover polymorphs in molecular crystals at finite temperature. The method is based on reproducing the crystallization process starting from the liquid and letting the system discover the relevant…

Chemical Physics · Physics 2020-04-10 Pablo M. Piaggi , Michele Parrinello

We report a numerical calculation of the total number of disordered jammed configurations $\Omega$ of $N$ repulsive, three-dimensional spheres in a fixed volume $V$. To make these calculations tractable, we increase the computational…

Statistical Mechanics · Physics 2016-01-29 Stefano Martiniani , K. Julian Schrenk , Jacob D. Stevenson , David J. Wales , Daan Frenkel

Most methods for estimating configurational entropy from molecular simulation data yield upper limits except for harmonic systems where they are exact. Problems arise at diffusive systems and the presence of conformational transitions.…

Chemical Physics · Physics 2019-10-22 Jürgen Schlitter , Matthias Massarczyk

For theoretical description of pseudospin systems with essential short-range and long-range interactions we use the method based on calculations of the free energy functional with taking into account the short-range interactions within the…

Statistical Mechanics · Physics 2019-05-21 R. R. Levitskii , S. I. Sorokov , O. R. Baran

We provide an efficient approximation for the exponential of a local operator in quantum spin systems using tensor-network representations of a cluster expansion. We benchmark this cluster tensor network operator (cluster TNO) for…

Strongly Correlated Electrons · Physics 2021-12-03 Bram Vanhecke , David Devoogdt , Frank Verstraete , Laurens Vanderstraeten

We calculate the configurational entropy of colloidal particles in a confined geometry interacting as hard disks using Monte Carlo integration method. In particular, we consider systems with three kinds of boundary conditions: hard,…

Soft Condensed Matter · Physics 2023-01-23 Duanduan Wan

The cluster variation - Pade` approximant method is a recently proposed tool, based on the extrapolation of low/high temperature results obtained with the cluster variation method, for the determination of critical parameters in Ising-like…

Statistical Mechanics · Physics 2009-10-31 Alessandro Pelizzola

Problems of probabilistic inference and decision making under uncertainty commonly involve continuous random variables. Often these are discretized to a few points, to simplify assessments and computations. An alternative approximation is…

Artificial Intelligence · Computer Science 2013-03-08 William B. Poland , Ross D. Shachter

We systematically extend the statement that the configurational entropy provides an alternative approach to studying gravitational stability of compact objects, carried out in the previous work of M. Gleiser and N. Jiang, Phys. Rev. D {\bf…

General Relativity and Quantum Cosmology · Physics 2023-03-20 P. S. Koliogiannis , G. A. Tsalis , C. P. Panos , Ch. C. Moustakidis

We describe a framework in which is possible to develop and implement algorithms for the approximation of invariant measures of dynamical systems with a given bound on the error of the approximation. Our approach is based on a general…

Dynamical Systems · Mathematics 2017-10-05 Stefano Galatolo , Isaia Nisoli

A simple third order compact finite element method is proposed for one-dimensional Sturm-Liouville boundary value problems. The key idea is based on the interpolation error estimate, which can be related to the source term. Thus, a simple…

Numerical Analysis · Mathematics 2021-08-17 Baiying Dong , Zhilin Li

For the generalized statistical mechanics based on the Tsallis entropy, a variational perturbation approximation method with the principle of minimal sensitivity is developed by calculating the generalized free energy up to the third order…

Statistical Mechanics · Physics 2007-05-23 Wen-Fa Lu

A systematic analysis of thermodynamic properties performed on Ce-base exemplary compounds allows to identify different types of behaviors as the system approaches the quantum critical region. They are recognized in the respective magnetic…

Strongly Correlated Electrons · Physics 2011-08-02 Julian G. Sereni

We propose a general framework for solving quantum state estimation problems using the minimum relative entropy criterion. A convex optimization approach allows us to decide the feasibility of the problem given the data and, whenever…

Quantum Physics · Physics 2013-01-29 Mattia Zorzi , Francesco Ticozzi , Augusto Ferrante

Variational methods are widely used for approximate posterior inference. However, their use is typically limited to families of distributions that enjoy particular conjugacy properties. To circumvent this limitation, we propose a family of…

Machine Learning · Computer Science 2012-06-22 Samuel Gershman , Matt Hoffman , David Blei

The success of the "Cluster Variation Method" (CVM) in reproducing quite accurately the free energies of Monte Carlo (MC) calculations on Ising models is explained in terms of identifying a cancellation of errors: We show that the CVM…

Materials Science · Physics 2009-10-31 Luiz G. Ferreira , C. Wolverton , Alex Zunger