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Polarized and unpolarized inelastic neutron scattering is used to study Haldane-gap excitations in the mixed-spin linear-chain antiferromagnet Nd2BaNiO5. The longitudinal mode, polarized along the direction of ordered moments, is observed…

Strongly Correlated Electrons · Physics 2009-10-31 S. Raymond , T. Yokoo , A. Zheludev , S. E. Nagler , A. Wildes , J. Akimitsu

Inelastic neutron scattering has been applied to the study of the spin dynamics of Cr-based antiferromagnetic octanuclear rings where a finite total spin of the ground state is obtained by substituting one Cr(III) ion (s = 3/2) with Zn (s =…

Quite a few low-dimensional magnets are quantum-disordered ``spin liquids'' with a characteristic gap in the magnetic excitation spectrum. Among these are antiferromagnetic chains of integer quantum spins. Their generic feature are…

Strongly Correlated Electrons · Physics 2009-11-11 A. Zheludev

We report inelastic neutron scattering experiments on single crystals of superconducting Ba0.67K0.33Fe2As2 (Tc = 38 K). In addition to confirming the resonance previously found in powder samples, we find that spin excitations in the normal…

Inelastic neutron scattering measurements were performed on the ferromagnetic chain system CsNiF_3 in the collinear antiferromagnetic ordered state below T_N = 2.67K. The measured spin wave dispersion was found to be in good agreement with…

Condensed Matter · Physics 2009-10-28 M. Baehr , M. Winkelmann , P. Vorderwisch , M. Steiner , C. Pich , F. Schwabl

We carried out inelastic neutron scattering experiments on a powdered sample of the antiferromagnetic (AFM) uniform spin-1/2 chain compound CuSb2O6.The magnetic excitations appear in the energy range of 1.8 to 13 meV at 2.5 K below the AFM…

Strongly Correlated Electrons · Physics 2026-04-20 Masashi Hasea , Minoru Soda , Takatsugu Masuda , Shinichi Itoh , Tetsuya Yokoo

We study the dynamic spin correlation function of a spin one antiferromagnetic chain with easy-plane single-ion anisotropy. We use exact diagonalization by the Lancz\H os method for chains of lengths up to N=16 spins. We show that a…

Condensed Matter · Physics 2009-10-22 O. Golinelli , Th. Jolicoeur , R. Lacaze

Inelastic neutron scattering experiments on the Haldane-gap quantum antiferromagnet NDMAP are performed in magnetic fields below and above the critical field Hc at which the gap closes. Quasi-elastic neutron scattering is found for H>Hc…

Strongly Correlated Electrons · Physics 2009-11-07 A. Zheludev , Z. Honda , Y. Chen , C. L. Broholm , K. Katsumata

Nuclear inelastic scattering (NIS) spectra were recorded for the spin-crossover complexes STP and ETP (STP = [Fe(1,1,1-trisf[N-(2-pyridylmethyl)-N-methylamino]methylg- ethane)](ClO4)2 and ETP =…

Inelastic neutron scattering experiments performed on a single crystal of the antiferromagnetic compound Ce$_{0.87}$La$_{0.13}$Ru$_{2}$Si$_{2}$ under applied pressures of up to 5 kbar are reported. A quantum critical point is reached at…

Strongly Correlated Electrons · Physics 2009-11-07 S. Raymond , L. P. Regnault , J. Flouquet , A. Wildes , P. Lejay

We have investigated the quasi-one dimensional Ni-chain compound PbMn$_2$Ni$_6$Te$_2$O$_{18}$ using theoretical DFT calculations, inelastic neutron scattering and optical spectroscopy in order to understand the nature of magnetic exchange…

We performed inelastic neutron scattering experiments on single crystal samples of a linear magnetoelectric material Mn$_{3}$Ta$_{2}$O$_{8}$, which exhibits a collinear antiferromagnetic order, to reveal the spin dynamics. Numerous modes…

Strongly Correlated Electrons · Physics 2025-04-08 Hodaka Kikuchi , SHunsuke Hasegawa , Shinichiro Asai , Tao Hong , Kenta Kimura , Tsuyoshi Kimura , Shinichi Itoh , Takatsugu Masuda

Neutron scattering is used to investigate the single-ion spin and orbital excitations below the Mott-Hubbard gap in CoO. Three excitations are reported at 0.870 $\pm$ 0.009 eV, 1.84 $\pm$ 0.03, and 2.30 $\pm$ 0.15 eV. These were…

Strongly Correlated Electrons · Physics 2015-06-17 R. A. Cowley , W. J. L. Buyers , C. Stock , Z. Yamani , C. Frost , J. W. Taylor , D. Prabhakaran

Single crystal inelastic neutron scattering is used to study spin wave excitations in the fully polarized state of the frustrated quantum ferro-antiferromagnet BaCdVO(PO$_4$)$_2$. The data analysis is based on a Heisenberg spin Hamiltonian…

Strongly Correlated Electrons · Physics 2021-04-07 V. K. Bhartiya , S. Hayashida , K. Yu. Povarov , Z. Yan , Y. Qiu , S. Raymond , A. Zheludev

The molecular coordination complex NiI$_2$(3,5-lut)$_4$ [where (3,5-lut) $=$ (3,5-lutidine) $=$ (C$_7$H$_9$N)] has been synthesized and characterized by several techniques including synchrotron X-ray diffraction, ESR, SQUID magnetometry,…

We report inelastic neutron scattering measurements of the spin dynamics in the layered hexagonal magnet 2H-AgNiO2 which has stacked triangular layers of antiferromagnetically-coupled Ni2+ spins (S=1) ordered in a collinear alternating…

Strongly Correlated Electrons · Physics 2009-03-25 E. M. Wheeler , R. Coldea , E. Wawrzynska , T. Sorgel , M. Jansen , M. M. Koza , J. Taylor , P. Adroguer , N. Shannon

Two quasi-1-dimensional S=1 quantum antiferromagnetic materials, PbNi2V2O8 and SrNi2V2O8, are studied by inelastic neutron scattering on powder samples. While magnetic interactions in the two systems are found to be very similar, subtle…

Strongly Correlated Electrons · Physics 2009-10-31 A. Zheludev , T. Masuda , I. Tsukada , Y. Uchiyama , K. Uchinokura , P. Boni , S. -H. Lee

Inelastic neutron scattering is used to identify single-particle and continuum spin excitations in the quasi-one-dimensional $S=1/2$ antiferromagnet \ba. In the data analysis, close attention is given to resolution effects. A gap in the…

Strongly Correlated Electrons · Physics 2007-05-23 A. Zheludev , M. Kenzelmann , S. Raymond , T. Masuda , K. Uchinokura , S. -H. Lee

Neutron spectroscopy measurements have been performed on single crystals of the antiferromagnetic van der Waals compound NiPS$_3$. Linear spin wave theory using a Heisenberg Hamiltonian with single-ion anisotropies has been applied to…

Strongly Correlated Electrons · Physics 2022-12-19 A. R. Wildes , J. R. Stewart , M. D. Le , R. A. Ewings , K. C. Rule , G. Deng , K. Anand

We performed inelastic neutron scattering (INS) experiments to measure spin dynamics on a polycrystalline sample of a spin tube candidate CsCrF$_{4}$. The compound exhibits a successive phase transition from a paramagnetic phase through an…

Other Condensed Matter · Physics 2023-05-17 Hodaka Kikuchi , Shinichiro Asai , Hirotaka Manaka , Masato Hagihala , Shinichi Itoh , Takatsugu Masuda