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A co-polycondensation reaction is discussed analytically and by Monte-Carlo simulations where two reactive units compete for reactions with an alternating third reactive unit, whereby irreversible reactions replace bonds which are able to…

Soft Condensed Matter · Physics 2021-05-26 Michael Lang , Frank Böhme

A popular concept which describes the structure of polymer interfaces by ``intrinsic profiles'' centered around a two dimensional surface, the ``local interface position'', is tested by extensive Monte Carlo simulations of interfaces…

Soft Condensed Matter · Physics 2009-10-31 A. Werner , F. Schmid , M. Mueller , K. Binder

The influence of monomer-monomer interactions on the scaling exponents and shape characteristics of a single polymer chain in a selective solvent is investigated using Langevin dynamics simulations. By systematically increasing the…

Soft Condensed Matter · Physics 2025-04-01 K. Haydukivska

We have evaluated conformational and orientational averages of binary interaction integrals for pairs of chains constituting atomistic representations of short polymer molecules. By considering A-A, B-B and A-B pairs, we relate these…

Chemical Physics · Physics 2009-05-29 Amirhossein Ahmadi , Juan J. Freire

We introduce a novel coarse-grained bead-spring model for flexible polymers to systematically examine the effects of an adjusted bonded potential on the formation and stability of structural macrostates in a thermal environment. The density…

Biological Physics · Physics 2019-02-11 Kai Qi , Benjamin Liewehr , Tomas Koci , Busara Pattanasiri , Matthew J. Williams , Michael Bachmann

Quantitative theory of interbilayer interactions is essential to interpret x-ray scattering data and to elucidate these interactions for biologically relevant systems. For this purpose Monte Carlo simulations have been performed to obtain…

Biological Physics · Physics 2009-10-31 Nikolai Gouliaev , John F. Nagle

The liquid crystalline model biomembrane system consisting of a stack of interacting membranes is studied by the newly developed Fourier Monte Carlo simulation technique. In comparison to perturbation theory, substantial quantitative…

Biological Physics · Physics 2007-05-23 Nikolai Gouliaev , John F. Nagle

We study a two-component reaction-diffusion system in which one of the reaction terms becomes singularly large. Assuming that the initial data are nonnegative and mutually segregated, we prove that the solution converges to that of the heat…

Analysis of PDEs · Mathematics 2025-06-12 Yuki Tsukamoto

A mean field rate theory description of the homo- and co-polymerization of $f$-functional molecules is developed, which contains the formation of short cyclic structures inside the network. The predictions of this model are compared with…

Soft Condensed Matter · Physics 2021-03-31 Michael Lang , Konrad Schwenke , Jens-Uwe Sommer

Solvent-free coarse grained models represent one of the most promising approaches for molecular simulations of mesoscopically large membranes. In these models, the size of the simulated membrane is limited by the slow relaxation time of…

Soft Condensed Matter · Physics 2009-11-13 Oded Farago

We present a Monte Carlo method to simulate asymmetric binary mixtures in the grand canonical ensemble. The method is used to study the colloid-polymer model of Asakura and Oosawa. We determine the phase diagram of the fluid-fluid unmixing…

Soft Condensed Matter · Physics 2007-05-23 R. L. C. Vink , J. Horbach

This paper reviews recent Monte Carlo simulation studies of the glassy behavior in thin polymer films. The simulations employ a version of the bond-fluctuation lattice model, in which the glass transition is driven by the competition…

Soft Condensed Matter · Physics 2007-05-23 C. Mischler , J. Baschnagel , K. Binder

We study polymer-polymer phase separation in a common good solvent by means of Monte Carlo simulations of the bond-fluctuation model. Below a critical, chain-length dependent concentration, no phase separation occurs. For higher…

Soft Condensed Matter · Physics 2009-11-11 Lei Guo , Erik Luijten

We present results of monomer-resolved Monte Carlo simulations for a system of amphiphilic dendrimers of second generation. Our investigations validate a coarse-grained level description based on the zero-density limit effective…

Soft Condensed Matter · Physics 2012-09-27 Dominic A. Lenz , Bianca M. Mladek , Christos N. Likos , Gerhard Kahl , Ronald Blaak

We investigate the phase behaviour of random copolymers melts via large scale Monte Carlo simulations. We observe macrophase separation into A and B--rich phases as predicted by mean field theory only for systems with a very large…

Soft Condensed Matter · Physics 2009-11-07 J. Houdayer , M. Mueller

To describe the full spectrum of surface fluctuations of the interface between phase-separated colloid-polymer mixtures from low scattering vector q (classical capillary wave theory) to high q (bulk-like fluctuations), one must take account…

Soft Condensed Matter · Physics 2009-11-13 Edgar M. Blokhuis , Joris Kuipers , Richard Vink

Understanding the phase behaviour of mixtures continues to pose challenges, even for systems that might be considered "simple". Here we consider a very simple mixture of two colloidal and one non-adsorbing polymer species which can be…

A three-dimensional atomistic Kinetic Monte Carlo model was developed and used to study the interaction between mobile solutes and a migrating interface. While the model was developed with a simplified energetic and topological description,…

Materials Science · Physics 2015-06-16 Aulia Tegar Wicaksono , Chad W. Sinclair , Matthias Militzer

Monte Carlo simulations of the Asakura-Oosawa (AO) model for colloid-polymer mixtures confined between two parallel repulsive structureless walls are presented and analyzed in the light of current theories on capillary condensation and…

Soft Condensed Matter · Physics 2009-11-13 Andres De Virgiliis , Richard L. C. Vink , Jürgen Horbach , Kurt Binder

We investigate by means of a number of different dynamical Monte Carlo simulation methods the self-assembly of equilibrium polymers in dilute, semidilute and concentrated solutions under good-solvent conditions. In our simulations, both…

Statistical Mechanics · Physics 2009-10-31 J. P. Wittmer , P. van der Schoot , A. Milchev , J. -L. Barrat