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Density functional theory (DFT) provides a theoretical framework for efficient and fairly accurate calculations of the electronic structure of molecules and crystals. The main features of density functional theory are described and DFT…

Chemical Physics · Physics 2012-06-12 Hauke Paulsen , Alfred Xaver Trautwein

Colloidal particles that are confined to an interface effectively form a two-dimensional fluid. We examine the dynamics of such colloids when they are subject to a constant external force, which drives them in a particular direction over…

Soft Condensed Matter · Physics 2011-06-24 Andrew J. Archer , Alexandr Malijevsky

We derive and analyze the dynamic equations for polar liquid crystals in two spatial dimensions in the framework of classical dynamical density functional theory (DDFT). Translational density variations, polarization, and quadrupolar order…

Soft Condensed Matter · Physics 2014-01-28 Raphael Wittkowski , Hartmut Löwen , Helmut R. Brand

Density Functional Theory (DFT) is widely used for atomistic simulations. However, its reach stays limited due to several limitations such as lack of accurate exchange-correlation functional, requirement of costly O(N 3) diagonalization…

Quantum Physics · Physics 2026-05-18 Namrata Manglani , Samrit Kumar Maity , Shashank Sharma , Soham Phulare , Sanjay Wandhekar

Density Functional Theory (DFT) is one of the most widely used methods for "ab initio" calculations of the structure of atoms, molecules, crystals, surfaces, and their interactions. Unfortunately, the customary introduction to DFT is often…

Physics Education · Physics 2010-12-07 Nathan Argaman , Guy Makov

We consider the phase behavior of two-dimensional ($2D$)system of particles with an isotropic core-softened potential introduced in our previous publications. As one can expect from the qualitative consideration for the three dimensional…

Soft Condensed Matter · Physics 2015-06-18 D. E. Dudalov , Yu. D. Fomin , E. N. Tsiok , V. N. Ryzhov

We investigate theoretically the freezing behaviour of a two-dimensional (2D) system of hard discs on a one-dimensional (1D) external potential (typically called laser-induced freezing). As shown by earlier theoretical and numerical…

Soft Condensed Matter · Physics 2020-08-26 Alexander Kraft , Sabine H. L. Klapp

Using molecular dynamics simulation, we study structural and dynamical heterogeneities at melting in two-dimensional one-component systems with 36000 particles. Between crystal and liquid we find intermediate hexatic states, where the…

Statistical Mechanics · Physics 2010-04-07 Hayato Shiba , Akira Onuki , Takeaki Araki

We perform extensive simulations of $10^4$ Lennard-Jones particles to study the effect of particle size dispersity on the thermodynamic stability of two-dimensional solids. We find a novel phase diagram in the dispersity-density parameter…

Materials Science · Physics 2009-10-30 M. Reza Sadr-Lahijany , Purusattam Ray , H. Eugene Stanley

The glass transition of a hard sphere system is investigated within the framework of the density functional theory (DFT). Molecular dynamics (MD) simulations are performed to study dynamical behavior of the system on the one hand and to…

Soft Condensed Matter · Physics 2007-05-23 Kang Kim , Toyonori Munakata

Stochastic and mixed stochastic-deterministic density functional theory (DFT) are promising new approaches for the calculation of the equation-of-state and transport properties in materials under extreme conditions. In the intermediate warm…

Computational Physics · Physics 2023-09-27 Vidushi Sharma , Lee A. Collins , Alexander J. White

In this study, we formulate a density functional theory (DFT) for systems of labeled particles, considering a two-dimensional bead-spring lattice with a magnetic dipole on every bead as a model for ferrogels. On the one hand, DFT has been…

Soft Condensed Matter · Physics 2019-07-22 Segun Goh , René Wittmann , Andreas M. Menzel , Hartmut Löwen

We study the two-dimensional kinetic Ising model below its equilibrium critical temperature, subject to a square-wave oscillating external field. We focus on the multi-droplet regime where the metastable phase decays through nucleation and…

Statistical Mechanics · Physics 2009-10-31 G. Korniss , C. J. White , P. A. Rikvold , M. A. Novotny

Two-dimensional melting transitions for model colloids in presence of a one-dimensional external periodic potential are investigated using Monte Carlo simulation and Finite Size Scaling techniques. Here we explore a hard disk system with…

Statistical Mechanics · Physics 2009-11-13 Florian Bürzle , Peter Nielaba

The solution of the mean spherical approximation (MSA) integral equation for isotropic multicomponent dipolar hard sphere fluids without external fields is used to construct a density functional theory (DFT), which includes external fields,…

Statistical Mechanics · Physics 2015-05-28 I. Szalai , S. Dietrich

We present a derivation of the recently proposed eighth order phase field crystal model [Jaatinen et al., Phys. Rev. E 80, 031602 (2009)] for the crystallization of a solid from an undercooled melt. The model is used to study the planar…

Materials Science · Physics 2015-05-20 A. Jaatinen , T. Ala-Nissila

Our previous molecular dynamic simulation studies of simple two-dimensional (2D) systems \cite{matt_big} suggested that both geometrical defects (localized, large-amplitude deviations from hexagonal ordering) and topological defects…

Statistical Mechanics · Physics 2007-05-23 Yves Lansac , Matthew A. Glaser , Noel A. Clark

The Kosterlitz-Thouless and the Hexatic phase transitions are celebrated examples of dipole (vortex, dislocation) induced transitions in condensed matter physics. For very clear reasons, these important ``topological" transitions are…

Statistical Mechanics · Physics 2025-07-16 Itamar Procaccia , Tuhin Samanta

Dynamical density functional theory (DDFT) is a powerful variational framework to study the nonequilibrium properties of colloids by only considering a time-dependent one-body number density. Despite the large number of recent successes,…

Soft Condensed Matter · Physics 2021-01-13 René Wittmann , Hartmut Löwen , Joseph M. Brader

We study the zero-temperature phase diagram of two-dimensional helium-4 using neural quantum states. Our variational description allows us to address liquid and solid phases using the same functional form as well as exploring possible…

Statistical Mechanics · Physics 2025-06-19 David Linteau , Gabriel Pescia , Jannes Nys , Giuseppe Carleo , Markus Holzmann