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Raman experiments on the spin-Peierls compound CuGeO$_3$ and the substituted (Cu$_{1- x}$,Zn$_x$)GeO$_3$ and Cu(Ge$_{1-x}$,Ga$_x$)O$_3$ compounds were performed in order to investigate the response of specific magnetic excitations of the…

Polarized inelastic light scattering experiments on Cu_(1-x)Zn_xGeO_3 (0<= x <= 0.045) single crystals show for x<>0 a new distinct mode at nearly half the energy of the singlet response below the spin-Peierls transition. The temperature,…

Strongly Correlated Electrons · Physics 2009-10-31 G. Els , G. S. Uhrig , P. Lemmens , H. Vonberg , P. H. M. van Loosdrecht , G. Guentherodt , O. Fujita , J. Akimitsu , G. Dhalenne , A. Revcolevschi

We have measured temperature dependence of low-frequency Raman spectra in CuGeO$_3$, and have observed the quasi-elastic scattering in the $(c,c)$ polarization above the spin-Peierls transition temperature. We attribute it to the…

We observed Raman scattering from magnon in frequency range from 10 to 65 cm-1 in BiFeO3 single crystals at cryogenic temperatures; the temperature dependence of the magnon frequency at 18.2 cm-1 approximates an S=5/2 Brillouin function up…

Materials Science · Physics 2008-01-28 Manoj K. Singh , Ram S. Katiyar , J. F. Scott

Neutron scattering measurements on a large single crystal of CuGeO$_3$ have been used to determine the temperature-dependence of the spin-Peierls energy gap. While the power law behavior of the intensity of structural superlattice peaks is…

Condensed Matter · Physics 2009-10-28 Michael C. Martin , G. Shirane , Y. Fujii , M. Nishi , O. Fujita , J. Akimitsu , M. Hase , K. Uchinokura

We have studied magnetic excitations in the dimerized spin-Peierls phase of CuGeO3, by high resolution inelastic neutron scattering. We measured the well-defined spin triplet dispersive mode which is gapped throughout the whole Brillouin…

Strongly Correlated Electrons · Physics 2009-10-31 M. Ain , J. E. Lorenzo , L. P. Regnault , G. Dhalenne , A. Revcolevschi , B. Hennion , Th. Jolicoeur

The magnetic moment induced by an external magnetic field of 5.8 T on the Co3+ ions in LaCoO3 has been measured by polarized neutron diffraction. Measurements were made at 100 K, near to the spin-state transition, at 1.5 K and at 285 K. The…

Strongly Correlated Electrons · Physics 2015-06-25 V. P. Plakhty , P. J. Brown , B. Grenier , S. V. Shiryaev , S. N. Barilo , S. V. Gavrilov , E. Ressouche

We investigated in detail the optical properties of several Cu(1-delta)Mg(delta)GeO3 (with delta=0,0.01), and CuGe(1-x)B(x)O3 with B=Si (x=0,0.007,0.05,0.1), and Al (x=0,0.01) single crystals, in the frequency range 20-32000 cm^-1. We…

Strongly Correlated Electrons · Physics 2009-10-31 A. Damascelli , D. van der Marel , G. Dhalenne , A. Revcolevschi

Polarized far-infrared transmittance spectra of CuGeO_3 single crystals were measured at different temperatures (6K < T < 300K). Two spectral lines, at 284.2 cm-1 in E||c polarization and at 311.7 cm-1 in E||b polarization, appear at the…

Strongly Correlated Electrons · Physics 2009-10-30 M. N. Popova , A. B. Sushkov , S. A. Golubchik , A. N. Vasil'ev , L. L. Leonyuk

Using Raman scattering we studied the effect of substitutions on 1D spin fluctuations in CuGeO_3 observed as a spinon continuum in frustration induced exchange scattering. For temperatures below the spin-Peierls transition (T_{SP}=14K) the…

