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A semi-grand-canonical Monte Carlo algorithm is employed in conjunction with the bond fluctuation model to investigate the critical properties of an asymmetric binary (AB) polymer mixture. By applying the equal peak-weight criterion to the…

Condensed Matter · Physics 2009-10-22 M. Mueller , N. B. Wilding

We show that one can employ well-established numerical continuation methods to efficiently calculate the phase diagram for thermodynamic systems. In particular, this involves the determination of lines of phase coexistence related to first…

Soft Condensed Matter · Physics 2021-01-22 Max Philipp Holl , Andrew J. Archer , Uwe Thiele

Block copolymer melts self-assemble in the bulk into a variety of nanostructures, making them perfect candidates to template the position of nanoparticles. The morphological changes of block copolymers are studied in the presence of a…

Soft Condensed Matter · Physics 2019-10-31 Javier Diaz , Marco Pinna , Andrei V. Zvelindovsky , Ignacio Pagonabarraga

Recently topological states of matter have witnessed a new physical phenomenon where both edge modes and gapless bulk coexist at topological quantum criticality. The presence and absence of edge modes on a critical line can lead to an…

Strongly Correlated Electrons · Physics 2023-05-12 Ranjith R Kumar , Nilanjan Roy , Y R Kartik , S Rahul , Sujit Sarkar

We find a series of topological phase transitions of increasing order, beyond the more standard second-order phase transition in a one-dimensional topological superconductor. The jumps in the order of the transitions depend on the range of…

Statistical Mechanics · Physics 2018-04-04 P. Cats , A. Quelle , O. Viyuela , M. A. Martin-Delgado , C. Morais Smith

This paper studies a polymer chain in the vicinity of a linear interface separating two immiscible solvents. The polymer consists of random monomer types, while the interface carries random charges. Both the monomer types and the charges…

Probability · Mathematics 2015-06-05 Frank den Hollander , Alex A. Opoku

In this paper we study a two-dimensional directed self-avoiding walk model of a random copolymer in a random emulsion. The copolymer is a random concatenation of monomers of two types, $A$ and $B$, each occurring with density 1/2. The…

Probability · Mathematics 2009-11-13 Frank den Hollander , Nicolas Pétrélis

We analyze a (1+1)-dimension directed random walk model of a polymer dipped in a medium constituted by two immiscible solvents separated by a flat interface. The polymer chain is heterogeneous in the sense that a single monomer may…

Probability · Mathematics 2007-05-23 Erwin Bolthausen , Giambattista Giacomin

Phase separation of sequence-disordered liquid crystalline polymers, a promising class of technological and biological relevance, is studied by field theory, and thermodynamic mechanisms responsible for orientational ordering observed in…

Statistical Mechanics · Physics 2016-08-31 L. Gutman , E. I. Shakhnovich

When two types of side chains (A,B) are densely grafted to a (stiff) backbone and the resulting bottle-brush polymer is in a solution under poor solvent conditions, an incompatibility between A and B leads to microphase separation in the…

Soft Condensed Matter · Physics 2015-05-28 Igor Erukhimovich , Panagiotis E. Theodorakis , Wolfgang Paul , Kurt Binder

We propose and study a model of polymer chains in a bilayer. Each chain is confined in one of the layers and polymer bonds on first neighbor edges in different layers interact. We also define and comment results for a model with…

Statistical Mechanics · Physics 2015-06-05 Pablo Serra , Jürgen F. Stilck

Twist grain boundaries are widely observed in lamellar phases of block copolymers. A mesoscopic model of the copolymer is used to obtain stationary configurations that include a twist grain boundary, and to analyze their stability against…

Soft Condensed Matter · Physics 2008-04-15 Xusheng Zhang , Zhi-Feng Huang , Jorge Viñals

Conformational properties of a single flexible polyelectrolyte chain in a poor solvent are studied using constant temperature molecular dynamics simulation. The effects of counterions are explicitly taken in to account. Structural…

Statistical Mechanics · Physics 2012-12-04 Anoop Varghese , Satyavani Vemparala , R. Rajesh

When interfaces between ordered domains are ordered clusters, frustration disappears. A phase with mixed ordered structures emerges but no length scale can be associated to. We show that sum of densities of each structure plays the role of…

Statistical Mechanics · Physics 2010-05-13 Y. Boughaleb , M. Noureddine , R. Nassif

Homogeneous nucleation of a new phase near an Ising-like critical point of another phase transition is studied. A scaling analysis shows that the free energy barrier to nucleation contains a singular term with the same scaling as the order…

Statistical Mechanics · Physics 2009-11-07 Richard P. Sear

A phenomenological mean-field theory is used to investigate the properties of solvent-diluted di-block copolymers (BCP), in which the two BCP components (A and B) form a variety of phases that are diluted by a solvent (S). Using this…

Soft Condensed Matter · Physics 2014-04-22 Shai Cohen , David Andelman

Strongly correlated materials often undergo a Mott metal-insulator transition, which is tipically first-order, as a function of control parameters like pressure. Upon doping, rich phase diagrams with competing instabilities are found. Yet,…

Linked cluster expansions are generalized from an infinite to a finite volume. They are performed to 20th order in the expansion parameter to approach the critical region from the symmetric phase. A new criterion is proposed to distinguish…

High Energy Physics - Lattice · Physics 2009-10-28 H. Meyer-Ortmanns , T. Reisz

Biological polymers, such as intrinsically disordered proteins, play a central role in cellular biology, including mediating phase separation and controlling activity of biological condensates. The physical properties and functions of…

A copolymer is a chain of repetitive units (monomers) that are almost identical, but they differ in their degree of affinity for certain solvents. This difference leads to striking phenomena when the polymer fluctuates in a nonhomogeneous…

Probability · Mathematics 2010-11-11 Francesco Caravenna , Giambattista Giacomin
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