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We develop an empirical potential for silicon which represents a considerable improvement over existing models in describing local bonding for bulk defects and disordered phases. The model consists of two- and three-body interactions with…

Materials Science · Physics 2016-08-31 Joao F. Justo , Martin Z. Bazant , Efthimios Kaxiras , V. V. Bulatov , Sidney Yip

Interatomic potentials approximate the potential energy of atoms as a function of their coordinates. Their main application is the effective simulation of many-atom systems. Here, we review empirical interatomic potentials designed to…

Materials Science · Physics 2022-11-11 Martin H. Muser , Sergey V. Sukhomlinov , Lars Pastewka

The electronic structure and dielectric properties of the diamond, body centered cubic diamond (bc8), and hexagonal diamond (lonsdaleite) phases of carbon are computed using density functional theory and many-body perturbation theory with…

Materials Science · Physics 2022-03-14 Kushal Ramakrishna , Jan Vorberger

A continuum model of crystalline solid equilibrium is presented in which the underlying periodic lattice structure is taken explicitly into account. This model also allows for both point and line defects in the bulk of the lattice and at…

Materials Science · Physics 2009-10-31 Paolo Cermelli , Shaun Sellers

A key starting assumption in many classical interatomic potential models for materials is a site energy decomposition of the potential energy surface into contributions that only depend on a small neighbourhood. Under a natural stability…

Mathematical Physics · Physics 2020-09-10 Jack Thomas

To reproduce the diamond structure of silicon, double lattice (DL) potential constructed from two interatomic potentials for face centered cubic (fcc) lattice, is proposed for molecular dynamics (MD) simulations. For the validity test of MD…

Materials Science · Physics 2020-08-12 Hui Zhang , Chongyang Wei , Zhongwu Liu , Xichun Zhong , Dongling Jiao , Wanqi Qiu , Hongya Yu

In Part I of this two part series, we presented a multi-neighbor dependent contact model for adhesive elastic-plastic particles built upon the method of dimensionality reduction that is valid for the elastic and fully-plastic contact…

Soft Condensed Matter · Physics 2023-09-15 William Zunker , Ken Kamrin

We propose a simple scheme to construct composition-dependent interatomic potentials for multicomponent systems that when superposed onto the potentials for the pure elements can reproduce not only the heat of mixing of the solid solution…

Materials Science · Physics 2012-01-31 B. Sadigh , P. Erhart , A. Stukowski , A. Caro

Choice of appropriate force field is one of the main concerns of any atomistic simulation that needs to be seriously considered in order to yield reliable results. Since, investigations on mechanical behavior of materials at micro/nanoscale…

Computational Physics · Physics 2016-07-12 Seyed Moein Rassoulinejad-Mousavi , Yijin Mao , Yuwen Zhang

An analytical framework is proposed to describe the elasticity, viscosity and fragility of metallic glasses in relation to their atomic-level structure and the effective interatomic interaction. The bottom-up approach starts with forming an…

Soft Condensed Matter · Physics 2016-08-15 Alexandra E. Lagogianni , Johannes Krausser , Zach Evenson , Konrad Samwer , A Zaccone

Understanding the size- and shape-dependent properties of platinum nanoparticles is critical for enabling the design of nanoparticle-based applications with optimal and potentially tunable functionality. Toward this goal, we evaluated nine…

Mesoscale and Nanoscale Physics · Physics 2021-08-05 Ingrid M. Padilla Espinosa , Tevis D. B. Jacobs , Ashlie Martini

We use numerical simulations and an effective-medium theory to study the rigidity percolation transition of the honeycomb and diamond lattices when weak bond-bending forces are included. We use a rotationally invariant bond-bending…

Disordered Systems and Neural Networks · Physics 2016-04-08 Danilo B. Liarte , O. Stenull , Xiaoming Mao , T. C. Lubensky

We use molecular simulation to construct equilibrium phase diagrams for two recently introduced model materials with isotropic, soft-repulsive pair interactions designed to favor diamond and simple cubic lattice ground states, respectively,…

Materials Science · Physics 2013-10-15 Avni Jain , Jeffrey R. Errington , Thomas M. Truskett

Using molecular dynamics simulations we study the thermodynamic behavior of a single-component covalent material described by the recently proposed Environment-Dependent Interatomic Potential (EDIP). The parameterization of EDIP for silicon…

Materials Science · Physics 2009-11-07 P. Keblinski , M. Z. Bazant , R. K. Dash , M. M. Treacy

The dependence of macroscopic detonation properties of a two-dimensional diatomic (AB) molecular system on the fundamental properties of the molecule were investigated. This includes examining the detonation velocity, reaction zone…

Simple models for spherical particles with a soft shell have been shown to self-assemble into numerous crystal phases and even quasicrystals. However, most of these models rely on a simple pairwise interaction, which is usually a valid…

Soft Condensed Matter · Physics 2020-09-03 Emanuele Boattini , Nina Bezem , Sudeep N. Punnathanam , Frank Smallenburg , Laura Filion

We report density-functional based molecular dynamics simulations, that show that, with increasing pressure, liquid carbon undergoes a gradual transformation from a liquid with local three-fold coordination to a 'diamond-like' liquid. We…

Other Condensed Matter · Physics 2009-11-10 Luca M. Ghiringhelli , Jan H. Los , Evert Jan Meijer , A. Fasolino , Daan Frenkel

Understanding the atomic-scale structure and dynamics of amorphous oxide surfaces is essential for interpreting their chemical reactivity, mechanical stability, and interfacial behavior, yet direct experimental characterization remains…

Materials Science · Physics 2026-05-08 Zheng Yu , Jiayan Xu , Abhirup Patra , Sharan Shetty , Detlef Hohl , Roberto Car

The approximate representation of a quantum solid as an equivalent composite semi-classical solid is considered for insulating materials. The composite is comprised of point ions moving on a potential energy surface. In the classical bulk…

Materials Science · Physics 2007-05-23 Aditi Mallik , Keith Runge , James W. Dufty , Hai-Ping Cheng

We study theoretically the equilibrium structure, as well as the response under external load, of characteristic carbon-based materials. The materials considered include diamond, amorphous carbon (a-C), ``amorphous diamond'' and…

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