Strongly Correlated Electrons · Physics 2016-08-31 M. Fischer , P. Lemmens , G. Güntherodt , M. Weiden , W. Richter , C. Geibel , F. Steglich

We report on the magnetic properties of the manganite Bi_{1-x}Ca_{x}MnO_3 (x=0.33) at low temperature. The analysis of the field expansion of the ac susceptibility and the observation of aging properties make clear that a spin glass phase…

Materials Science · Physics 2009-11-13 M. Giot , A. Pautrat , G. Andre , D. Saurel , M. Hervieu , J. Rodriguez-Carvajal

Transitions between the ground singlet state to the excited triplet state has been observed in CuGeO3 by means of submillimeter wave electron spin resonance. The strong absorption intensity shows the break down of the selection rule. The…

Strongly Correlated Electrons · Physics 2009-10-31 H. Nojiri , H. Ohta , S. Okubo , O. Fujita , J. Akimitsu , M. Motokawa

CuGeO$_3$ undergoes a transition from a spin-Peierls phase to an incommensurate phase at a critical field of $H_c\approx 12.5$ T. In the high-field phase a lattice of solitons forms, with both structural and magnetic components, and these…

Single crystals of the spin-gap system $\rm (VO)_2P_2O_7$ have been investigated by means of Raman scattering. At temperatures below T=75 K~$\approx 2\Delta_{01}({\bf k}=0)$, with $\Delta_{01}$ the singlet-triplet gap, a shoulder appears at…

Superconductivity · Physics 2009-10-31 M. Grove , P. Lemmens , G. Güntherodt , B. C. Sales , F. Büllesfeld , W. Assmus

A pressure and temperature dependent Raman study of the vibrational and spin dynamics in CuGeO3 is presented. A new low temperature, high pressure phase has been identified, and a pressure-temperature phase-diagram is proposed for CuGeO3.…

Strongly Correlated Electrons · Physics 2009-10-28 P. H. M. van Loosdrecht , J. Zeman , G. Martinez , G. Dhalenne , A. Revcolevschi , .

We present a theory for the spin-Peierls transition in CuGeO_3. We map the elementary excitations of the dimerized chain (solitons) on an effective Ising model. Inter-chain coupling (or phonons) then introduce a linear binding potential…

Condensed Matter · Physics 2009-10-30 Ralph Werner , Claudius Gros

We investigated the infrared reflectivity of several Mg- and Si-substituted CuGeO3 single crystals. The temperature dependent b-axis and c-axis optical response is reported. For T<Tsp we detected the activation of zone-boundary phonons…

Strongly Correlated Electrons · Physics 2009-10-30 A. Damascelli , D. van der Marel , F. Parmigiani , G. Dhalenne , A. Revcolevschi

Temperature ($2.3<T<40$\ K) and magnetic field ($0<B<17$\ T) dependent far infrared absorption spectroscopy on the spin-Peierls coumpound CuGeO$_3$\ has revealed several new absorption processes in both the dimerised and high field phase of…

Condensed Matter · Physics 2009-10-28 P. H. M. van Loosdrecht , S. Huant , G. Martinez , G. Dhalenne , A. Revcolevschi

We present the detailed inelastic neutron scattering measurements of the noncollinear antiferromagnet Mn$_3$Ge. Time-of-flight and triple-axis spectroscopy experiments were conducted at the temperature of 6~K, well below the high magnetic…

Strongly Correlated Electrons · Physics 2019-07-01 A. S. Sukhanov , M. S. Pavlovskii , Ph. Bourges , H. C. Walker , K. Manna , C. Felser , D. S. Inosov

We investigated the far- and mid-infrared reflectivity (20-6000 wavenumber) of several pure and doped CuGeO3 single crystals. The b-axis and c-axis optical response is presented for different temperatures between 4 K and 300 K. Moreover, a…

Strongly Correlated Electrons · Physics 2009-10-30 A. Damascelli , D. van der Marel , F. Parmigiani , G. Dhalenne , A. Revcolevschi
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