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The Kitaev candidate material Na$_2$Co$_2$TeO$_6$ is proposed to be proximate to a quantum spin liquid state but a suitable spin model and the nature of its ground states are still under debate. Our high-frequency/high-field electron spin…

Strongly Correlated Electrons · Physics 2025-09-08 Luca Bischof , Jan Arneth , Raju Kalaivanan , Raman Sankar , Kwang-Yong Choi , Rüdiger Klingeler

We report an inelastic light scattering study of single-crystalline NaCu$_2$O$_2$, a spin-chain compound known to exhibit a phase with helical magnetic order at low temperatures. Phonon excitations were studied as a function of temperature…

Strongly Correlated Electrons · Physics 2009-11-11 K. -Y. Choi , V. P. Gnezdilov , P. Lemmens , L. Capogna , M. R. Johnson , M. Sofin , A. Maljuk , M. Jansen , B. Keimer

Bulk magnetic measurements and inelastic neutron scattering were used to investigate the spin-singlet ground state and magnetic gap excitations in BaCuSi2O6, a quasi-2-dimensional antiferromagnet with a bilayer structure. The results are…

Condensed Matter · Physics 2009-10-28 Y. Sasago , K. Uchinokura , A. Zheludev , G. Shirane

Spin-phonon coupling, the interaction of spins with surrounding lattice is a key parameter to understand the underlying physics of multiferroics and engineer their magnetization dynamics. Elementary excitations in multiferroic materials are…

Materials Science · Physics 2020-11-05 Bommareddy Poojitha , Anjali Rathore , Ankit Kumar , Surajit Saha

We report magnetization and heat capacity measurements of single crystal samples of the spin gap compound Sr$_2$Cu(BO$_3$)$_2$. Low-field data show that the material has a singlet ground state comprising dimers with intradimer coupling J =…

Strongly Correlated Electrons · Physics 2011-12-08 Suchitra E. Sebastian , D. Yin , P. Tanedo , G. A. Jorge , N. Harrison , M. Jaime , Y. Mozharivskyj , G. Miller , J. Krzystek , S. A. Zvyagin , I. R. Fisher

A huge increase of thermal conductivity k is observed at the phase transition in stoichiometric NaV2O5. This anomaly decreases and gradually disappears with deviation from stoichiometry in Na(1-x}V2O5 (x = 0.01, 0.02, 0.03, and 0.04). This…

Strongly Correlated Electrons · Physics 2009-10-31 A. N. Vasil'ev , V. V. Pryadun , D. I. Khomskii , G. Dhalenne , A. Revcolevschi , M. Isobe , Y. Ueda

We present a model compound that forms a mixed-spin ferromagnetic chain. Our material design, based on the organic radicals, affords a verdazyl-based complex (p-Py-V)2[Mn(hfac)2]. The molecular orbital calculations of the compound indicate…

Strongly Correlated Electrons · Physics 2022-09-19 H. Yamaguchi , S. C. Furuya , S. Morota , S. Shimono , T. Kawakami , Y. Kusanose , Y. Shimura , K. Nakano , Y. Hosokoshi

We investigated the magnetotransport of InAs nanowires grown by selective area metal-organic vapor phase epitaxy. In the temperature range between 0.5 and 30 K reproducible fluctuations in the conductance upon variation of the magnetic…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 S. Estévez Hernández , M. Akabori , K. Sladek , Ch. Volk , S. Alagha , H. Hardtdegen , N. Demarina , D. Grützmacher , Th. Schäpers , M. G. Pala

Magnetic susceptibility and specific heat versus temperature measurements on polycrystalline samples of Sr3Cr2O8 and the isostructural, nonmagnetic compound Sr3V2O8 are reported. A Curie-Wiess fit to the high-temperature susceptibility data…

Strongly Correlated Electrons · Physics 2010-11-17 Yogesh Singh , D. C. Johnston

Using soft x-ray absorption spectroscopy and magnetic circular dichroism at the Co-$L_{2,3}$ edge we reveal that the spin state transition in LaCoO$_{3}$ can be well described by a low-spin ground state and a triply-degenerate high-spin…

Revealing the spin excitations of complex quantum magnets is key to developing a minimal model that explains the underlying magnetic correlations in the ground state. We investigate the low-energy magnons in $\alpha$-RuCl$_3$ by combining…

Strongly Correlated Electrons · Physics 2019-09-04 Ilkem Ozge Ozel , Carina A. Belvin , Edoardo Baldini , Itamar Kimchi , Seunghwan Do , Kwang-Yong Choi , Nuh Gedik

The phonon density of states (DOS) and magnetic excitation spectrum of polycrystalline BiFeO$_3$ were measured for temperatures $200 \leq T \leq 750\,$K, using inelastic neutron scattering (INS). Our results indicate that the magnetic…

Materials Science · Physics 2012-02-27 Olivier Delaire , Matthew B. Stone , Jie Ma , Ashfia Huq , Delphine Gout , Craig Brown , Kefeng Wang , Zhifeng Ren

Magnetic excitations and magnetic structure of EuRbFe$_4$As$_4$ were investigated by inelastic neutron scattering (INS), neutron diffraction, and random phase approximation (RPA) calculations. Below the superconducting transition…

Magnetic Raman scattering from a frustrated spin-1/2 Heisenberg-chain is considered with a focus on the uniform phase of the spin-Peierls compound CuGeO_3. The Raman intensity is analyzed in terms of a Loudon-Fleury scattering process using…

Strongly Correlated Electrons · Physics 2016-08-31 Wolfram Brenig

From low-temperature Synchrotron X-ray diffraction, a precise thermal characterization of octahedral distortions in single phase Ruddlesden-Popper Ca3Mn2O7 is performed. Highly sensitive close-steps temperature dependences of Mn-O-Mn bond…

Materials Science · Physics 2020-04-24 Pooja Sahlot , A. K. Sinha , A. M. Awasthi

We have used time-of-flight inelastic neutron scattering to measure the spin wave spectrum of the canonical half-doped manganite Pr$_{0.5}$Ca$_{0.5}$MnO$_{3}$, in its magnetic and orbitally ordered phase. The data, which cover multiple…

Strongly Correlated Electrons · Physics 2016-07-25 R. A. Ewings , T. G. Perring , O. Sikora , D. L. Abernathy , Y. Tomioka , Y. Tokura

A systematic electron spin resonance (ESR) investigation of the low temperature regime for the (ET)2SF5CF2SO3 system was performed in the frequency range of ~200-700 GHz, using backward wave oscillator sources, and at fields up to 25 T.…

We present two experiments that provide information on spin anisotropy and the magnetic structure of NaxCoO2. First, we report low-energy neutron inelastic scattering measurements of the zone-center magnetic excitations in the magnetically…

Strongly Correlated Electrons · Physics 2007-05-23 L. M. Helme , A. T. Boothroyd , R. Coldea , D. Prabhakaran , A. Stunault , G. J. McIntyre , N. Kernavanois

The structural properties of LaCoO3 were studied by means of high-resolution neutron powder diffraction in the temperature range 5<T<1000 K. Changes of the Co+3 spin states in this temperature interval are shown to affect not only the unit…

Strongly Correlated Electrons · Physics 2009-11-07 Paolo G. Radaelli , Sang-Wook Cheong

We have carried out inelastic neutron scattering experiments to study magnetic excitations in ordered double perovskite Ca$_2$FeReO$_6$. We found a well-defined magnon mode with a bandwidth of $\sim$50meV below the ferri-magnetic ordering…

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